TY - JOUR
AU - Qin, Yuling
AU - Wang, Hongliang
AU - Ruan, Hao
AU - Feng, Maoqi
AU - Yang, Bin
PY - 2018
M3 - Original Research
TI - High Catalytic Efficiency of Lignin Depolymerization over Low Pd-Zeolite Y Loading at Mild Temperature
JO - Frontiers in Energy Research
UR - https://www.frontiersin.org/articles/10.3389/fenrg.2018.00002
VL - 6
SN - 2296-598X
N2 - This article reported a novel low-temperature process for aromatics production through lignin depolymerization catalyzed by 0.1 wt% Pd-zeolite Y catalyst prepared by a facile method. Under the same reactive condition, the as-prepared Pd-zeolite Y catalysts exhibited much higher catalytic efficiency than zeolite Y or commercial Pd/Al2O3–zeolite composites. The selectivity of the Pd-zeolite Y toward lignin depolymerization was also much higher than the other commercial zeolite-based catalysts. With the presence of hydrogen, aromatics were the predominant products with high yields of phenols and dimers (over 99%). The as-obtained aromatics can be promising feedstock for production of fuels or chemicals for various applications. Results revealed that the Pd-zeolite Y catalyst is a highly active catalyst for the cleavage of lignin interlinkages, especially the C–O–C bonds by hydrogenolysis.
ER -