Abstract
In this work, we present validation test results of fully coupled neutronics and thermal-hydraulics models of the Molten Salt Reactor Experiment (MSRE) against experimental data of the zero power pump transients and the natural circulation tests at low power. To capture the strong coupling between neutronics and thermal-hydraulics due to fuel circulation, and to account for the delayed neutron precursor (DNP) distribution, the porous media thermal-hydraulics solver Pronghorn was fully coupled to the spatial neutron dynamics code Griffin, which solves the neutron diffusion equation, and to the 0-D point kinetics solver Squirrel, using a 2-D homogenized representation of the MSRE. The validation test results show very good agreement with experimental data for both point kinetics and spatial dynamics simulations, capturing the strong feedback effect and DNP losses in the MSRE. The 0-D code Squirrel accurately predicted the time-dependent behavior in the MSRE given the steady-state spatial dynamics solution of Griffin.
1 Introduction
The Molten Salt Reactor Experiment (MSRE) was conducted in the 1960s at Oak Ridge National Laboratory. It provided important experimental experience and data on the operation of molten-salt reactors (MSRs) with liquid flowing fuel (). The MSRE fuel was dissolved in liquid salt, which flowed through the core, simultaneously generating and extracting heat. The flowing salt distinguishes MSRs from other reactor designs. In such reactors, the fluid dynamics and neutronics are strongly coupled through a large negative temperature feedback due to salt expansion and Doppler broadening ().
The strong thermal feedback and the redistribution of the delayed neutron source in the core () require a different treatment compared to other advanced reactor designs (). The flowing fuel distinguishes MSRs from solid fuel reactors, and modeling the behavior of MSRs necessitates a tightly coupled multiphysics simulation that accounts for fuel flow, thermal feedback, and the shifting of the delayed neutron source due to advection of the delayed neutron precursors (DNPs). Even though the delayed neutron fraction is small, the change in the effective reactivity reserve needs to be accounted for.
With the renewed interest in MSRs, more appropriate modeling tools are being developed. Oak Ridge National Laboratory developed one of the pioneering programs to analyze DNP movement in the MSRE in the 1960s (). Since the inception of that program, several projects have developed new analysis tools dedicated to MSRs (; ; ; ). The Monte Carlo N-Particle () and Serpent codes () are actively being developed to account for the changed delayed neutron source. To enable transients, deterministic methods are used, such as GeN-Foam (), which combines coars mesh thermal hydraulics with a deterministic neutronics code capable of modeling the impact of DNP drift (). Several low-fidelity codes, such as the MOlten SAlt Incompressible Calculation System known as MOSAICS (), LiCore (), and the System Analysis Module (SAM) (), have shown the ability to evaluate transients in MSRs on a system code level.
Idaho National Laboratory is actively working on modeling the MSRE by coupling the thermal-hydraulics codes Pronghorn () and SAM () to the neutronics solver Griffin (). These efforts have shown that Pronghorn and Griffin (; ) and SAM and Griffin () can be successfully coupled to model MSRs. Also, the Griffin-SAM coupling has been validated against MSRE zero power pump transients (). Griffin solves the neutron diffusion equation with discrete energy groups. The DNP drift is evaluated by reconstructing the delayed flux from the DNP field provided by Pronghorn.
Since 2023 researchers at the Technical University of Denmark have been developing the modified Point Kinetics (PK) solver Squirrel into the MOOSE framework. It is able to account for spatial deviations in the DNP field () by weighting the spatial DNP field with the adjoint flux. Additionally, Squirrel can estimate the temperature feedback by weighting the change in temperature with the adjoint flux. The importance of spatially weighting the DNPs during transients is discussed in ().
In this work, we compare the solutions of the neutron spatial dynamics Griffin and the 0-D neutronics solver Squirrel coupled to Pronghorn for modeling the MSRE under the MOOSE framework. The model and the coupling scheme between Pronghorn and Griffin or Squirrel are validated against the experimental data obtained from the MSRE reports. The validation is done for three different transients: pump start-up, pump coast-down, and natural circulation. Furthermore, the neutronics codes are verified against each other. The verification and validation are done within the same reactor model and on the same mesh. This approach allows for a detailed comparison of the PK solver and the spatial neutron dynamics solver codes with a consistent thermal-hydraulics simulation. Isolating the results of the neutronics codes from the thermal-hydraulics simulation enables a detailed comparison of the differences in the simulation results of both neutronics codes.
This paper is structured as follows: Section 2 provides a description of the solvers used in the analyses and discusses the coupling scheme between the neutronics and thermal-hydraulics codes. Section 3 presents the developed computational model of the MSRE and the modeling assumptions. Section 4 presents the simulation results for a static reactor at 8 MW obtained by Griffin coupled with Pronghorn, including the temperature field, the flow field, and the evaluated temperature coefficients. The static reactivity loss due to the DNP advection is calculated with Griffin and Squirrel for 235U and 233U fuels. Furthermore, the simulation results calculated with both neutronics codes are validated against the experimental data from the pump start-up, pump coast-down, and natural circulation transients. Additionally, the simulated DNP density during the pump start-up and the simulated power density and salt temperature during the natural circulation transient are discussed. Finally, Section 5 provides a summary and the conclusions of the study.
2 Analysis methodology
The methodology used in the neutronics codes Griffin and Squirrel and the coarse-mesh thermal-hydraulics code Pronghorn to obtain the flowing-fuel solutions are introduced in this section. Also, the multiphysics coupling scheme between the neutronics and thermal hydraulics, including the advection of the DNPs, is presented.
2.1 Neutronics methods
In the neutronics calculations we employ the spatial neutron diffusion code (Griffin) and the 0-D PK solver (Squirrel) to model the effect of the flowing fuel and the redistribution of DNPs during steady-state and transient calculations. The solutions of Squirrel, which is a modified PK solver for flowing-fuel MSRs, are verified against the solutions of Griffin’s diffusion solver. Squirrel can account for the time-dependent spatial distribution of the DNPs in the reactor by considering a proper weighting function.
2.1.1 Griffin: spatial dynamics solver
Griffin is a deterministic neutronics solver for analyzing advanced reactors. It can analyze the flowing-fuel behavior in MSRs () by calculating the prompt and delayed fission source separately. The delayed fission source is calculated using the advected DNP field provided by Pronghorn. The delayed fission source is then added to the prompt fission source to obtain the total flux. Griffin solves the linearized Boltzmann equationwhere is the neutron flux at time , at position , and of energy group . , , and are the total, scattering, and fission macroscopic cross sections, respectively. is the eigenvalue of the system, is the neutron yield per fission, is the total delayed neutron fraction, is the diffusion coefficient, is the neutron velocity, and are the prompt and delayed neutron spectra, and are the DNPs of group and it’s corresponding decay constant. The term represents the delayed neutron source, which can be determined by solving the DNP concentration equations for MSRs with flowing fuel. Modeling flowing fuel introduces an extra term to the DNP equations to account for the drift of DNPs in the core, and their decay outside the core as given in Equation 2 for the group:where is the fuel salt velocity, and the delayed neutron fraction of group . The advection term is added to the DNP equations to account for the DNP movement due to fuel flow, while the diffusion of DNPs is not considered in this work. Equation 2 is solved along with the homogeneous boundary condition to determine the concentrations of the DNPs at the core inlet, taking into account their decay while residing in the outer loop. Equations 1, 2 are strongly coupled through the delayed neutron source and the fission source. By including the advection term in the DNP tracking, the tight multiphysics coupling is expanded with the thermal-fluids code.
In the current work, the fission source is provided to the thermal-fluids code Pronghorn. The resulting distribution of DNPs obtained from the thermal-fluids code, is then transferred to Griffin. With the delayed neutron source Griffin can calculate the total neutron flux.
Griffin does not have the capability to calculate the kinetics parameters for flowing-fuel reactors, which require a more sophisticated approach to obtain the adjoint solution of the system. However, Griffin does calculate the kinetics parameters of stationary fuel reactors, which can be used to obtain the effective delayed neutron fraction for flowing fuel aswhere is the reactivity loss due to the DNPs advection with the fuel flow and the decay of the DNPs. This reactivity change can be calculated by taking the reciprocal difference of the stationary fuel eigenvalue and the flowing-fuel eigenvalue :
In Griffin three feedback mechanisms are considered in modeling MSRs:
• Temperature: affects the fuel salt (Doppler) and solid moderator microscopic cross sections.
• Density: affects concentration of the salt nuclides within the core due to fuel salt expansion.
• Velocity: affects DNP distributions in the core and outer loop.
In Griffin, the thermal feedback coefficient of the fuel salt accounts for changes in microscopic cross section and fuel salt expansion due to temperature and corresponding density changes. The thermal feedback coefficient of the reactor is then calculated by changing the temperature by globally, and as a result the density, relative to the temperature in a reference simulation. The temperature feedback coefficient is then calculated from the ratio of the reactivity change to the temperature change as
2.1.2 Squirrel: point kinetics solver
Squirrel is a PK solver developed for the transient analysis of MSRs () under the MOOSE framework. Squirrel solves a modified version of the PK equation to account for the advection of DNPs in the core and their decay outside the core by weighting the time-dependent DNPs with an importance function spatially, and it accounts for temperature distribution changes in the reactor. The details of the derivation of the PK equation for MSR applications is described in and will be discussed briefly in this section.
The PK formulation used in Squirrel is derived from the multigroup neutron flux equations by integrating Equations 1, 2 over energy and assuming a critical reactor so that yields the one group flux equation asand the corresponding DNP concentration equation as
First the one group neutron flux is factored into a purely time-dependent amplitude function and a time- and space-dependent shape function as
This factorization is a simple separation of the flux and is not an approximation. This separation is, in general, not unique and requires a second equation to ensure its uniqueness. We use a space integral over the shape function to keep the time dependence in the amplitude function. The chosen constraint condition is given bywith the steady-state one group adjoint flux function and a constant . is used as the importance weighting function of the reactor.
By multiplying
Equation 6with
, integrating it over space, and dividing the equation by the static importance-weighted neutron source yields
with the following parameters:
• The neutron lifetime
• The delayed neutron fraction
• The reactivity
• The static importance-weighted neutron source
and can be evaluated initially in a steady-state reactor so that the neutron lifetime and the delayed neutron fraction are time independent. The reactivity is split into three parts:with representing the reactivity response due to temperature changes in the reactor, the external reactivity insertions, and the reactivity necessary to keep the reactor critical when fuel is flowing. A common choice in the literature is to substitute the reduced DNP concentration, such as , into Equation 16. The final PK equations evaluated in Squirrel are
Squirrel relies on a thermal-hydraulics solver to obtain the spatial distribution of the DNP concentration given by Equation 2. In a critical steady-state reactor the left-hand side of Equation 10 is zero and can be defined through rearranging so that
This quantity is particularly interesting since it describes the static reactivity loss due to fuel motion.
The temperature’s effect on the reactivity is estimated by evaluating the deviation between the current and reference state (steady state):where is the reactor reference temperature and is the temperature feedback coefficient that is obtained from Equation 5. In the following analysis, the neutron flux and neutron fission source density are obtained from a steady-state eigenvalue calculation with Griffin. Also, the forward neutron flux was used to evaluate the reactivity components in Equations 16, 18 for simplicity.
2.2 Thermal-hydraulics methods: Pronghorn
Pronghorn is a coarse-mesh finite-volume thermal-hydraulics solver implemented in the MOOSE framework. It supports the development of nuclear reactors at the engineering scale ().
In this work, Pronghorn solves for the fluid flow distribution in the reactor, the DNP scalar field, and the fluid and solid enthalpy fields. The equations solved for thermal-hydraulics modeling in Pronghorn are the single-phase weakly compressible Navier-Stokes and energy conservation in porous media. The porous medium formulation assumes that the liquid fuel and the internal reactor structures occupy the same homogenized volume. It is primarily used to model the reactor core as a homogeneous system. The porosity is defined as the ratio between fluid volume and total volume.
In this context, the conservation of mass is given bywith the porosity , the fluid density , and the superficial velocity .
The conservation of momentum is given bywhere is the dynamic viscosity, is the turbulent viscosity using the 0-D turbulent mixing length model (), a time-dependent forcing term that represents the pumping force, the gravitational vector , the pressure , and the pressure drop coefficient using the Darcy and Forchheimer friction models.
The conservation of energy for the fluid phase is given byand the conservation of energy for the solid phase is given bywhere is the specific enthalpy of the fluid, is the specific enthalpy of the solid, is the fluid temperature, is the solid temperature, is the solid density, is the thermal conductivity of the fluid, is the turbulent heat diffusivity, is the solid thermal conductivity tensor, is the fluid-porosity-averaged volumetric heat exchange coefficient between the liquid and solid phases, is the heat source being deposited directly in liquid fuel (e.g., fission heat source), and is the heat source in the solid (e.g., residual power production in structures). For an assembly modeled as a porous medium, the fission source is defined as the total power of the assembly divided by its total volume.
The convective heat transfer between the porous core region and the solid core barrel is also included in the model through a computed heat transfer coefficient. The value of the porosity in the core region is 0.222. The pressure in the closed loop is fixed by fixing one pressure point at the reactor outlet. To avoid the appearance of a checkerboard pattern in the pressure field caused by the separation of velocity and pressure, Pronghorn employs the collocated formulation of the Rhie-Chow interpolation method. In this method the velocity flux at the faces is computed using the difference between the direct and cell-interpolated pressure gradients, suppressing the formation of strong pressure gradients at the cell centers, which enables the discontinuities in the porosity and body forces like drag or a pump force to be simulated without resulting in velocity oscillations. A more detailed description of the implementation can be found in , and a more general discussion of the topic can be found in . Pronghorn also calculates the DNP production, decay, and transport for Griffin Equation 2 and for Squirrel Equation 16.
3 MSRE specifications and developed models
3.1 MSRE description
The MSRE was a thermal spectrum reactor in which liquid fuel salt flowed through graphite moderator channels. The main reactor parameters considered in this work are listed in Table 1. A diagram of the reactor layout, including the core, the primary circuit, the primary heat exchanger, and the secondary system, is shown in Figure 1 (). The MSRE lattice was made of vertical graphite stringers with a 5.08 by 5.08 cm cross section, while the fuel salt flowed through a rectangular channel of 3.05 by 1.016 cm with round corners of radius 0.508 cm on the sides of the stringers (). The MSRE core configuration is shown in Figure 2. The left and top-right plots show the MSRE reactor assembly, while the bottom-right plot shows the MSRE 4-halves fuel salt channels with graphite stringers ().
TABLE 1
| Parameter | Value | Unit |
|---|---|---|
| Design Core Power | 8.00 | MWth |
| Core Height | 1.39 | m |
| Core Diameter | 1.63 | m |
| Fuel Salt Composition | LiF-BeF2-ZrF4-UF4 | – |
| Fuel Salt Molar Mass | 235U: 65.00-29.17-5.00-0.83 | % |
| 233U: 64.50-30.18-5.19-0.13 | % | |
| Fuel Enrichment | 235U: 33.0 | % |
| 233U: 91.5 | % | |
| Core Inlet temperature | 905.0 | K |
| Core Outlet temperature | 928.0 | K |
| Fuel Circulation Time | 25.2 | s |
The main reactor specifications of the MSRE.
FIGURE 1
FIGURE 2

Axial (left) and radial (top right) views of the cross-section-generation model for the MSRE core assembly. The view of the graphite lattice (bottom right) shows the 4-halves fuel salt channels.
The MSRE’s liquid fuel salt was a FLiBe base salt bearing U and Zr, composed of LiF-BeF2-ZrF4-UF4. The main fissile isotope was 235U, which was later replaced with 233U. The atomic fractions of the fuel salt isotopes are provided in Table 2 (
TABLE 2
| Isotope | Atom Fraction | |
|---|---|---|
| 235U Fuel | 233U Fuel | |
| Li-7 | 2.634E-01 | 2.618E-01 |
| F-19 | 5.948E-01 | 5.936E-01 |
| Be-9 | 1.179E-01 | 1.229E-01 |
| U-233 | — | 4.977E-04 |
| U-234 | — | 3.118E-05 |
| U-235 | 1.203E-03 | 3.778E-06 |
| U-238 | 2.443E-03 | 1.069E-06 |
| Zr-90 | 1.042E-02 | 1.085E-02 |
| Zr-91 | 2.273E-03 | 2.366E-03 |
| Zr-92 | 3.474E-03 | 3.616E-03 |
| Zr-94 | 3.521E-03 | 3.665E-03 |
| Zr-96 | 5.673E-04 | 5.904E-04 |
MSRE fuel salt atomic concentration.
TABLE 3
| Parameter | Fuel Salt | Graphite | Unit |
|---|---|---|---|
| Density | 2,263.0@900K | 1,860.0 | kg/m3 |
| Thermal Conductivity | 1.4 | 40.1 | W/m. K |
| Specific Heat | 1868.0 | 1757.3 | J/kg. K |
| Dynamic Viscosity | 0.008268 | – | Pa. s |
Fuel salt and graphite thermophysical properties.
3.2 Developed models
The MSRE model was developed using a 2-D axisymmetric domain in R-Z coordinates for both the spatial-dynamics neutronics and thermal-hydraulics calculations based on a model of the MSRE previously developed by Idaho National Laboratory (
A cut-through view of the reactor core vessel is provided on the left panel of Figure 3 (
FIGURE 3

MSRE core on the left (
The MSRE reactor geometry was simplified so the simulation and analysis could be efficient. The control rods and the outside regions of the active core, including the reactor vessel, the insulator, the gap between the reactor vessel and insulator, and the thermal shield, were not developed as part of the core configuration. The secondary loop was also not considered in the model. The temperature of the secondary side of the heat exchanger was set to a constant. The azimuthal symmetry of the MSRE model ignores some of the details of the real reactor system, but it preserves the important quantities of the core. The modeled core barrel has a radius of 0.70485 m, while the graphite-moderated core has a radius of 0.6914 m and a height of 1.6637 m. The lower plenum is 0.12954 m high, and the upper plenum is 0.21336 m high. The total salt volume in the reactor is 1.64 .
The fuel’s total circulation time in the whole system is 25.2 s; the fuel transitions through the core, lower plenum, and upper plenum in 17 s. In the pump block, the fuel is accelerated by a uniformly distributed momentum source in the momentum equation with a total value equal to m/s2. The volumes of the in-core and out-of-core regions reflect the volumes and circulation times reported in Refs.
A full 3D core model was developed for the MSRE using the Monte Carlo code OpenMC (
The fuel salt and graphite volume fractions in the reactor core region are 22.29% and 77.71%, respectively. This ratio is considered in obtaining cross-section homogenization and in the porous flow model implemented in Pronghorn. Additionally, the model considers the heat deposited in the solid graphite due to neutron thermalization and gamma heating. The considered value is of the total power produced in the reactor, which was calculated from previous OpenMC simulations presented in
TABLE 4
| Group | 235U Fuel | 233U Fuel | ||
|---|---|---|---|---|
| (pcm) | () | (pcm) | () | |
| 1 | 22.84 | 0.013336 | 25.45 | 0.012911 |
| 2 | 118.08 | 0.032739 | 68.22 | 0.034738 |
| 3 | 112.78 | 0.120780 | 53.12 | 0.11928 |
| 4 | 252.81 | 0.302780 | 104.95 | 0.28617 |
| 5 | 103.84 | 0.849490 | 34.21 | 0.7877 |
| 6 | 43.47 | 2.853000 | 12.28 | 2.4417 |
| Total | 653.82 | — | 298.23 | — |
MSRE delayed neutron precursor data.
3.3 Multiphysics coupling scheme
The multiphysics model of the MSRE was developed using the MOOSE MultiApps system, in which the coupling between the thermal-hydraulics solver and neutronics solvers is designed to allow for flexibility in exchanging problem variables using different neutronics models coupled to the same thermal model. Figure 4 shows the coupling scheme and the transferred parameters between the main application (Pronghorn) and the sub-applications (Griffin and Squirrel).
FIGURE 4

Coupling scheme between Pronghorn and the respective neutronics solver (Squirrel or Griffin).
Pronghorn is the main application, and it solves the Navier-Stokes equations, the DNP field for Griffin, and the reduced DNP field for Squirrel. Griffin provides the power density and fission source distributions to Pronghorn. The power density distribution is used to obtain fuel and moderator temperatures, density, pressure, and velocity fields. The fuel and moderator temperatures and the fuel density are used to update the cross sections for Griffin calculations. The fission source distribution is used in the calculation of the DNPs distribution to determine the delayed neutron source and reconstruct the total fission neutron source in the core region, considering their decay in the outer loop.
Squirrel relies on the initial neutron flux, power density, fission source density, and the kinetics parameters calculated by the steady-state Griffin simulation. Squirrel scales the power density and neutron flux during the transient calculations with a power amplitude function, where the steady-state power distribution or shape function is used throughout the entire transient simulation.
Since the neutronics solvers follow two different approaches, the key aspect of the coupling is to maintain the flexibility to swap each solver in each transient while maintaining the same Pronghorn simulation. This approach eliminates differences in the performance of the diffusion based neutronics solvers and the PK solver originating from thermal-hydraulics solutions.
In this work, we performed validation tests encompassing steady-state, pump start-up, pump coast-down, and natural circulation tests. The details of the coupling need to be different for each simulation. In this paper, the following three cases are evaluated:
1. Steady state: The eigenvalue problem is solved by Griffin, considering the steady-state diffusion equation with DNP concentration distributions based on the thermal field and DNP concentration distributions provided by Pronghorn, assuming a constant power level. Pronghorn solves a time-dependent problem until a steady-state solution is achieved at each Picard iteration.
2. Pump start-up and coast-down: The reference state is obtained at a very low power level and without fuel flow. Then, at each time step, new DNP concentration distributions are calculated by Pronghorn based on the pump head changes, and these distributions are used to reconstruct a new fission source and perform an eigenvalue calculation in Griffin to determine the reactivity losses due to fuel movement using Equation 4, while Squirrel solves Equation 16 to obtain the change in reactivity. During this simulation, Pronghorn solves a time-dependent problem, while the neutronics solve a steady-state problem. Since a constant low power level was maintained, thermal feedback is ignored, and the change in the eigenvalue can be attributed to the change in the DNP field.
3. Natural circulation test: Both neutronics codes and Pronghorn solve a time-dependent or transient problem starting from the initial steady-state solution to adapt to the power change. At each time step, Pronghorn exchanges the required variables with the neutronics solver to calculate the new power and temperature distributions.
4 Verification and validation tests
In this section, we provide a code-to-code verification between Griffin and Squirrel for transient analysis and validate these codes’ results against the experimental data of the MSRE. First, the steady-state solutions obtained from coupled Griffin-Pronghorn calculations are presented. Then, the results obtained with the multiphysics model employing Griffin and Squirrel are validated against the experimental measurements for the pump start-up and coast-down at zero power, along with natural circulation test results.
4.1 Steady-state results
In this sub-section, we provide the steady-state solutions of the MSRE model obtained from coupled Griffin and Pronghorn calculations for isothermal temperature coefficients and effective delayed neutron fractions of stationary and circulating fuels, along with steady-state distributions of the power, temperature, and DNP concentrations, which Squirrel needs to initiate coupled transient calculations.
Table 5 provides the calculated values of the isothermal temperature coefficients of the 235235U and 233U fuel salts. Due to the temperature dependency assumed for density in Equation 23, the temperature coefficients involve both the density and Doppler feedback. The isothermal temperature coefficient is calculated by globally varying the temperature in the reactor between 850 and 1000 K using Equation 5 and considering stationary fuel. The calculated values are also compared to values measured during operations of the MSRE, as reported in
TABLE 5
| Fuel Type | Measured ( | Griffin |
|---|---|---|
| 235U | ||
| 233U |
Isothermal temperature coefficient (pcm/K) at 923 K for 235U and 233U fuels calculated by Griffin.
Figure 5 shows the reactor field variables obtained from coupled steady-state Griffin-Pronghorn calculations for power density, fuel salt temperature, and fuel salt velocity. The majority of the power is generated at the center of the active core region, while the outer core does not get heated. There are two apparent peaks in power density in the upper and lower plenum regions due to the massive increase in fuel salt volume and the absence of the graphite moderator in these regions.
FIGURE 5

Steady-state field variables: power density, fuel salt temperature, and salt superficial velocity.
The middle plot of Figure 5 shows the fuel salt temperature distribution. The temperature distribution is skewed toward the top of the core, as expected, with an approximate maximum fuel temperature of 950 K at the top of the graphite block, close to the core’s center. In the upper plenum, colder salt from the outer regions of the core is drawn toward the riser located above the core’s center. There, the cooler salt mixes with the hotter salt from the core’s center, significantly reducing the fuel salt temperature.
The right plot of Figure 5 shows the fuel salt superficial velocity with streamlines indicating the fuel salt path. The salt enters the lower plenum from the downcomer and flows radially inward into the graphite block region, then flows upward without any lateral movement. In the upper plenum, the salt flows again radially inward toward the riser. In the riser, the flow rate is the highest since the cross-sectional area is the smallest. In the pump, the salt is forced to move through the elbow into the downcomer and back to the lower plenum again, with a total circulation time of 25.2 s.
For the flowing-fuel case, the DNPs are advected in the reactor core and the primary loop, resulting in the redistribution of the DNPs based on their half-lives, which leads to reactivity losses as DNPs decay in regions of lower importance. Outside of the active core, the importance of the DNPs is almost zero. Figure 6 depicts the distribution of the six groups of DNPs within the fuel salt for the reactor operating with 233U fuel salt. The longest-lived DNP group (Group 1) decays outside the active core region and peaks toward the top region of the core. The undecayed DNPs flow back into the core through the lower plenum, resulting in almost homogeneous mixing in the core. Groups 2 and 3 of the DNPs decay mostly in the outer region of the core, resulting in larger delayed neutron losses. For the shortest-lived group (Group 6), the DNPs decay at almost the same location as their initial position and peak toward the core center, resulting in smaller delayed neutron losses.
FIGURE 6

Steady-state DNP concentration () distributions in the MSRE 233U fuel salt. Group 1 at the top left is the longest lived, and Group 6 at the bottom right is the shortest lived.
Table 6 provides the effective delayed neutron fraction of stationary and flowing fuels, and the loss in effective delayed neutron fraction for both 235U and 233U fuel salts. The reported MSRE values of the 235U fuel salt are from
TABLE 6
| 235U | 233U | ||||
|---|---|---|---|---|---|
| MSRE | Griffin | Squirrel | Griffin | Squirrel | |
| (pcm) | 666 | 654 | — | 298 | — |
| (pcm) | 212 | 223 | 220 | 110 | 113 |
| (pcm) | 454 | 431 | 434 | 188 | 185 |
| (%) | 31.8 | 34.1 | 33.6 | 36.9 | 37.9 |
Steady-state effective delayed neutron fraction of 235U and 233U fuels for stationary and flowing fuels.
4.2 Pump start-up and coast-down
In this section we discuss the results of the validation test against the experimental data of the pump start-up and coast-down tests. These tests were performed with 235U fuel salt at a low power level (zero power or cold conditions). A detailed description of the experimental setup of this transient can be found in
During the pump start-up test, as the fuel salt mass flow rate started increasing, the DNPs flowed outside the active core region and decayed in regions of lower importance and in the outer loop, resulting in increased reactivity losses. In the pump start-up simulation, the pump force in the thermal hydraulics model was adjusted to achieve a fuel mass flow rate change from 0% to 100% in approximately 8 s, while in the pump coast-down simulation the pump force was adjusted to achieve a fuel mass flow rate change from 100% to 0% in approximately 20 s. The slower coast-down of the fuel flow can be explained by the hydraulic inertia that the system had at maximum flow rate. The measured and calculated mass flow rates for both test cases are displayed in Figure 7, along with the normalized pump force values used in Pronghorn.
FIGURE 7

Relative pump force and mass flow rate evolution during the pump start-up and coast-down tests. The experimental data is from (
The estimated uncertainty for the measured reactivity considered in this work originates from the following parameters:
• Control rod position indicator: The uncertainty in the control rod position measurement during the zero power tests was estimated to be 0.01 inches.
• Integral worth curve: The stable period was determined by averaging the slopes of the two curves, which usually agreed within 2%.
• Fuel salt advection: Both the sensitivity of the rod-drop experiment and the fuel circulation indicate that the reactivity calculated from the integral worth curve may underestimate the value. For this reason, it is assumed that the uncertainty in the integral worth curve for the final loading is 2%.
Figures 8, 9 display, on the left-hand side, the experimental values of the reactivity along with simulation results for pump start-up and coast-down, respectively. During the pump start-up test, the redistribution and decay of the DNPs led to a maximum reactivity loss of 284 pcm after 13 s. As the undecayed DNPs reentered the active core region, the measured reactivity loss was reduced again and started oscillating at approximately 212 pcm until it reached steady-state conditions. During the pump coast-down test, the reactivity loss decreased as the fuel salt flow rate decreased due to the fact that the DNPs decay rate in the active core region increases. Finally, the reactivity loss reaches a zero value at zero-flow conditions, as the system returns to its initial state.
FIGURE 8

Reactivity loss during the pump start-up transient. The experimental data is from
FIGURE 9

Reactivity loss during the pump coast-down transient. The experimental data is from
The simulation results of both codes show very good agreement for both pump tests. For the pump start-up test, both codes are in good agreement with the measured experimental values and captured the initial increase in reactivity loss and the final oscillation in reactivity loss, although they failed to capture the measured peak reactivity loss of 284 pcm by 34 pcm. The reason for this discrepancy is not fully understood, but it could be related to one or more of the following:
• Channel effect: The fuel channels are not resolved in the homogenized core model investigated here. The flow pattern in the fuel channels of the MSRE might cause a larger reactivity effect that the porous media approximation can not capture.
• Bubbles: Bubbles in the fuel salt have a negative reactivity effect, which is not considered in the current model. When the fuel starts to flow, bubbles are entrained from the cover gas in the reactor pump and advected through the primary circuit.
• Control rod servo: The flux servo controller kept the reactor critical during the experiment. Its precision during transients is not fully understood and it could have led to an overshooting after a fast change in reactivity.
For the pump coast-down test, both codes are in good agreement with the measured values for the entire period of the test. Additionally the difference in the simulation results obtained with Squirrel and Griffin is shown on the right axis of Figures 8, 9. The maximum difference between the two codes is 3.5 pcm for the pump start-up and 2.5 pcm for the coast-down. Since DNP advection has a minimal effect on the fundamental mode, good agreement between the codes is expected, as the assumption posed in Equation 9 is mostly fulfilled.
These transients increase our confidence that the circulation time and fuel volume are used properly, and they demonstrate that the neutronics solvers correctly evaluated the effect the shifted spatial distribution of the DNPs had on the reactivity.
In Figure 10, the density of the longest-lived DNP group (Group 1) is shown during the pump start-up test at different times up to 50 s. Initially, the DNP shape matches the fission source density in the core since there is no fuel flow. As the pump starts, the DNPs move upward into the riser (at approximately 10 s) and then down through the downcomer. At 20 s, the DNPs reenter the core from the bottom. This return of the DNPs into the core is responsible for the reduction in reactivity loss observed in Figure 8. The DNPs that are present at 30 s are advected out of the core, and at this time the returning DNPs have not yet reached the upper region of the core, leaving a region of lower DNP density in the middle of the reactor. At 50 s, the maximum DNP density is inside the core. Throughout the process, the DNPs are being mixed in the core.
FIGURE 10

DNP concentration () distribution of Group 1 shown at different times during the pump start-up transient.
In Figure 11, the density of the longest-lived DNP group (Group 1) is shown during the pump coast-down test at different times up to 50 s. Initially, the DNPs are well mixed throughout the core. As the fuel flow is reduced (pump force reduced), more DNPs decay in the active core region, resulting in a decrease in reactivity losses. At 20 s, significantly fewer DNPs reenter the core from the bottom, clearly showing that fewer DNPs are advected through the outer core. At 50 s, the DNP shape matches the fission source density in the core. During the coast-down transient, the DNP density in the core increases steadily with minor oscillations.
FIGURE 11

DNP concentration () distribution of Group 1 shown at different times during the pump coast-down transient.
4.3 Natural circulation test
In this test, the MSRE’s natural circulation was examined. The fuel pump was turned off and the fuel salt circulated through the system due to natural circulation. The main test characteristics can be summarized as follows:
• The reactor was operated with 233U fuel salt with the primary pump turned off.
• The regulating control rod remained in its initial position for the entire test.
• The reactor’s initial power was 4.1 kW, assuming the reactor was at equilibrium steady-state conditions.
• The fuel salt inlet temperature was slowly decreased by adjusting the flow rate on the secondary side.
• The uncertainty in the measured power signal was assumed to be 2%.
The reduction in the fuel salt temperature led to a positive reactivity insertion (due to the negative temperature coefficient); therefore, the power of the reactor increased as the temperature decreased. This increase in power and the resulting heating of the fuel increased the fuel temperature. The hotter fuel caused the power to stabilize at a new level. This process of reducing the fuel temperature was repeated several times, and multiple power plateaus were reached. The maximum power was 351 kW, and the final power was 324 kW. During the transient, the reactor power developed fully unprotected, with the control rod remaining in its initial position, and the reactor was fully driven by temperature feedback during the test. The effect of the DNP movement in the circulating fuel was minimal due to the very low fuel-flow rate (
During the simulation, the inlet temperature was prescribed by adjusting the secondary temperature of the heat exchanger. The model used is not able to reproduce the reported fuel flow with natural circulation, most likely because it lacks the correct height difference between the core and the heat exchanger. Therefore, the mass flow rate was adjusted by changing the pump force in Pronghorn. The transient was induced by the prescribed change in inlet temperature and the adjustment of the pump force. With colder fuel entering the core, the power increases due to the positive temperature feedback. The increasing power heats up the core. The reactor reaches a steady power when the inlet temperature is kept constant, which happened multiple times during the transient.
Figure 12 shows the inlet mass flow rate and the inlet and outlet fuel temperatures alongside the measured inlet and outlet fuel temperatures reported in
FIGURE 12

Mass flow rate and temperature evolution during the natural circulation test. The left axis shows inlet and outlet temperatures, and the right axis shows the mass flow rate. The experimental data is reported in
FIGURE 13

n values (left axis) of Griffin and Squirrel and the MSRE (
Figure 14 shows the spatial power density in the reactor core at different times during the natural circulation test, as calculated by Griffin. Initially, the power density is low at 19.0 kW/m3; during the transient the power density increases up to 1.5 MW/m3 at 240 min. After that, it decreases slightly. At all times, the power density is highest in the center region of the core, and there is no measurable shift in the shape of the power density. Figure 15 shows the fuel salt temperature at different times during the natural circulation test. At the beginning of the transient, the inlet temperature increased up to 910 K, and it reached 960 K at the end of the transient. The difference in the simulated power obtained with Squirrel and Griffin is shown on the right axis of Figure 15. The maximum difference between the codes is 7.5 kW.
FIGURE 14

Power density (W ) distribution shown at different times during the natural circulation test, as calculated by Griffin.
FIGURE 15

Fuel salt temperature (K) distribution shown at different times during the natural circulation test.
5 Summary
In this work, verification and validation test results were presented for the multiphysics modeling of the MSRE using coupled neutronics and thermal-hydraulics solvers developed under the MOOSE framework. The thermal-hydraulics calculations were performed with the Pronghorn code, which used an axisymmetric domain in R-Z coordinates with a porous media approximation. The neutronics calculations were performed with either the spatial neutron dynamics solver Griffin, which used an axisymmetric domain in R-Z coordinates with diffusion approximation in a homogenized domain, or the 0-D solver Squirrel with PK approximation. The developed model’s dimensions and its material’s thermophysical properties were obtained from the open literature, as were the experimental test data of the MSRE.
The models that were developed demonstrate the codes’ capability of modeling liquid flowing fuel and the resulting reactivity changes caused by the redistribution and decay of the DNPs. Both solution approaches were verified against each other and validated against the experimental data of the pump start-up, pump coast-down, and natural circulation tests. During the pump start-up and coast-down tests, both approaches predicted the reactivity loss resulting from fuel salt flow changes without thermal feedback effects. The test results of both approaches and their measured values show very good agreement. The maximum difference in reactivity loss between the two approaches is 3.5 pcm, indicating that the advection effects of the DNPs were captured accurately. For the natural circulation test, the fully coupled time evolution of the codes was tested. In this test, the inlet mass flow rate and inlet temperature were prescribed by adjusting the pump force and the secondary side inlet temperature to match the experimental data of the MSRE. Both approaches accurately predicted the power evolution during the test and captured the thermal feedback of the system.
A comparison of the results of the 0-D neutronics solver Squirrel and the spatial dynamics code Griffin, both coupled to the same thermal-hydraulics solver, showed that both codes yield similar results for the three tests, confirming that the codes capture the same physics qualitatively and quantitatively. This agreement in results suggests that the spatial weighting of DNPs used in the PK equation captures the physics to a degree similar to that of the spatial diffusion solver. While both neutronics solvers agreed on the presented transients, spatial dynamics offers a higher fidelity that the PK equation might not be able to capture. The PK equation is known to not being able to properly account for fast and local transients (
). In a MSR these transients conditions might occur when:
• A fuel channel is blocked.
• The fuel salt is drained.
• Bubbles are formed locally and enter the core region.
• Over-cooled fuel enters the core.
• The reactor is over-fueled.
Future work will focus on testing spatial dynamics and PK codes on transients that are challenging to capture with the 0-D solver Squirrel, particularly fast and local transients. The separability assumption of flux shape and amplitude may not always hold for these scenarios. Additionally, strategies to mitigate the shortcomings of PK such as the improved quasi-static method in Griffin to update the shape function may help in the future.
Statements
Data availability statement
The raw data supporting the conclusions of this article will be made available by the authors, without undue reservation.
Author contributions
PP: Writing – review and editing, Writing – original draft. MJ: Writing – review and editing, Writing – original draft. MT: Writing – original draft, Writing – review and editing. RF: Writing – review and editing, Writing – original draft. SW: Writing – original draft, Writing – review and editing. JO: Writing – original draft, Writing – review and editing.
Funding
The author(s) declare that financial support was received for the research and/or publication of this article. The software development activities in this article were funded by the DOE Nuclear Energy Advanced Modeling and Simulation program. This research made use of the resources of the High Performance Computing Center at Idaho National Laboratory, which is supported by the Office of Nuclear Energy of the U.S. Department of Energy and the Nuclear Science User Facilities.
Conflict of interest
The authors declare that the research was conducted in the absence of any commercial or financial relationships that could be construed as a potential conflict of interest.
Generative AI statement
The author(s) declare that no Generative AI was used in the creation of this manuscript.
Publisher’s note
All claims expressed in this article are solely those of the authors and do not necessarily represent those of their affiliated organizations, or those of the publisher, the editors and the reviewers. Any product that may be evaluated in this article, or claim that may be made by its manufacturer, is not guaranteed or endorsed by the publisher.
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Summary
Keywords
MSRE, PKE, DNP, start-up, coast-down
Citation
Pfahl P, Jaradat MK, Tano ME, Freile RO, Walker SA and Ortensi J (2025) Comparison of spatial dynamics and point kinetics approaches in multiphysics modeling of the molten salt reactor experiment. Front. Nucl. Eng. 4:1617048. doi: 10.3389/fnuen.2025.1617048
Received
23 April 2025
Accepted
17 June 2025
Published
11 August 2025
Volume
4 - 2025
Edited by
Fabio Giannetti, Sapienza University of Rome, Italy
Reviewed by
Andrea Di Ronco, Polytechnic University of Milan, Italy
Antonio Cervone, University of Bologna, Italy
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Copyright
This work is authored in part by Philip Pfahl, Mustafa K. Jaradat, Mauricio E. Tano, Ramiro O. Freile, Samuel A. Walker and Javier Ortensi, © 2025 Battelle Energy Alliance, LLC.
This is an open-access article distributed under the terms of the Creative Commons Attribution License (CC BY). The use, distribution or reproduction in other forums is permitted, provided the original author(s) and the copyright owner(s) are credited and that the original publication in this journal is cited, in accordance with accepted academic practice. No use, distribution or reproduction is permitted which does not comply with these terms.
*Correspondence: Philip Pfahl, philip.j.f.pfahl@gmail.com
ORCID: Philip Pfahl, orcid.org/0009-0001-9130-3634; Mustafa K. Jaradat, orcid.org/0000-0003-2750-6055; Mauricio E. Tano, orcid.org/0000-0003-3417-3869; Ramiro O. Freile, orcid.org/0000-0003-0729-7081; Samuel A. Walker, orcid.org/0000-0003-1442-9636; Javier Ortensi, orcid.org/0000-0003-1685-3916
Disclaimer
All claims expressed in this article are solely those of the authors and do not necessarily represent those of their affiliated organizations, or those of the publisher, the editors and the reviewers. Any product that may be evaluated in this article or claim that may be made by its manufacturer is not guaranteed or endorsed by the publisher.