AUTHOR=Wiss Thierry , Konings Rudy J. M. , Staicu Dragos , Benedetti Alessandro , Colle Jean-Yves , Rondinella Vincenzo V. , Maugeri Emilio , Talip Zeynep , Janssen Arne , Dieste Oliver , Cognini Luana , De Bona Emanuele , Baldinozzi Gianguido , Guéneau Christine TITLE=Impact of alpha-damage and helium production on the heat capacity of actinide oxides JOURNAL=Frontiers in Nuclear Engineering VOLUME=Volume 4 - 2025 YEAR=2025 URL=https://www.frontiersin.org/journals/nuclear-engineering/articles/10.3389/fnuen.2025.1495360 DOI=10.3389/fnuen.2025.1495360 ISSN=2813-3412 ABSTRACT=The heat capacity of alpha-damaged uranium, plutonium, and americium mixed dioxide (Uu, Puv, Amw)O2±x samples was measured during thermal annealing. The excess of heat released was assessed and the recovery stages associated with various defects described by integrating results from transmission electron microscopy, helium desorption spectroscopy, thermal diffusivity, and XRD annealing studies. It is shown that different defect-annealing stages could be singled out. It could also be evidenced that the excess of energy stored in defects tends to saturate after rather low damage levels, but that, with increasing radiogenic helium production, another contribution of stored energy appears which can be attributed to the formation of He-defect complexes that cannot be annihilated until higher temperatures are reached.