Abstract
Recently, as a strong candidate for artificial muscle, dielectric elastomer actuators (DEAs) have been given the spotlight due to their attractive benefits from fast, large, and reversible electrically-controllable actuation in ultra-lightweight structures. Meanwhile, for practical use in mechanical systems such as robotic manipulators, the DEAs are facing challenges in their non-linear response, time-varying strain, and low load-bearing capability due to their soft viscoelastic nature. Moreover, the presence of an interrelation among the time-varying viscoelasticity, dielectric, and conductive relaxations causes difficulty in the estimation of their actuation performance. Although a rolled configuration of a multilayer stack DEA opens up a promising route to enhance mechanical properties, the use of multiple electromechanical elements inevitably causes the estimation of the actuation response to be more complex. In this paper, together with widely used strategies to construct DE muscles, we introduce adoptable models that have been developed to estimate their electro-mechanical response. Moreover, we propose a new model that combines both non-linear and time-dependent energy-based modeling theories for predicting the long-term electro-mechanical dynamic response of the DE muscle. We verified that the model could accurately estimate the long-term dynamic response for as long as 20 min only with small errors as compared with experimental results. Finally, we present future perspectives and challenges with respect to the performance and modeling of the DE muscles for their practical use in various applications including robotics, haptics, and collaborative devices.
1 Introduction
Artificial muscles have been given great attention as the next-generation actuators for robotics and collaborative systems owing to their versatility in motion and inherent flexibility enabling the robots to be suitable for use in a safe working environment. As one of the promising candidates for artificial muscles, dielectric elastomer actuators (DEAs) have been intensively studied (). Generally, the DEA is composed of a DE membrane and a couple of thin compliant electrodes. These electrodes are established on both surfaces of the DE membrane through various methods, including brushing, spraying, and sputtering. When an electrical voltage is applied across the compliant electrode, the DEA, pre-stretched and clamped onto a rigid frame, is compressed by electrostatic force in the thickness direction and simultaneously expands to the in-plane direction (). The electrically-induced actuation performance is scalable by following a simple electrostatic model, which can be expressed by the equation below.where is the effective pressure, is the permittivity of free space, is the relative permittivity of the dielectric elastomer, V is the voltage input, and z is the thickness. Since the relative permittivity is one of the crucial parameters to determine the achievable area strain of the DEAs, researchers have adopted diverse dielectric materials including acrylic elastomers, silicone elastomers, and polyurethanes for the DEAs (; ; ).
Due to the attractive benefits from large strain actuation, high energy density, and mechanical resilience coming from a highly flexible structure, the DEAs have been exploited for various applications such as haptic devices, soft grippers, wearable interfaces, and locomotion (; Yun et al., 2019; ; ; ; Youn et al., 2021). For better usability in these applications, the integration of stiff frame, fiber, fluid, and pneumatics into a dielectric elastomer has been also attempted to improve the actuation performance of the DEAs (; Zhang C et al., 2015; ; ; ; ; ; ; ). Depending on the purpose, researchers have proposed DEAs with different designs such as multilayer stack, extender, bending beam, diaphragm, and rolled structures for eliciting linear elongations, out-of-plane expansions, or bending movements from the fundamental in-plane expansion behavior responding to electrical stimulation ().
Of these proposed configurations, we investigate rolled DEAs in detail. Rolled DEAs, as the name suggests, are fabricated by rolling dielectric elastomer films into a cylindrical shape (). From the rolling process, multiple DE layers are created and the actuator can withstand higher load and more actuation cycles compared to single-layer DEAs (). When a spring core is embedded in the fabrication stage, the configuration is termed the spring-rolled DEA. Owing to the use of the compressed spring structure enabling axial stretching via a spring being restored from its compressed state, spring-rolled DEA could produce electrically controllable and linear tensile stroke while maintaining its structure without the need for an external frame or clamping mechanism ().
However, despite the evolution of DEAs with various aspects, difficulty in their fine control is a huge obstacle to exploiting DEAs for practical use in robotic applications. Although many models have been proposed to establish a control strategy, long-term and/or dynamic actuation responses of the DEAs rarely allow accurate estimation due to the presence of inherent non-linear and complex time-dependent viscoelastic behavior, which is interrelated with dielectric and conductive relaxations (Zhao et al., 2011; ). Adding to the complexity, the DEA is also affected by cyclic relaxations. With repeated loading and unloading in dynamic actuation, the decrease in relaxation modulus becomes less with the increasing number of loading cycles (; ).
In this paper, studies on the rolled DEAs are reviewed with respect to fabrication methodologies and models for predicting their actuation responses. Moreover, we propose a new model integrating hyperelastic and viscoelastic models that is capable of estimating the long-term viscoelastic creep deformation as well as temporal and frequency responses of the spring-rolled DEA. Lastly, we discuss practical considerations and perspectives for implementing DE actuators in diverse application fields.
2 Dielectric elastomer muscle
For rolled DE configurations, commercially available 3 M VHB acrylic elastomers, as well as silicone elastomers, are widely used thanks to their soft and elastic nature, and relatively high dielectric properties (). As a compliant electrode for the DEA, carbon-based conductive materials and metallic nanowires have been mainly adopted due to their cost-effectiveness, facile coating process in large areas, and high tolerance to electrical excitation up to several kilovolts (; ; ).
Generally, as illustrated in Figure 1, depending on the material adopted for the DE membrane, the rolled DEAs can be prepared by following two different processes. Figure 1A presents a stepwise fabrication process of a silicone-based rolled DEA. Both Ecoflex and Sylgard, commercially-available polydimethylsiloxane (PDMS), have been widely exploited for the silicone-based DE membrane (). Unlike pre-cured elastomers, silicone elastomers allow thickness control, as they can be solidified at an arbitrary shape because liquid elastomers can maintain chain mobility at room temperature for over an hour, which provides enough time for structural forming via bar coating or spin-coating. A single-layered DEA is prepared by curing the thin liquid elastomer, followed by establishing a thin conductive layer on both surfaces and the DEA can be a multi-layered structure by repeating the fabrication process. Particularly, their rolled configuration can be achieved by cutting the membrane DEA into a strip, rolling, and then integrating a couple of rigid covers onto both ends of the structure.
FIGURE 1
In parallel, 3 M VHB acrylic elastomer-based rolled DEAs can be constructed by following the fabrication process illustrated in Figure 1B. Firstly, two acrylic DE membranes are cut from a 3 M VHB tape batch. Then, the membranes are bi-axially pre-stretched and conductive layers are established. The pre-stretching is done to enhance actuation performance by improving the material’s electromechanical properties, such as its electrical breakdown strength, response time, and pull-in stability (
Applications of the silicone-based DEAs are depicted in Figures 1C–E. The wing flapper shown in Figure 1C is driven by a silicon-based rolled DEA, which is made of BJB TC-5005 silicone as adopting graphite powder for compliant electrodes, and it is reinforced with a shell structure. This structure is bio-inspired from insects’ thoracic mechanism, and it serves to maintain DEA’s pre-stretch, provide external structure, and function as a mechanical amplifier. The prototype dynamically produces a strain of 6.1% at 1 Hz under an electric voltage of 6 kV (
Figures 1F–H depict applications of the acrylic elastomer-based spring-rolled DEAs. Figure 1F shows a walking robot using the spring-rolled DEA (
3 Time-dependent modeling of dielectric elastomer muscle
3.1 General modeling methods
Since the development of spring-rolled DEA, several modeling approaches have been proposed in order to estimate the electro-mechanical actuation response of DEAs. The modeling approaches can be categorized into two main types, stress-strain models and analytical electromechanical models. In the case of the stress-strain modeling method, the actuation behavior is analyzed by considering the internal physics of the actuator, such as the stress-strain relationship and energy equilibrium within the actuator components. In the beginning stages, the force-actuation stroke relationship of spring-roll DEAs was modeled by considering their geometry. Based on the simulation, it was reported that the output force of the DEA is proportional to its roll stiffness (
Meanwhile, the analytical electromechanical modeling method considered the step voltage response and frequency response of the DEAs. These responses are analyzed by using conventional electro-mechanical system models, which were expressed as a combination of parameters achieved from experiments. The electrical system could be expressed with the parameters of inductance (L), resistance (R), and capacitance (C). The parameters of mass (m), damping coefficient (c), and spring constant (k) were used for the mechanical system. For an analytical modeling method using the second-order mass-spring-damper model, the model parameters including damped frequency, damping ratio, and damping coefficient are obtained from the step voltage response of the DEA. This work focused on the methodology that could extract system parameters from transient measurements under a fixed voltage level (Tryson et al., 2010). In a wider scope, a dynamic response model formulated by integrating the mechanical mass-spring-damper model with the electrical model composed of R and C was proposed. The expanded analytical model could allow the formulation of static step response as well as frequency dependence in the actuator performance. However, the model requires practical verification and comparison with experimental results (Zhao et al., 2018).
3.2 Modeling hyperelasticity under stationary load
As introduced in the previous section, the stress-strain modeling method exhibited limitations in accurately estimating large strain actuation. As the solution, hyperelasticity models have been proposed since the models consider the non-linear nature of dielectric elastomers resulting from long and flexible polymer chains (
3.3 Modeling time-dependency under dynamic load
Although it is reported DEAs are capable of producing electrically-controllable strain, their actuation strain to the applied electric field is non-linear and time-dependent. DEAs also suffer from the viscoelastic creep phenomenon originating from dissipative relaxations within the material. These time-dependent and rate-dependent phenomena are not observed in stationary load conditions, but they prevail under dynamic loading cases. Therefore, addressing the viscoelastic behavior of the DEAs along with hyperelastic modeling is a key factor in improving accuracy in the estimation of their stationary and dynamic actuation performance. In viscoelastic modeling methods, the elastomer could be described by rheological models. As can be seen in the conventional 2-branch general Maxwell model (Zhang J et al., 2015;
Meanwhile, in our previous study, we investigated the dynamic behavior of the rolled DEA with a compressed spring core for a period of as long as 20 min (
FIGURE 2

(A) Schematic of the DE artificial muscle experimental setup and apparatus. (B) Comparison of the long-term 5-branch model simulation (red) and experimental data (black). (C) Comparison of the 2-branch model simulation (blue) and experimental data (black).
Further experiments are conducted to verify the proposed model. The spring-rolled DEA is fabricated following the steps outlined in Section 2 using 3 M VHB F9473PC. As the elastomer’s thickness is 254 μm, instead of manually pre-stretching it before rolling, it was pre-stretched after using the compressed spring’s restoration. To observe and verify the estimation capability of the model, a robotic arm assembly was prepared and the DEA was installed to control the arm, as shown in Figure 2A. An encoder was placed at the hinge and the DEA’s deformation was calculated from the angular data. For the experiment, a sinusoidal voltage input of 0.5 Hz frequency and 4000 V amplitude was applied and the actuator’s response was measured for 1,200 s.
The parameters on the left-hand side of the first equation can be obtained from the experimental setup and the fabrication stage, refer to Table 1. and J can be derived from initial conditions, the initial actuator length, assuming no load is applied to the system. Then, only eight unknown parameters remain, which comprise the time constants of each rheological model branch, . In the model-fit process, in order to minimize computational burden, and are assumed to be powers of 10, and , so that , as the rise time of the actuator response is more than 20 min. For the value optimization, the set of parameters that yields the lowest cost function, compared to the experimental data, is selected. The cost function is composed of root-mean-square error and actuation stroke error. The optimized parameters for the data in Figure 2B are , , , , , , , .
TABLE 1
| Parameter | Value |
|---|---|
| DE material | 3 M VHB F9473PC |
| Relative permittivity | 4.08 |
| Initial DE film dimensions (mm) (Lx, Ly, Lz) | 60, 250, 0.254 |
| Electrode material | Carbon powder |
| Electrode dimensions (mm) (L1, L2) | 40, 230 |
| Initial spring length, Ls (mm) | 110 |
| Spring diameter (mm) | 7 |
| Spring constant, k (N/m) | 180 |
| Horizontal end point, a (mm) | 60 |
| Vertical end point, b (mm) | 110 |
| Passive region length, w (mm) | 47.3 |
| Applied weight, P (g) | 72.6 |
| Applied voltage, (V, Hz) | 4000, 0.5 |
| Stretch limit, J | 200 |
Dielectric elastomer muscle fabrication parameters.
Figure 2B clearly depicts that the actuator’s relaxation phenomenon (black) is time-dependent and prolongs without reaching an equilibrium when actuated under the dynamic loading condition. The figure verifies that the proposed model addresses both the hyperelasticity and time-dependency of the dielectric elastomer, and as a consequence, it is able to accurately estimate the long-term dynamic response of the actuator. The proposed model’s performance on a different loading condition has been tested and verified as well. Its detailed modeling process and results are included in the Supplementary Material S1. Figure 2C depicts the simulation result of the actuator when the 2-branch rheological model is used. The optimal model parameters are , and . It can be observed that for the long-term actuation and under dynamic loading, the conventional 2-branch model is insufficient to accurately model the complex long-term response of the DEA. Therefore, the introduction of multiple branches to the rheological model is necessary, if the DEA were to be operated in practical and long-term applications. As mentioned, the optimization method was selected to minimize the computational burden and the results prove its potential. However, this method has its limitations. For a more accurate estimation of the long-term response, the number of branches in the rheological model can be increased. This in turn increases the number of unknown parameters. As a consequence, despite using the optimization method presented, the computation time for selecting optimal values increases. In Section 4, we further discuss the tradeoff relationship between accuracy and efficiency that follow in the multiple parameter estimation methods.
4 Future perspectives and challenges
4.1 Artificial intelligence-based data-driven modeling of non-linear response
In the current stress-strain modeling method, the rheological model describing the viscoelasticity of the actuator contains unknown parameters that need to be determined. These parameters are found empirically from experiments. Considering DE muscles’ long-term behavior and their application, the rheological model with multiple branches needs to be used. However, the current parameter optimization process is bound to result in a greater computational burden with the increase in the number of parameters. In addition to the increased burden, the optimization process is prone to fall into local minima, and thus a thorough examination is required.
● Data-driven modeling: Considering the complexity of multiple parameter models, approaching the problem with artificial intelligence-based data-driven modeling seems appropriate.
● Real-time multiple parameter estimation with computation efficiency: Increasing the accuracy of the model is of great issue. However, as can be seen in experiments by
4.2 Practical considerations for application
Owing to their actuation capability, producing a large and controllable electrically-induced strain with fast response speed, and soft and lightweight configuration, DEAs have been given great attention as a promising candidate for artificial muscle. Advances in DEA technology with respect to material and structural design could contribute to eliciting outstanding actuation performance on par with or exceeding that of a natural muscle. Moreover, the recent development of rolled DEAs opened up opportunities for exploiting them for practical applications since DE muscles could produce much larger force and energy output than conventional membrane DEAs under the same electric voltage.
However, there are still technical challenges in several aspects. In fabrication, multi-layered stacking for most silicone elastomers requires a complicated process, superposing each membrane DEA while suffering from low yield and non-uniformity of layers resulting from curing the liquid resin cast. Operating voltage for the DEAs is also limited due to electro-mechanical instability (EMI) impeding recovery from a deformed state, electrical safety for human contact, and the necessity of a compact power source for miniaturization of the control system. Particularly, for practical use in the fields of robotics, tactile display, and human-assistive devices, the following aspects need to be considered further.
• Robotic kinematic application: DE muscles have been utilized to operate robotic systems. A robotic hand, where DE muscles move fingers through a pulley mechanism (
• Tactile/haptic display: Proposed tactile or haptic feedback devices include the force feedback glove (
• Bio-inspired robot: DE muscles are frequently used for soft robots, as their actuation resembles the motions of nature and animals. Several designs have been proposed, ranging from locomotion robots mimicking inchworms (
Statements
Data availability statement
The raw data supporting the conclusion of this article will be made available by the authors, without undue reservation.
Author contributions
SJ wrote the first draft of the manuscript, and HM, SY, and K-UK contributed to manuscript revision, read, and approved the submitted version.
Funding
This research was supported by the R&D Program through the Korea Creative Content Agency grant funded by the Ministry of Culture, Sports and Tourism in 2022 (R20201040018), by the R&D Program (2022R1A2B5B0200207411) of the National Research Foundation (NRF), Korea, and by the internal grant of Electronics and Telecommunications Research Institute (ETRI) [22YS1200, Development of light driven three-dimensional morphing technology for tangible visuo-haptic interaction].
Conflict of interest
The authors declare that the research was conducted in the absence of any commercial or financial relationships that could be construed as a potential conflict of interest.
Publisher’s note
All claims expressed in this article are solely those of the authors and do not necessarily represent those of their affiliated organizations, or those of the publisher, the editors and the reviewers. Any product that may be evaluated in this article, or claim that may be made by its manufacturer, is not guaranteed or endorsed by the publisher.
Supplementary material
The Supplementary Material for this article can be found online at: https://www.frontiersin.org/articles/10.3389/fbioe.2023.1006346/full#supplementary-material
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Summary
Keywords
dielectric elastomer, soft actuator, modeling, dynamic actuation, simulation
Citation
Jeong SM, Mun H, Yun S and Kyung K-U (2023) Modeling dynamic behavior of dielectric elastomer muscle for robotic applications. Front. Bioeng. Biotechnol. 11:1006346. doi: 10.3389/fbioe.2023.1006346
Received
29 July 2022
Accepted
30 January 2023
Published
10 February 2023
Volume
11 - 2023
Edited by
Hung-Yin Lin, National University of Kaohsiung, Taiwan
Reviewed by
Yifan Wang, Nanyang Technological University, Singapore
Raj Kumar Sahu, National Institute of Technology Raipur, India
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Copyright
© 2023 Jeong, Mun, Yun and Kyung.
This is an open-access article distributed under the terms of the Creative Commons Attribution License (CC BY). The use, distribution or reproduction in other forums is permitted, provided the original author(s) and the copyright owner(s) are credited and that the original publication in this journal is cited, in accordance with accepted academic practice. No use, distribution or reproduction is permitted which does not comply with these terms.
*Correspondence: Ki-Uk Kyung, kyungku@kaist.ac.kr
This article was submitted to Bionics and Biomimetics, a section of the journal Frontiers in Bioengineering and Biotechnology
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