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<front>
<journal-meta>
<journal-id journal-id-type="publisher-id">Front. Mater.</journal-id>
<journal-title>Frontiers in Materials</journal-title>
<abbrev-journal-title abbrev-type="pubmed">Front. Mater.</abbrev-journal-title>
<issn pub-type="epub">2296-8016</issn>
<publisher>
<publisher-name>Frontiers Media S.A.</publisher-name>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="publisher-id">790987</article-id>
<article-id pub-id-type="doi">10.3389/fmats.2021.790987</article-id>
<article-categories>
<subj-group subj-group-type="heading">
<subject>Materials</subject>
<subj-group>
<subject>Original Research</subject>
</subj-group>
</subj-group>
</article-categories>
<title-group>
<article-title>Coiling-Up Space Metasurface for High-Efficient and Wide-angle Acoustic Wavefront Steering</article-title>
<alt-title alt-title-type="left-running-head">Chen et&#x20;al.</alt-title>
<alt-title alt-title-type="right-running-head">Coiling-Up Space Metasurface</alt-title>
</title-group>
<contrib-group>
<contrib contrib-type="author">
<name>
<surname>Chen</surname>
<given-names>Shuang</given-names>
</name>
<uri xlink:href="https://loop.frontiersin.org/people/1517624/overview"/>
</contrib>
<contrib contrib-type="author" corresp="yes">
<name>
<surname>Fan</surname>
<given-names>Yuancheng</given-names>
</name>
<xref ref-type="corresp" rid="c001">&#x2a;</xref>
<uri xlink:href="https://loop.frontiersin.org/people/278581/overview"/>
</contrib>
<contrib contrib-type="author">
<name>
<surname>Yang</surname>
<given-names>Fan</given-names>
</name>
</contrib>
<contrib contrib-type="author">
<name>
<surname>Sun</surname>
<given-names>Kangyao</given-names>
</name>
<uri xlink:href="https://loop.frontiersin.org/people/1536608/overview"/>
</contrib>
<contrib contrib-type="author">
<name>
<surname>Fu</surname>
<given-names>Quanhong</given-names>
</name>
<uri xlink:href="https://loop.frontiersin.org/people/1139532/overview"/>
</contrib>
<contrib contrib-type="author">
<name>
<surname>Zheng</surname>
<given-names>Jianbang</given-names>
</name>
</contrib>
<contrib contrib-type="author" corresp="yes">
<name>
<surname>Zhang</surname>
<given-names>Fuli</given-names>
</name>
<xref ref-type="corresp" rid="c001">&#x2a;</xref>
<uri xlink:href="https://loop.frontiersin.org/people/755057/overview"/>
</contrib>
</contrib-group>
<aff>Key Laboratory of Light Field Manipulation and Information Acquisition, Ministry of Industry and Information Technology and School of Physical Science and Technology, Northwestern Polytechnical University, <addr-line>Xi&#x2019;an</addr-line>, <country>China</country>
</aff>
<author-notes>
<fn fn-type="edited-by">
<p>
<bold>Edited by:</bold> <ext-link ext-link-type="uri" xlink:href="https://loop.frontiersin.org/people/1160861/overview">Ke Chen</ext-link>, Nanjing University, China</p>
</fn>
<fn fn-type="edited-by">
<p>
<bold>Reviewed by:</bold> <ext-link ext-link-type="uri" xlink:href="https://loop.frontiersin.org/people/1254812/overview">Xumin Ding</ext-link>, Harbin Institute of Technology, China</p>
<p>
<ext-link ext-link-type="uri" xlink:href="https://loop.frontiersin.org/people/1257191/overview">Cheng Zhang</ext-link>, Wuhan University of Technology, China</p>
<p>
<ext-link ext-link-type="uri" xlink:href="https://loop.frontiersin.org/people/1245536/overview">Yadong Xu</ext-link>, Soochow University, China</p>
</fn>
<corresp id="c001">&#x2a;Correspondence: Yuancheng Fan, <email>phyfan@nwpu.edu.cn</email>; Fuli Zhang, <email>fuli.zhang@nwpu.edu.cn</email>
</corresp>
<fn fn-type="other">
<p>This article was submitted to Metamaterials, a section of the journal Frontiers in Materials</p>
</fn>
</author-notes>
<pub-date pub-type="epub">
<day>07</day>
<month>12</month>
<year>2021</year>
</pub-date>
<pub-date pub-type="collection">
<year>2021</year>
</pub-date>
<volume>8</volume>
<elocation-id>790987</elocation-id>
<history>
<date date-type="received">
<day>07</day>
<month>10</month>
<year>2021</year>
</date>
<date date-type="accepted">
<day>09</day>
<month>11</month>
<year>2021</year>
</date>
</history>
<permissions>
<copyright-statement>Copyright &#xa9; 2021 Chen, Fan, Yang, Sun, Fu, Zheng and Zhang.</copyright-statement>
<copyright-year>2021</copyright-year>
<copyright-holder>Chen, Fan, Yang, Sun, Fu, Zheng and Zhang</copyright-holder>
<license xlink:href="http://creativecommons.org/licenses/by/4.0/">
<p>This is an open-access article distributed under the terms of the Creative Commons Attribution License (CC BY). The use, distribution or reproduction in other forums is permitted, provided the original author(s) and the copyright owner(s) are credited and that the original publication in this journal is cited, in accordance with accepted academic practice. No use, distribution or reproduction is permitted which does not comply with these&#x20;terms.</p>
</license>
</permissions>
<abstract>
<p>The recent advent of acoustic metasurface displays tremendous potential with their unique and flexible capabilities of wavefront manipulations. In this paper, we propose an acoustic metagrating made of binary coiling-up space structures to coherently control the acoustic wavefront steering. The acoustic wave steering is based on the in-plane coherent modulation of waves in different diffraction channels. The acoustic metagrating structure with a subwavelength thickness is realized with 3D printed two coiling-up space metaunits. By adjusting structural parameters of the metaunits, the &#x2212;1st-order diffraction mode can be retained, and the rest of the diffraction orders are eliminated as much as possible through destructive interference, forming a high-efficiency anomalous reflection in the scattering field. The anomalous reflection performance of the designed metagrating is achieved over a wide range of incident angles with high efficiency.</p>
</abstract>
<kwd-group>
<kwd>metasurface (MS)</kwd>
<kwd>acoustic metamaterial (AMM)</kwd>
<kwd>beam steering (BS)</kwd>
<kwd>wavefront control</kwd>
<kwd>retroreflected beam</kwd>
<kwd>anomalous reflection</kwd>
</kwd-group>
</article-meta>
</front>
<body>
<sec id="s1">
<title>Introduction</title>
<p>The recently appeared acoustic metasurfaces, as the two-dimensional (2D) version of metamaterials with subwavelength thicknesses, have shown outstanding capabilities in manipulating acoustic waves compared to natural materials (<xref ref-type="bibr" rid="B24">Li et&#x20;al., 2013</xref>; <xref ref-type="bibr" rid="B54">Zhao et&#x20;al., 2013</xref>; <xref ref-type="bibr" rid="B34">Ma et&#x20;al., 2014</xref>; <xref ref-type="bibr" rid="B48">Xie et&#x20;al., 2014</xref>; <xref ref-type="bibr" rid="B46">Xie et&#x20;al., 2017</xref>; <xref ref-type="bibr" rid="B1">Assouar et&#x20;al., 2018</xref>; <xref ref-type="bibr" rid="B58">Zhu et&#x20;al., 2018</xref>; <xref ref-type="bibr" rid="B3">Chen et&#x20;al., 2019</xref>; <xref ref-type="bibr" rid="B32">Long et&#x20;al., 2020</xref>; <xref ref-type="bibr" rid="B53">Zhang et&#x20;al., 2020</xref>). Metasurfaces originally have been introduced and progressed for manipulating electromagnetic waves (<xref ref-type="bibr" rid="B50">Yu et&#x20;al., 2011</xref>; <xref ref-type="bibr" rid="B49">Yang et&#x20;al., 2019</xref>; <xref ref-type="bibr" rid="B15">Guan et&#x20;al., 2020a</xref>; <xref ref-type="bibr" rid="B5">Ding et&#x20;al., 2020</xref>; <xref ref-type="bibr" rid="B51">Yuan et&#x20;al., 2020</xref>; <xref ref-type="bibr" rid="B8">Fan et&#x20;al., 2021</xref>) and then are expanded to steer the acoustic waves given that both of the them obey the generalized Snell&#x2019;s law. Basically, the uniqueness of metasurfaces rested with their ability of easily adjusting the phase and/or amplitude so as to fully control the wave fields. At present, acoustic metasurfaces with various profiles have been proposed for different functions and applications, including (but not limited to) Helmholtz-resonator-like (<xref ref-type="bibr" rid="B23">Li et&#x20;al., 2015</xref>; <xref ref-type="bibr" rid="B45">Wang et&#x20;al., 2016</xref>; <xref ref-type="bibr" rid="B52">Zhang et&#x20;al., 2021</xref>), membrane-type (<xref ref-type="bibr" rid="B34">Ma et&#x20;al., 2014</xref>; <xref ref-type="bibr" rid="B44">Tang et&#x20;al., 2019</xref>; <xref ref-type="bibr" rid="B31">Liu et&#x20;al., 2020</xref>), and coiling-up space (<xref ref-type="bibr" rid="B48">Xie et&#x20;al., 2014</xref>; <xref ref-type="bibr" rid="B26">Liang and Li, 2012</xref>; <xref ref-type="bibr" rid="B36">N. Almeida et&#x20;al., 2021</xref>). By properly designing the inner structures of metasurfaces, a great deal of fascinating features has been realized, such as anomalous reflection and refraction (<xref ref-type="bibr" rid="B28">Liu et&#x20;al., 2017</xref>; <xref ref-type="bibr" rid="B20">Li et&#x20;al., 2018</xref>; <xref ref-type="bibr" rid="B27">Liu and Jiang, 2018</xref>; <xref ref-type="bibr" rid="B37">Qian et&#x20;al., 2019</xref>; <xref ref-type="bibr" rid="B42">Su and Liu, 2020</xref>), asymmetric propagation (<xref ref-type="bibr" rid="B39">Shen et&#x20;al., 2016</xref>; <xref ref-type="bibr" rid="B25">Li et&#x20;al., 2017</xref>; <xref ref-type="bibr" rid="B41">Song et&#x20;al., 2019</xref>), orbital angular momentum (<xref ref-type="bibr" rid="B40">Shi et&#x20;al., 2019</xref>; <xref ref-type="bibr" rid="B13">Gao et&#x20;al., 2021</xref>; <xref ref-type="bibr" rid="B16">Hou et&#x20;al., 2021</xref>), near-perfect absorption (<xref ref-type="bibr" rid="B57">Zhu et&#x20;al., 2019</xref>; <xref ref-type="bibr" rid="B18">Kumar and Lee, 2020</xref>; <xref ref-type="bibr" rid="B6">Donda et&#x20;al., 2021</xref>; <xref ref-type="bibr" rid="B29">Liu et&#x20;al., 2021a</xref>), beam focusing (<xref ref-type="bibr" rid="B33">Ma et&#x20;al., 2018</xref>; <xref ref-type="bibr" rid="B30">Liu et&#x20;al., 2021b</xref>; <xref ref-type="bibr" rid="B47">Xie and Hou, 2021</xref>), self-bending beams (<xref ref-type="bibr" rid="B22">Li and Assouar, 2015</xref>), acoustic cloaking (<xref ref-type="bibr" rid="B17">Jin et&#x20;al., 2019</xref>; <xref ref-type="bibr" rid="B19">Li et&#x20;al., 2019</xref>; <xref ref-type="bibr" rid="B55">Zhao et&#x20;al., 2019</xref>; <xref ref-type="bibr" rid="B7">Fan et&#x20;al., 2020</xref>; <xref ref-type="bibr" rid="B56">Zhou et&#x20;al., 2021</xref>), and convolution operation and addition operation (<xref ref-type="bibr" rid="B2">Cao et&#x20;al., 2021</xref>).</p>
<p>Most of the demonstrated metasurfaces for anomalous reflection based on generalized Snell&#x2019;s law requires the arrangement of multi-metaunits with gradient indexes to provide additional phases of the scattered waves. Furthermore, the phase-gradient metasurface shows poor power efficiency due to mismatched wave impedances, because it cannot direct all incident energy to the required direction and eliminate the undesired scattered waves (<xref ref-type="bibr" rid="B35">Mohammadi Estakhri and Al&#xf9;, 2016</xref>; <xref ref-type="bibr" rid="B4">D&#xed;az-Rubio and Tretyakov, 2017</xref>). In addition, complex structural metaunits lead to unavoidable viscosity loss and non-negligible coupling effect between adjacent metaunits, and both of them will influence the efficiency of wavefront manipulation (<xref ref-type="bibr" rid="B43">Tang et&#x20;al., 2021</xref>). Therefore, tremendous research studies have been devoted to achieving high-efficiency anomalous reflection. Retroreflector is a device that can reflect electromagnetic waves or acoustic waves back to the incident direction. Shen et&#x20;al. proposed an acoustic retroreflector on the basis of conventional gradient-index metasurfaces without parasitic diffraction (<xref ref-type="bibr" rid="B38">Shen et&#x20;al., 2018</xref>). D&#xed;az-Rubio et&#x20;al. presented a new synthesis method that introduces nonlocal response or local and nonsymmetric response into reflection and refraction, respectively. This method overcomes the radical limitations of traditional designs, permits complete control of the acoustic energy flow, and achieves perfect anomalous reflection and refraction (<xref ref-type="bibr" rid="B4">D&#xed;az-Rubio and Tretyakov, 2017</xref>). Fu et&#x20;al. investigated theoretically and experimentally phase gradient metagratings (PGMs), which can completely reverse the anomalous transmission and reflection through higher-order diffraction by changing the integer parity of the PGM design (<xref ref-type="bibr" rid="B11">Fu et&#x20;al., 2019a</xref>). Li et&#x20;al. induced self-induced surface waves into acoustic metasurfaces to meet the local power conservation requirements and cultivated an approach to design bianisotropic metasurfaces for arbitrary beam splitting and anomalous reflection with theoretically power efficiency of 100% (<xref ref-type="bibr" rid="B21">Li et&#x20;al., 2020</xref>). However, these studies are proposed with complex theories and designed by metaunits with full phase range that make the designs difficulty to realize. Therefore, a new metasurface, i.e.,&#x20;metagrating, has been proposed to steer the acoustic wavefront with simpler methodology (<xref ref-type="bibr" rid="B10">Fu et&#x20;al., 2019b</xref>; <xref ref-type="bibr" rid="B12">Fu et&#x20;al., 2020a</xref>; <xref ref-type="bibr" rid="B9">Fu et&#x20;al., 2020b</xref>). Guan et&#x20;al. utilized metagrating to achieve helicity-switching and helicity-preserving performances in electromagnetic field (<xref ref-type="bibr" rid="B14">Guan et&#x20;al., 2020b</xref>). Fu et&#x20;al. reported a simple metagrating to achieve multifunctional reflection in acoustic field, which provides an alternative way for the manipulation of acoustic waves with high efficiency (<xref ref-type="bibr" rid="B46">Xie et&#x20;al., 2017</xref>). However, this study is not yet verified in experiments.</p>
<p>In this paper, we propose an acoustic metagrating on the basis of the in-plane coherent modulation of acoustic waves in different diffraction channels, which does not need to be based on the generalized Snell&#x2019;s law. The metagrating is made of binary coiling-up space metaunits to coherently control the wavefront steering. In our study, two 3D printed metaunits whose reflected waves satisfy the coherent condition are periodically arranged to form a metagrating that can realize high-efficiency anomalous reflection of acoustic waves. The validity of the wavefront manipulation method is proved in simulations and experiments. At last, the wide-angle characteristic of the designed metagrating is demonstrated in a range of 40&#xb0; with high efficiency.</p>
</sec>
<sec sec-type="materials|methods" id="s2">
<title>Materials and Methods</title>
<p>Because the propagation of acoustic waves follows the Huygens-Fresnel principle, the effect of acoustic diffraction can be easily understood. As shown in <xref ref-type="fig" rid="F1">Figure&#x20;1A</xref>, the acoustic waves with an incident angle <inline-formula id="inf1">
<mml:math id="m1">
<mml:mi>&#x3b1;</mml:mi>
</mml:math>
</inline-formula> incident on the surface of a grating. The grating constant is <italic>d</italic>. When the incident wavelength <inline-formula id="inf2">
<mml:math id="m2">
<mml:mrow>
<mml:msub>
<mml:mi>&#x3bb;</mml:mi>
<mml:mn>0</mml:mn>
</mml:msub>
</mml:mrow>
</mml:math>
</inline-formula> is sufficiently short compared to the grating constant <italic>d</italic>, one or more diffraction modes could be motivated with a non-specular diffraction angle. Therefore, we can adjust <italic>d</italic> to remain one of the reflection diffraction modes and eliminated as much as possible by destructive interference, so as to realize anomalous reflection. This structure with optional diffraction modes is called metagrating, which combines the diffraction ability of the acoustic grating with the phase control capacity of the metasurface. The concept of metagrating renders a valid platform to realize the control of the acoustic wavefront. When a single-frequency acoustic wave travels in the same medium, the length difference of different transmission paths will cause phase difference between them. According to the two reflection paths in <xref ref-type="fig" rid="F1">Figure&#x20;1A</xref>, the path difference can be calculated by the geometric analysis. When the value is an integer of the wavelength, constructive interference occurs, that is, it satisfies<disp-formula id="e1">
<mml:math id="m3">
<mml:mrow>
<mml:mi>K</mml:mi>
<mml:msub>
<mml:mi>&#x3bb;</mml:mi>
<mml:mn>0</mml:mn>
</mml:msub>
<mml:mo>&#x3d;</mml:mo>
<mml:mi>d</mml:mi>
<mml:mrow>
<mml:mo>(</mml:mo>
<mml:mrow>
<mml:mi>sin</mml:mi>
<mml:mo>&#x2061;</mml:mo>
<mml:msub>
<mml:mi>&#x3b2;</mml:mi>
<mml:mi>K</mml:mi>
</mml:msub>
<mml:mo>&#x2212;</mml:mo>
<mml:mi>sin</mml:mi>
<mml:mo>&#x2061;</mml:mo>
<mml:mi>&#x3b1;</mml:mi>
</mml:mrow>
<mml:mo>)</mml:mo>
</mml:mrow>
</mml:mrow>
</mml:math>
<label>(1)</label>
</disp-formula>where <italic>K</italic>&#x20;&#x3d; 0, &#xb1;1, &#xb1;2, &#x2026;, &#x3bb;<sub>0</sub> is the wavelength, and <inline-formula id="inf3">
<mml:math id="m4">
<mml:mrow>
<mml:msub>
<mml:mi>&#x3b2;</mml:mi>
<mml:mi>K</mml:mi>
</mml:msub>
</mml:mrow>
</mml:math>
</inline-formula> is the reflected angle of diffraction order <italic>K</italic>. When the grating constant <italic>d</italic> satisfies <xref ref-type="disp-formula" rid="e1">Eq. 1</xref>, diffractions of different orders will occur in the acoustic field due to constructive interference. When <italic>K</italic> is 0, it is the normal specular reflection of 0th order. Metagrating is an artifical structure designed by the grating theory, which is made of metaunits instead of the traditional materials with different indexes. To obtain anomalous reflection based on acoustic metagrating, it is necessary to use two artificial metaunits in one grating period to eliminate the extra diffraction orders by means of destructive interference. Here, the &#x2212;1st anomalous reflection is desired in our study. To make sure of the reflected acoustic waves without 2nd-order or higher-order diffraction components, the grating constant <italic>d</italic> and incident angle <inline-formula id="inf4">
<mml:math id="m5">
<mml:mi>&#x3b1;</mml:mi>
</mml:math>
</inline-formula>should satisfy<disp-formula id="e2">
<mml:math id="m6">
<mml:mrow>
<mml:mn>2</mml:mn>
<mml:msub>
<mml:mi>&#x3bb;</mml:mi>
<mml:mn>0</mml:mn>
</mml:msub>
<mml:mo>&#x3e;</mml:mo>
<mml:mi>d</mml:mi>
<mml:mrow>
<mml:mo>(</mml:mo>
<mml:mrow>
<mml:mn>1</mml:mn>
<mml:mo>&#x2b;</mml:mo>
<mml:mrow>
<mml:mo>&#x7c;</mml:mo>
<mml:mrow>
<mml:mi>sin</mml:mi>
<mml:mo>&#x2061;</mml:mo>
<mml:mi>&#x3b1;</mml:mi>
</mml:mrow>
<mml:mo>&#x7c;</mml:mo>
</mml:mrow>
</mml:mrow>
<mml:mo>)</mml:mo>
</mml:mrow>
</mml:mrow>
</mml:math>
<label>(2)</label>
</disp-formula>
</p>
<fig id="F1" position="float">
<label>FIGURE 1</label>
<caption>
<p>
<bold>(A)</bold> The geometric paths of two parallel acoustic beams. <bold>(B)</bold> The schematic of a binary metagrating for coherent modulation of acoustic waves.</p>
</caption>
<graphic xlink:href="fmats-08-790987-g001.tif"/>
</fig>
<p>In this work, we hope to obtain the anomalous reflection with a &#x2212;1st-order diffraction, so the designed metagrating should eliminate the 0th order and &#x2b;1st-order diffraction. When <inline-formula id="inf5">
<mml:math id="m7">
<mml:mrow>
<mml:mi>&#x3b1;</mml:mi>
<mml:mo>&#x2260;</mml:mo>
<mml:msup>
<mml:mrow>
<mml:mn>90</mml:mn>
</mml:mrow>
<mml:mi>o</mml:mi>
</mml:msup>
</mml:mrow>
</mml:math>
</inline-formula>, the essential condition for grating without &#x2b;1st-order diffraction given by<disp-formula id="e3">
<mml:math id="m8">
<mml:mrow>
<mml:msub>
<mml:mi>&#x3bb;</mml:mi>
<mml:mn>0</mml:mn>
</mml:msub>
<mml:mo>&#x3e;</mml:mo>
<mml:mi>d</mml:mi>
<mml:mrow>
<mml:mo>(</mml:mo>
<mml:mrow>
<mml:mn>1</mml:mn>
<mml:mo>&#x2212;</mml:mo>
<mml:mrow>
<mml:mo>&#x7c;</mml:mo>
<mml:mrow>
<mml:mi>sin</mml:mi>
<mml:mo>&#x2061;</mml:mo>
<mml:mi>&#x3b1;</mml:mi>
</mml:mrow>
<mml:mo>&#x7c;</mml:mo>
</mml:mrow>
</mml:mrow>
<mml:mo>)</mml:mo>
</mml:mrow>
</mml:mrow>
</mml:math>
<label>(3)</label>
</disp-formula>Therefore, the anomalous reflection can be achieved by eliminating the 0th-order diffraction, as shown in <xref ref-type="fig" rid="F1">Figure&#x20;1B</xref>. In this case, only two metaunits with phase difference of <inline-formula id="inf6">
<mml:math id="m9">
<mml:mi>&#x3c0;</mml:mi>
</mml:math>
</inline-formula> for constructive interference are needed in a grating period. As a result, the 0th-order reflection is eliminated, and only the &#x2212;1st-order diffraction is remained.</p>
<p>The designed metagrating includes two coiling-up space metaunits, as shown in <xref ref-type="fig" rid="F2">Figure&#x20;2A</xref>. Each metaunit is designed with width of <italic>m</italic>&#x20;&#x3d; 5&#xa0;cm, height of <italic>p</italic>&#x20;&#x3d; 6&#xa0;cm, and wall thickness of <italic>w</italic>&#x20;&#x3d; 4&#xa0;mm. By adjusting the length of the branches in the metaunits, the propagation path of acoustic waves will be changed and the reflected phase will be modulated accordingly. The length of branches of unit A is <italic>l</italic>
<sub>
<italic>1</italic>
</sub> &#x3d; 3.18&#xa0;cm, and parametric sweep of the length of branches in unit B is performed so that the reflected phase difference of the two metaunits is <inline-formula id="inf7">
<mml:math id="m10">
<mml:mi>&#x3c0;</mml:mi>
</mml:math>
</inline-formula> to eliminate the 0th-order acoustic wave as much as possible. In this case, the acoustic grating constant is <italic>d</italic>&#x20;&#x3d; 10&#xa0;cm. When the wavelength<inline-formula id="inf8">
<mml:math id="m11">
<mml:mrow>
<mml:msub>
<mml:mi>&#x3bb;</mml:mi>
<mml:mn>0</mml:mn>
</mml:msub>
</mml:mrow>
</mml:math>
</inline-formula>is slightly larger than the acoustic grating constant, with any incident angle <inline-formula id="inf9">
<mml:math id="m12">
<mml:mi>&#x3b1;</mml:mi>
</mml:math>
</inline-formula>, both (<xref ref-type="disp-formula" rid="e2">2</xref>) and (<xref ref-type="disp-formula" rid="e3">3</xref>) are all satisfied, which means that the acoustic waves are coherently controlled in different diffraction channels and higher-order diffraction modes are eliminated in the acoustic fields.</p>
<fig id="F2" position="float">
<label>FIGURE 2</label>
<caption>
<p>
<bold>(A)</bold> The inner structures of the binary coiling-up space metaunits. <bold>(B)</bold> The reflection phase difference between unit A and unit B varying with <italic>l</italic>
<sub>
<italic>2</italic>
</sub>. <bold>(C)</bold> The normalized coefficients of each diffraction order in the reflection fields with difference <italic>l</italic>
<sub>2</sub>, where the dotted lines represent the &#x2212;1st orders and the solid lines represents the 0th orders. <bold>(D)</bold> Phase curves (green and blue) and phase difference curves (orange) of unit A and unit B when the selected optimal structure <italic>l</italic>
<sub>
<italic>2</italic>
</sub> &#x3d; 2.89&#xa0;cm.</p>
</caption>
<graphic xlink:href="fmats-08-790987-g002.tif"/>
</fig>
<p>The COMSOL Multiphysics software is used to perform the numerical of the distribution of the acoustic fields. The speed of acoustic waves and mass density of air are <italic>c</italic>
<sub>
<italic>0</italic>
</sub> &#x3d; 343&#xa0;m/s and <italic>&#x3c1;</italic>
<sub>
<italic>0</italic>
</sub> &#x3d; 1.21&#xa0;kg/m<sup>3</sup>, respectively, the incident angle <inline-formula id="inf10">
<mml:math id="m13">
<mml:mi>&#x3b1;</mml:mi>
</mml:math>
</inline-formula>is 45&#xb0;, and the amplitude of the incident plane wave is 1&#xa0;Pa. According to the diffraction equation, the &#x2212;1st diffraction angle is <inline-formula id="inf11">
<mml:math id="m14">
<mml:mrow>
<mml:msub>
<mml:mi>&#x3b3;</mml:mi>
<mml:mn>1</mml:mn>
</mml:msub>
<mml:mo>&#x3d;</mml:mo>
<mml:mi>arcsin</mml:mi>
<mml:mrow>
<mml:mo>(</mml:mo>
<mml:mrow>
<mml:mi>sin</mml:mi>
<mml:mo>&#x2061;</mml:mo>
<mml:mi>&#x3b1;</mml:mi>
<mml:mo>&#x2212;</mml:mo>
<mml:mi>&#x3bb;</mml:mi>
<mml:mo>/</mml:mo>
<mml:mi>d</mml:mi>
</mml:mrow>
<mml:mo>)</mml:mo>
</mml:mrow>
</mml:mrow>
</mml:math>
</inline-formula>. The phase difference between unit A and unit B is shown in <xref ref-type="fig" rid="F2">Figure&#x20;2B</xref>; when <italic>l</italic>
<sub>
<italic>2</italic>
</sub> &#x3d; 2.85, 2.87, and 2.89&#xa0;cm, there are two frequency points where the phase difference is <inline-formula id="inf12">
<mml:math id="m15">
<mml:mi>&#x3c0;</mml:mi>
</mml:math>
</inline-formula>, and at <italic>l</italic>
<sub>
<italic>2</italic>
</sub> &#x3d; 2.91&#xa0;cm, one frequency point of the phase difference is close to <inline-formula id="inf13">
<mml:math id="m16">
<mml:mi>&#x3c0;</mml:mi>
</mml:math>
</inline-formula>. These frequencies are generally around 2,500&#x2013;2,600&#xa0;Hz. <xref ref-type="fig" rid="F2">Figure&#x20;2C</xref> shows the normalized diffraction coefficients of diffraction modes. It can be seen that, for different values of <italic>l</italic>
<sub>2</sub> of unit B, the normalized diffraction coefficients of the 0th-order and &#x2212;1st-order diffractions of the unit B are different. For <italic>l</italic>
<sub>
<italic>2</italic>
</sub> &#x3d; 2.85, 2.87, and 2.89&#xa0;cm, the 0th-order diffraction curve has two minimum frequency points, and the distance between the two minimum points gradually decreases with the increase of <italic>l</italic>
<sub>
<italic>2</italic>
</sub>. At the same time, there is a maximum frequency point between the two minimum values, and the normalized diffraction coefficients of 0th order at this point gradually decreases with the increase of <italic>l</italic>
<sub>
<italic>2</italic>
</sub>. When <italic>l</italic>
<sub>
<italic>2</italic>
</sub> increases to 2.91&#xa0;cm, there is only one minimum frequency point for 0th-order diffraction. It is in good agreement with the phase difference curves of the two metaunits in <xref ref-type="fig" rid="F2">Figure&#x20;2B</xref>, that is, the closer the phase difference is to<inline-formula id="inf14">
<mml:math id="m17">
<mml:mi>&#x3c0;</mml:mi>
</mml:math>
</inline-formula>, the smaller proportion of 0th order in the reflected fields. It also proves that the 0th-order diffraction in the reflected fields shows destructive interference due to the phase adjustment of the two metaunits. Meanwhile, this study also provides a strong proof of the validity of diffraction-based acoustic metagrating in wavefront control.</p>
<p>According to the discussions above, the 0th diffraction angle is 45&#xb0; because of specular reflection and the &#x2212;1st diffraction angle is <inline-formula id="inf15">
<mml:math id="m18">
<mml:mrow>
<mml:msub>
<mml:mi>&#x3b3;</mml:mi>
<mml:mn>1</mml:mn>
</mml:msub>
<mml:mo>&#x3d;</mml:mo>
<mml:mi>arcsin</mml:mi>
<mml:mrow>
<mml:mo>(</mml:mo>
<mml:mrow>
<mml:mi>sin</mml:mi>
<mml:mo>&#x2061;</mml:mo>
<mml:mi>&#x3b1;</mml:mi>
<mml:mo>&#x2212;</mml:mo>
<mml:mi>&#x3bb;</mml:mi>
<mml:mo>/</mml:mo>
<mml:mi>d</mml:mi>
</mml:mrow>
<mml:mo>)</mml:mo>
</mml:mrow>
</mml:mrow>
</mml:math>
</inline-formula>according to the diffraction equation. Therefore, the normalized diffraction coefficients can be obtained by the normalization of integrals of far-field acoustic intensity around the diffraction angles. Under the consideration of the high efficiency of &#x2212;1st-order diffraction, we choose <italic>l</italic>
<sub>
<italic>2</italic>
</sub> &#x3d; 2.89&#xa0;cm and the workting frequency is <italic>f</italic>
<sub>2</sub> &#x3d; 2,590&#xa0;Hz where the theoretical diffraction coefficient of anomalous reflection is 0.97. As shown in <xref ref-type="fig" rid="F2">Figure&#x20;2D</xref>, the green and the blue curves represent the reflection phase of unit A and unit B, respectively, and the orange curve is the phase difference curve of the two. It is obvious that the phase difference curves of the two metaunits are much smoother than respective reflection phase curves, and anomalous reflection can also be achieved in a certain frequency bandwidth, although the theoretical efficiency is less than&#x20;100%.</p>
<p>
<xref ref-type="fig" rid="F3">Figure&#x20;3</xref> shows the acoustic pressure distributions of incident waves and reflected waves at <italic>f</italic>
<sub>1</sub> &#x3d; 2,890&#xa0;Hz and <italic>f</italic>
<sub>2</sub> &#x3d; 2,590&#xa0;Hz. After comparison, it can be clearly seen that, when the incident angle is 45&#xb0;, the 0th-order diffraction plays a dominant role at <italic>f</italic>
<sub>1</sub>, and the propagation of acoustic waves is specular reflection with a reflection angle <inline-formula id="inf16">
<mml:math id="m19">
<mml:mrow>
<mml:msub>
<mml:mi>&#x3b2;</mml:mi>
<mml:mn>1</mml:mn>
</mml:msub>
</mml:mrow>
</mml:math>
</inline-formula> of 45&#xb0;. At <italic>f</italic>
<sub>2</sub>, the reflected acoustic waves are also plane waves, but the propagation direction is negative, coexisting with the incident acoustic wave on the same side of the interface normal. According to the acoustic pressure fields, the diffraction angle can be estimated to be about &#x2212;38&#xb0;, which is consistent with the diffraction angle calculated by the diffraction equation.</p>
<fig id="F3" position="float">
<label>FIGURE 3</label>
<caption>
<p>
<bold>(A)</bold> Incident acoustic fields with plane wave. <bold>(B)</bold> Reflected pressure fields at non-working frequency <italic>f</italic>
<sub>1</sub> &#x3d; 2,890&#xa0;Hz. <bold>(C)</bold> Reflected pressure fields at working frequency <italic>f</italic>
<sub>2</sub> &#x3d; 2,590&#xa0;Hz.</p>
</caption>
<graphic xlink:href="fmats-08-790987-g003.tif"/>
</fig>
</sec>
<sec sec-type="results" id="s3">
<title>Results</title>
<p>In simulation, the designed binary metagrating is used to achieve high-efficiency anomalous reflections. To further verify the wavefront manipulation capability of the designed metagrating, we prepare the model using 3D printing technology, and the printing material is polylactic acid. A scanning stage is used to perform the measurement, as shown in <xref ref-type="fig" rid="F4">Figure&#x20;4A</xref>. A 2D waveguide is made of two paralleled plexiglass plates (1.2&#xa0;&#xd7; 2.2&#xa0;m<sup>2</sup>), and absorbing sponges are installed around the waveguide closely to minimize the echo and environmental noise. To form a plane wave in the waveguide, a sine signal is generated by a computer and transmitted to an amplifier by a digital collector that converts the digital signal into an acoustic signal. A loudspeaker array is arranged on the top of the waveguide that is motivated by the amplifier. The acoustic pressure in the waveguide is measured by two microphones, one for detection and one for reference. Then, the acoustic signal is achieved and transmitted back to the computer by the collector through different channels.</p>
<fig id="F4" position="float">
<label>FIGURE 4</label>
<caption>
<p>
<bold>(A)</bold> Schematic diagram of experimental waveguide system. The dashed line box in the figure represents the measurement area where a single microphone is used to scan and measure acoustic pressure. The insert is the picture of the coiling-up space metaunits. <bold>(B)</bold> Total pressure fields after the plane acoustic wave passing through the sample. <bold>(C)</bold> Total pressure fields of plane acoustic wave passing through hard plane boundary.</p>
</caption>
<graphic xlink:href="fmats-08-790987-g004.tif"/>
</fig>
<p>When the incident angle <inline-formula id="inf17">
<mml:math id="m20">
<mml:mi>&#x3b1;</mml:mi>
</mml:math>
</inline-formula> is 45&#xb0;, the 3D printed metaunits are arranged periodically in the waveguide periodically. Because of the platform design, the loudspeaker array can only propagate acoustic waves along the long axis of the waveguide. We place the sample at an angle of 45&#xb0;, which is equivalent to an incident angle of 45&#xb0;. Microphone is used to scan the acoustic pressure value at multiple points and obtain the fields distribution in the area of the blue dashed line box. For comparison, we measured the total pressure fields after the plane acoustic waves incident into the metagrating and hard boundary plane, respectively. It is clear that there is a great difference between the two. When the reflective interface is hard boundary plane, the reflection angle is the same as the incident angle at 45&#xb0;, and the incident waves and reflected waves interfere to form a standing wave field, as shown in <xref ref-type="fig" rid="F4">Figure&#x20;4C</xref>. <xref ref-type="fig" rid="F4">Figure&#x20;4B</xref> shows the total pressure fields when the reflective interface is a designed model. The pressure field is almost a plane wave along the horizontal direction, which is formed by the interference of the &#x2212;1st-order diffraction and the incident acoustic&#x20;waves.</p>
<p>As illustrated in all these simulations and experiments, the metagrating made of coiling-up space metaunits can modulate the reflection behavior of the objects effectively. It indicates that the metagrating provide a feasible means to realize wavefront control. The most outstanding feature of the metagrating is that each grating period contains only two metaunits for coherent modulation of waves, and it simplifies the process of realizing anomalous reflection greatly. Compared with acoustic metasurface with reflected phases from 0 to 2<inline-formula id="inf18">
<mml:math id="m21">
<mml:mi>&#x3c0;</mml:mi>
</mml:math>
</inline-formula> based on generalized Snell&#x2019;s law, metagrating with only two reflected phases of 0 and <inline-formula id="inf19">
<mml:math id="m22">
<mml:mi>&#x3c0;</mml:mi>
</mml:math>
</inline-formula> is easier to obtain in experiment.</p>
</sec>
<sec sec-type="discussion" id="s4">
<title>Discussion</title>
<p>Because metagrating is proposed on the basis of the coherent modulation of waves, the anomalous reflection performances of the designed metagrating with different incident angles are also studied in simulations. According to the diffraction equation of metagrating, the incident angle range for metagrating with &#x2212;1st-order diffraction and without 1st-order diffraction is <inline-formula id="inf20">
<mml:math id="m23">
<mml:mrow>
<mml:mtext>&#x3b1;</mml:mtext>
<mml:mo>&#x3e;</mml:mo>
<mml:mn>18.6</mml:mn>
<mml:mo>&#xb0;</mml:mo>
</mml:mrow>
</mml:math>
</inline-formula> when the working frequency is 2,590&#xa0;Hz and the grating constant is 10&#xa0;cm. The normalized &#x2212;1st-order diffraction coefficients of the metgrating with varying incident angles are shown in <xref ref-type="fig" rid="F5">Figure&#x20;5A</xref>. Over the range from <inline-formula id="inf21">
<mml:math id="m24">
<mml:mrow>
<mml:mn>23</mml:mn>
<mml:mo>&#xb0;</mml:mo>
</mml:mrow>
</mml:math>
</inline-formula> to <inline-formula id="inf22">
<mml:math id="m25">
<mml:mrow>
<mml:mn>61</mml:mn>
<mml:mo>&#xb0;</mml:mo>
</mml:mrow>
</mml:math>
</inline-formula>, the normalized diffraction coefficients are larger than 0.85, where the phase difference between the binary metaunits approaches to <inline-formula id="inf23">
<mml:math id="m26">
<mml:mtext>&#x3c0;</mml:mtext>
</mml:math>
</inline-formula>. It means that high-efficiency anomalous reflection is achieved over a wide range of incident angle of <inline-formula id="inf24">
<mml:math id="m27">
<mml:mrow>
<mml:mn>38</mml:mn>
<mml:mo>&#xb0;</mml:mo>
</mml:mrow>
</mml:math>
</inline-formula>. The simulation results satisfy the predicted range of incident angles for the occurrence of &#x2212;1st-order diffraction. However, under the incident angles that approach to <inline-formula id="inf25">
<mml:math id="m28">
<mml:mrow>
<mml:mn>45</mml:mn>
<mml:mo>&#xb0;</mml:mo>
</mml:mrow>
</mml:math>
</inline-formula>, the efficiency of anomalous reflection do not reach the desired value of 1 because of partial destructive interference of the 0th diffractions of the binary metaunits.</p>
<fig id="F5" position="float">
<label>FIGURE 5</label>
<caption>
<p>
<bold>(A)</bold> Normalized &#x2212;1st-order diffraction coefficients and phase difference between the binary metaunits at 2,590&#xa0;Hz under different incident angles. The gray area represents the region of the value larger than 0.85. <bold>(B</bold>&#x2013;<bold>D)</bold> Incident acoustic fields under incident angles of <inline-formula id="inf26">
<mml:math id="m29">
<mml:mrow>
<mml:mn>23</mml:mn>
<mml:mo>&#xb0;</mml:mo>
</mml:mrow>
</mml:math>
</inline-formula>, <inline-formula id="inf27">
<mml:math id="m30">
<mml:mrow>
<mml:mn>40</mml:mn>
<mml:mo>&#xb0;</mml:mo>
</mml:mrow>
</mml:math>
</inline-formula>, and <inline-formula id="inf28">
<mml:math id="m31">
<mml:mrow>
<mml:mn>61</mml:mn>
<mml:mo>&#xb0;</mml:mo>
</mml:mrow>
</mml:math>
</inline-formula>. <bold>(E</bold>&#x2013;<bold>G)</bold> Reflected acoustic fields under incident angles of <inline-formula id="inf29">
<mml:math id="m32">
<mml:mrow>
<mml:mn>23</mml:mn>
<mml:mo>&#xb0;</mml:mo>
</mml:mrow>
</mml:math>
</inline-formula>, <inline-formula id="inf30">
<mml:math id="m33">
<mml:mrow>
<mml:mn>40</mml:mn>
<mml:mo>&#xb0;</mml:mo>
</mml:mrow>
</mml:math>
</inline-formula>, and <inline-formula id="inf31">
<mml:math id="m34">
<mml:mrow>
<mml:mn>61</mml:mn>
<mml:mo>&#xb0;</mml:mo>
</mml:mrow>
</mml:math>
</inline-formula>.</p>
</caption>
<graphic xlink:href="fmats-08-790987-g005.tif"/>
</fig>
<p>Here, we demonstrate the anomalous reflection performance under incident angles of <inline-formula id="inf32">
<mml:math id="m35">
<mml:mrow>
<mml:mn>23</mml:mn>
<mml:mo>&#xb0;</mml:mo>
</mml:mrow>
</mml:math>
</inline-formula>, <inline-formula id="inf33">
<mml:math id="m36">
<mml:mrow>
<mml:mn>40</mml:mn>
<mml:mo>&#xb0;</mml:mo>
</mml:mrow>
</mml:math>
</inline-formula> and <inline-formula id="inf34">
<mml:math id="m37">
<mml:mrow>
<mml:mn>61</mml:mn>
<mml:mo>&#xb0;</mml:mo>
</mml:mrow>
</mml:math>
</inline-formula>, where the normalized &#x2212;1st-order diffraction coefficients are 0.85, 0.99, and 0.85, respectively. The incident acoustic fields are shown in <xref ref-type="fig" rid="F5">Figures 5B&#x2013;D</xref>, and the corresponding reflected acoustic fields are shown in <xref ref-type="fig" rid="F5">Figures 5E&#x2013;G</xref>. It can be seen that obvious anomalous reflections are acquired under the three incident angles. Therefore, the wide-angle performance of the designing metagrating is verified in simulations with high efficiency.</p>
</sec>
<sec sec-type="conclusion" id="s5">
<title>Conclusion</title>
<p>In summary, we proposed a kind reflective acoustic metasurface on the basis of the coherent control of acoustic wave for wide-angle acoustic wavefront control. By coherently modulating the reflected waves in different&#x20;diffraction channels, the high-efficiency anomalous reflection is obtain over a wide range of incident angles with high efficiency. The major idea is to utilize the binary coiling-up space metaunits for the in-plane destructive interference of extra diffraction orders in an acoustic grating period and only remain one needed diffraction order. The feasibility has been verified both in simulations and experiments. Compared with the previous wavefront control method based on the generalized Snell&#x2019;s law, the mechanism of coherent modulation of waves needs lower requirements on the number and phase control capability of metaunits and is valid in wide range of incident angles. This control method renders a feasible way for future research on the interaction between acoustic artificial microstructures and acoustic waves. In addition, to extend this method to a wideband, tunable acoustic metagrating is considered for the control of acoustic wavefront.</p>
</sec>
</body>
<back>
<sec id="s6">
<title>Data Availability Statement</title>
<p>The original contributions presented in the study are&#x20;included in the article/Supplementary Material; further&#x20;inquiries can be directed to the corresponding authors.</p>
</sec>
<sec id="s7">
<title>Author Contributions</title>
<p>YF and FZ conceived the idea and guided the research. FY and SC designed the metasurface. SC, FY, and KS prepared the samples, characterized the samples, and prepared the draft. All authors discussed the results and commented on the paper.</p>
</sec>
<sec id="s8">
<title>Funding</title>
<p>The authors would like to acknowledge financial support&#x20;from National Natural Science Foundation of China (NSFC) (grants nos. 61771402, 12074314, and 11674266); NPU AoXiang New Star program; Science, Technology and Innovation Commission of Shenzhen Municipality (JCYJ20170817162221169); Shaanxi Province Postdoctoral Science Foundation (no. 2018BSHEDZZ64); and Natural Science Basic Research Plan in Shaanxi&#x20;Province of China (nos. 2018JM6024 and 2020JM-145).</p>
</sec>
<sec sec-type="COI-statement" id="s9">
<title>Conflict of Interest</title>
<p>The authors declare that the research was conducted in the absence of any commercial or financial relationships that could be construed as a potential conflict of interest.</p>
</sec>
<sec sec-type="disclaimer" id="s10">
<title>Publisher&#x2019;s Note</title>
<p>All claims expressed in this article are solely those of the authors and do not necessarily represent those of their affiliated organizations or those of the publisher, the editors, and the reviewers. Any product that may be evaluated in this article, or claim that may be made by its manufacturer, is not guaranteed or endorsed by the publisher.</p>
</sec>
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