REVIEW article

Front. Microbiol., 04 December 2018

Sec. Food Microbiology

Volume 9 - 2018 | https://doi.org/10.3389/fmicb.2018.02745

Chitosan, a Biopolymer With Triple Action on Postharvest Decay of Fruit and Vegetables: Eliciting, Antimicrobial and Film-Forming Properties

  • 1. Department of Agricultural, Food and Environmental Sciences, Marche Polytechnic University, Ancona, Italy

  • 2. Department of Crop Sciences, Postharvest Technology Group, Tshwane University of Technology, Pretoria, South Africa

Abstract

Chitosan is a natural biopolymer from crab shells that is known for its biocompatibility, biodegradability, and bioactivity. In human medicine, chitosan is used as a stabilizer for active ingredients in tablets, and is popular in slimming diets. Due to its low toxicity, it was the first basic substance approved by the European Union for plant protection (Reg. EU 2014/563), for both organic agriculture and integrated pest management. When applied to plants, chitosan shows triple activity: (i) elicitation of host defenses; (ii) antimicrobial activity; and (iii) film formation on the treated surface. The eliciting activity of chitosan has been studied since the 1990’s, which started with monitoring of enzyme activities linked to defense mechanisms (e.g., chitinase, β-1,3 glucanase, phenylalanine ammonia-lyase) in different fruit (e.g., strawberry, other berries, citrus fruit, table grapes). This continued with investigations with qRT-PCR (Quantitative Real-Time Polymerase Chain Reaction), and more recently, with RNA-Seq. The antimicrobial activity of chitosan against a wide range of plant pathogens has been confirmed through many in-vitro and in-vivo studies. Once applied to a plant surface (e.g., dipping, spraying), chitosan forms an edible coating, the properties of which (e.g., thickness, viscosity, gas and water permeability) depend on the acid in which it is dissolved. Based on data in literature, we propose that overall, the eliciting represents 30 to 40% of the chitosan activity, its antimicrobial activity 35 to 45%, and its film-forming activity 20 to 30%, in terms of its effectiveness in the control of postharvest decay of fresh fruit. As well as being used alone, chitosan can be applied together with many other alternatives to synthetic fungicides, to boost its eliciting, antimicrobial and film-forming properties, with additive, and at times synergistic, interactions. Several commercial chitosan formulations are available as biopesticides, with their effectiveness due to the integrated combination of these three mechanisms of action of chitosan.

Introduction

Chitosan is the linear polysaccharide of glucosamine and N-acetylglucosamine units joined by β-1,4-glycosidic links and it is obtained by deacetilation of chitin through exposure to NaOH solutions or to the enzyme chitinase. Chitosan and chitin are naturally occurring polymers. For their biocompatibility and biosafety, their applications are widespread in many industries, such as cosmetology, food, biotechnology, pharmacology, medicine, and agriculture (Ding et al., 2013; Lei et al., 2014). In particular, chitosan has increasing interest in plant protection as a natural fungicide and plant defense booster, and meets the interest of many researchers, that used it to prolong the storage of an array of fruit and vegetables worldwide. Chitosan was the first compound in the list of basic substances approved in the European Union for plant protection purposes (Reg. EU 66 2014/563), for both organic agriculture and integrated pest management. A comprehensive review on the available data on the effectiveness of chitosan was published recently, for its preservation of fruit and vegetables, both alone and in combination with other treatments, and its mechanisms of action (Romanazzi et al., 2017). However, the increasing knowledge of this biopolymer (Figure 1) and the fast advances in basic and applied research in this field require a more focused and schematic update based on the last 5 years of investigations (2013–2018). The reader can then focus on specific aspects from the long list of other reviews that have appeared on the subject, among which some have focused on the applications of chitosan to fruit and vegetables (Bautista-Baňos et al., 2006; Bautista-Baòos et al., 2016; Zhang et al., 2011). When applied to plants, chitosan shows triple activity: (i) elicitation of host defenses; (ii) antimicrobial activity; and (iii) film formation on the treated surface. We will cover the recent information on these issues in the following sections, which is also listed comprehensively in the Tables, with examples of these applications.

FIGURE 1

Effectiveness of Chitosan in the Control of Postharvest Decay of Fruit

The potential effectiveness of chitosan as a coating for fresh fruit was first proposed by Muzzarelli (1986). The first in-vivo application of chitosan on fruit was in the Josep Arul Laboratory, by Ahmed El Ghaouth, who produced a list of papers through the last decade of the last century. These included El Ghaouth et al. (1992), where they applied chitosan to strawberries and other fruit, both alone and in combinations with other potential biocontrol agents, which then contributed to the develop of some commercial formulations. Following these promising investigations, and with the growing need for alternatives to the use of synthetic fungicides, chitosan use became popular, and it was proposed to be part of a new class of plant protectants (Bautista-Baňos et al., 2006). Chitosan coatings have now been applied to numerous temperate and subtropical fruit, both alone and in combination with other treatments (Tables 13), with generally additive, and in some cases synergistic, effectiveness (Romanazzi et al., 2012).

Table 1

FruitDecay agentCombination with chitosanReference
Table grapesBotrytis cinereaSalicylic acidShen and Yang, 2017
General decayGlucose complexGao et al., 2013
Aspergillus niger, Rhizopus stoloniferde Oliveira et al., 2014
Fusarium oxysporumIrkin and Guldas, 2014
General decayFeliziani et al., 2013a
General decayUltraviolet-CFreitas et al., 2015
General decayAl-Qurashi and Mohamed, 2015
Aspergillus niger, Botrytis cinerea, Penicillium expansum, Rhizopus stoloniferMenta essential oilGuerra et al., 2016
Botrytis cinereaSalvia officinalis essential oilKanetis et al., 2017
StrawberryBotrytis cinereaLavander and thyme essential oilSangsuwan et al., 2016
General decayPoeny extractPagliarulo et al., 2016
Penicillium expansum, Rhizopus stoloniferOlive oil processing wasteKhalifa et al., 2016
Total microbial loadNatamycin, nisin, pomegranate, grape seed extractDuran et al., 2016
Total microbial loadQuinoa protein-chitosan and quinoa protein-chitosan-sunflower oilValenzuela et al., 2015
Total microbial loadSodium benzoate and potassium sorbateTreviño-Garza et al., 2015
Botrytis cinereaZataria multiflora essential oilMohammadi et al., 2015
Rhizopus stoloniferCinnamon leaf essential oil containing oleic acidPerdones et al., 2014
General decayBenhabiles et al., 2013
General decayGeraniol and thymolBadawy et al., 2017
General decayCarboxymethyl cellulose, hydroxypropylmethyl celluloseGol et al., 2013
Botrytis cinereaNanosized silver-chitosan compositeMoussa et al., 2013
General decayBeeswaxVelickova et al., 2013
Botryosphaeria sp.Wang et al., 2017
PearGeneral decayCellulose nanocrystalsDeng et al., 2017
General decayAcylated soy protein isolate and stearic acidWu et al., 2017
AppleGeneral decayOlive waste extractsKhalifa et al., 2017, 2016
Penicillium expansumDarolt et al., 2016
Venturia inaequalisFelipini et al., 2016
Penicillium expansumLi et al., 2015
Calyx senescenceVDeng et al., 2016
CitrusPenicillium digitatum, Penicillium italicumSilver nanoparticlesAl-Sheikh and Yehia, 2016
Colletotrichum gloeosporioidesPichia membranaefaciensZhou et al., 2016
Penicillium digitatum, Penicillium italicumCress and/or pomegranate extractsTayel et al., 2016
Penicillium digitatumClove oilShao et al., 2015
Penicillium digitatumCyclic lipopeptide antibiotics from Bacillus subtilisWaewthongrak et al., 2015
General decayCarboxymethyl celluloseArnon et al., 2014
Total microbial loadSilver and zinc oxide nanoparticlesKaur et al., 2017
PeachMonilinia laxaPolyethylene terephthalate punnets containing thyme oil and sealed with chitosan/boehmite nanocomposite lidding filmsCindi et al., 2015
General decayγ-rayElbarbary and Mostafa, 2014
Monilinia fructicolaMa et al., 2013
Monilinia laxa, Botrytis cinerea, Rhizopus stoloniferFeliziani et al., 2013b
Sweet cherryGeneral decayPasquariello et al., 2015
Hydroxypropyl methylcelluloseShanmuga Priya et al., 2014
PlumGeneral decayAscorbic acidLiu et al., 2014

Postharvest chitosan treatments with other applications for storage decay of temperate fruit.

Table 2

FruitDecay agentCombination with chitosanReference
MangoAnthracnose (Colletotrichum gloeosporioides)SpermidineJongsri et al., 2017
Anthracnose (Colletotrichum gloeosporioides), stem-end rot (L. theobromae strains)Lactoperoxidase system incorporated chitosan filmsKouakou et al., 2013
AnthracnoseMentha piperita L. essential oilde Oliveira et al., 2017
Anthracnose (Colletotrichum gloeosporioides), stem-end rot (L. theobromae strains)Lactoperoxidase system incorporated chitosan filmsKouakou et al., 2013
AnthrcanoseMentha piperita L. essential oilde Oliveira et al., 2017
CitrusGreen mold (Penicillium digitatum)Bacillus subtilis ABS-S14Waewthongrak et al., 2015
Anthracnose (Colletotrichum gloeosporioides)Pichia membranifaciensZhou et al., 2016
AvocadoAnthracnose (Colletotrichum gloeosporioides)Thyme oilBill et al., 2014
TomatoAlternaria alternataMethyl jasmonateChen et al., 2014
Aspergillus niger, Rhizopus stoloniferEssential oil from Origanum vulgare LBarreto et al., 2016
PomegranatePenicillium spp., Pilidiella granatiLemongrass filmMunhuweyi et al., 2017

Postharvest chitosan treatments with other applications for storage decay of subtropical fruit.

Table 3

FruitDecayCombination with chitosanReference
CitrusPenicillium digitatumRhodosporidium paludigenumLu et al., 2014
PeachGeneral decayCalcium chlorideGayed et al., 2017
Jujube fruitAlternaria alternata
Table grapesBotrytis cinereaSalicylic acidShen and Yang, 2017
Botrytis cinereaFeliziani et al., 2013a
StrawberryBotrytis cinerea and Rhizopus stoloniferRomanazzi et al., 2013; Feliziani et al., 2015
Botrytis cinereaLopes et al., 2014
General decaySaavedra et al., 2016
Sweet cherryMonilinia laxa, Botrytis cinerea, and Rhizopus stoloniferFeliziani et al., 2013a

Preharvest chitosan treatments with other applications for storage decay of temperate fruit.

Chitosan Eliciting Activity

Chitosan is known to elicit plant defences against several classes of pathogens, including fungi, viruses, bacteria and phytoplasma (El Hadrami et al., 2010). Moreover, in some studies, its eliciting activity was reported to be effective on pests (Badawy and Rabea, 2016). Based on our experience, the eliciting activity of chitosan accounts for 30 to 40% of its effectiveness in the control of postharvest decay of fresh fruit (Figure 2). The extent of this eliciting activity depends on the reactivity of the fruit tissues, and it is well known that fruit responses to stress decline with ripening (Romanazzi et al., 2016). This eliciting activity of chitosan has been studied since the 1990’s, which started with monitoring of the activities of enzymes linked to the defense mechanisms (e.g., chitinase) in different fruit (e.g., strawberries) (El Ghaouth et al., 1992). This was followed by investigations on other berries, citrus fruit and table grapes, among others. More recently, tools such as qRT-PCR and in recent years RNA-Seq (RNA-Sequencing) have allowed important information to be gained, first at the level of single gene expression, and then later at the level of global gene expression (Xoca-Orozco et al., 2017). This has provided good understanding of the multiple actions of chitosan applications and how they affect a number of physiological changes in fruit. As an example, the application of chitosan to strawberries at different times before harvest can affect the expression of a thousand or more genes (Landi et al., 2017). Some examples that have become available in the literature over the last 5 years are listed in Table 4, which deal with the physiological changes that can occur in chitosan-treated fruit, both when the biopolymer is applied alone, and when it is combined with other treatments. The eliciting activity of chitosan is particularly effective toward latent infections, as a more reactive fruit can stop the infection process, through a balance that resembles quorum sensing, which is well known for bacterial infections (Papenfort and Bassler, 2016).

FIGURE 2

Table 4

FruitPhysiological changeCombination with chitosanReference
Apple20 genes involved in defence responses, metabolism, signal transduction, transcription factors, protein biosynthesis, cytoskeleton.Li et al., 2015
Total phenolic, flavonoids, antioxidants, pigments, weight lossOlive waste extractKhalifa et al., 2017
PeachMalondialdehyde contentγ-rayElbarbary and Mostafa, 2014
Catalase, peroxidase, β-1,3-glucanase and chitinaseMa et al., 2013
Total soluble solids, weight loss, ascorbic acid contentSilver and zinc oxide nanoparticlesKaur et al., 2017
Color and fruit firmnessPolyethylene terephthalate punnets containing thyme oil and sealed with chitosan/boehmite nanocomposite lidding filmsCindi et al., 2015
Fruit firmness, weight loss, total soluble solids, total phenolic content, and titratable acidityCalcium chlorideGayed et al., 2017
PlumFruit firmness, respiration rate, fruit color, polygalacturonase, superoxide dismutase, peroxidase, catalase, polyphenol oxidase, phenylalanine ammonia lyase and pectin methylesterase activities, superoxide free radicals, malondialdehyde contentAscorbic acidLiu et al., 2014
Sweet cherryMalondialdehyde content and superoxide dismutase, catalase, ascorbate peroxidase, polyphenol oxidase, guaiacol peroxidase lipoxygenase activitiesPasquariello et al., 2015
StrawberryOver 5000 differently expressed genesLandi et al., 2017
18 defence genesLandi et al., 2014
Fruit colorFeliziani et al., 2015
Fruit firmness, anthocyanin and total phenol contentSaavedra et al., 2016
Weight loss, titratable acidity, pH, total soluble solids, total phenols, anthocyanin and ascorbic acid content, activity of polygalacturonase, pectin methyl esterase, β-galactosidase and celluloseCarboxymethyl cellulose, hydroxypropylmethyl celluloseGol et al., 2013
Weight lossLavander and thyme essential oilSangsuwan et al., 2016
Titratable acidity, soluble solids contentBenhabiles et al., 2013
pH and soluble solids contentNatamycin, nisin, pomegranate, grape seed extractDuran et al., 2016
Weight loss, ascorbic acidPoeny extractPagliarulo et al., 2016
Weight loss, respiration rate, skin and flesh color, firmness, pH, titratable acidity, soluble solids content, reducing sugars contentBeeswaxVelickova et al., 2013
Weight loss, firmness, color and total soluble solids contentSodium benzoate, potassium sorbateTreviño-Garza et al., 2015
Weight losses, total soluble solids and titratable acidityOlive waste extractKhalifa et al., 2016
Allergen-related genePetriccione et al., 2017
Table grapesPhenylalanine ammonia lyase, chitinase, and β-1, 3-glucanase, phenolic compounds, respiration rate, weight loss, total soluble solids, titratable aciditySalicylic acidShen and Yang, 2017
Total phenols, flavonoids and ascorbic acid content, activities of peroxidase, polyphenoloxidase, polygalacturonase, and xylanase, fruit firmnessAl-Qurashi and Mohamed, 2015
Fruit colorIrkin and Guldas, 2014
Weight loss, titratable acidity, pH and soluble solids content, resveratrol contentUltraviolet-CFreitas et al., 2015
Weight loss, soluble solids content and titratable aciditySalvia officinalis essential oilKanetis et al., 2017
Firmness, titratable acidity, soluble solids, color, weight lossMenta essential oilGuerra et al., 2016
Total soluble solids, ascorbic acid content, titratable acidity, weight loss, respiration rate, activities of peroxidase and superoxide dismutaseGlucose complexGao et al., 2013
Titratable acidity, soluble solids, color, firmnessde Oliveira et al., 2014
Chitinase activity, quercetin, myricetin, and resveratrol contentFeliziani et al., 2013b
CitrusChitinase and phenylalanine ammonia lyaseLu et al., 2014
640 differentially expressed genes, many involved in secondary metabolism and hormone metabolism pathwaysCoqueiro et al., 2015
Fruit firmness, weight loss, total soluble solidsCarboxymethyl celluloseArnon et al., 2014
Peroxidase and phenylalanine ammonia-lyaseCyclic lipopeptide antibiotics from Bacillus subtilisWaewthongrak et al., 2015
Contents of chlorophylls and total carotenoids
Phenylalanine ammonia-lyase, β-1,3-glucanase, chitinase
JujubeFruit firmness, cellulase, pectinaseGuo et al., 2017
PearTotal phenolic and flavonoid contents, superoxide dismutase, peroxidase and catalase activities, total antioxidant activityCalcium chlorideKou et al., 2014a
Malic acid-metabolising enzymes and related genes expressionCalcium chlorideKou et al., 2014b
MangoPeroxidase (POD) and polyphenol oxidase (PPO) gene expressionGutierrez-Martinez et al., 2017
KiwifruitInduced gene expression and increased enzymatic activity of catalase, superoxide dismutase and ascorbate peroxidaseZheng et al., 2017

Physiological changes that can occur in fresh fruit after chitosan treatment, alone or in combination with other applications.

Chitosan Antimicrobial Activity

Numerous studies on chitosan inhibitory activities toward numerous microrganisms have been carried out since the first report of almost half a century ago (Allan and Hadwiger, 1979). The antimicrobial activities of chitosan against a wide range of plant pathogens have been confirmed by any of in-vitro and in-vivo studies. The antimicrobial activity of chitosan is one of its main properties, and this depends on the concentration at which it is applied. In the control of postharvest decay of fresh fruit, the antimicrobial activity can account for 35–45% of its effectiveness, as an antifungal barrier on a fruit inhibits the germination of fungal spores and slows down the rate of decay-causing fungi of already infected fruit, both latently and actively (Figure 2). A standard application rate of chitosan to provide a significant control of postharvest decay of fruit and vegetables can be considered 1%, except for the control of Penicillia, where higher concentrations may be needed to provide a good effectiveness. The degree of deacetylation and the molecular weight of chitosan characterize its properties, such as the number of positively charges of amino groups and therefore, its electrostatic interactions with different substrate and organisms at different pH. Chitosan with a higher degree of deacetylation, which has greater numbers of positive charges, would also be expected to have stronger antibacterial activities. On the other hand, numerous studies have generated different results relating to correlations between the chitosan bactericidal activities and its molecular weight (Romanazzi et al., 2017). In addition, there are many differences between the chitosan antifungal and antibacterial activities and several mechanisms relating to these remain still unclear and further researches are needed (Romanazzi et al., 2017).

Chitosan Film-Forming Properties

Once applied to a plant surface by dipping or spraying, chitosan can form an edible coating, the properties of which (e.g., thickness, viscosity, gas, and water permeability) greatly depend on the acid in which the biopolymer is dissolved. The film-forming properties of chitosan account for 20–30% of the chitosan effectiveness in the control of postharvest decay of fruit and vegetables (Figure 2). Coating produces a barrier for gas exchanges and reduced respiration, and slows down fruit ripening. Of note, a less ripe fruit is less sensitive to postharvest decay.

Toward Large-Scale Commercial Applications

When first used in experimental trials, chitosan needed to be dissolved in an acid (e.g., hydrochloric acid, acetic acid, which were among the most effective ones; see Romanazzi et al., 2009), and then taken to the optimal pH (∼5.6) This approach can even take 1–2 days, and it is impractical for use by growers. More recently, several commercial chitosan formulations that can be dissolved in water have become available on the market to be used as a biopesticides (Table 5). Some of these are formulated as powders, and then the cost of shipping is lower (although still higher compared to most of the commercially available synthetic fungicides), although the chitosan needs to be dissolved in water, in some cases a few hours before its application. This makes chitosan more difficult to use, as the grower wants to use an alternative to synthetic fungicides in the same way as a commercial compound, such that it should have the same effectiveness. This objective can be achieved with liquid formulations, which have concentrations of 2–15%. In this case, the cost of shipping is higher, as the volumes are larger due to the amounts of water that travel with the chitosan. In tests of three different commercial products, even when used at the same concentration, differential effectiveness was seen (Feliziani et al., 2013a). The higher cost of chitosan treatment compared to standard applications might also induce companies toward the use of low doses (e.g., even well below 0.1%), Based on data in literature, the optimal dose is around 1%, while decreasing the concentration, the effectiveness declines. Furthermore, when the concentration of chitosan is decreased, its effectiveness also declines. However, applications to the plant canopy also need to take in account possible phytotoxic effects, mainly if repeated applications occur. This has been shown for grapevines (Romanazzi et al., 2016a), such that for these purposes a good concentration might be 0.5%. However, under some particular conditions, even low concentrations of chitosan (e.g., 0.02%) in a commercial formulation can be beneficial, such as for the improved storage of litchi (Jiang et al., 2018).

Table 5

Product trade nameCompany (Country)FormulationActive ingredient (%)
Chito plantChiPro GmbH (Bremen, Germany)Powder99.9
Chito plantChiPro GmbH (Bremen, Germany)Liquid2.5
OII-YSVenture Innovations (Lafayette, LA, United States)Liquid5.8
KaitoSolAdvanced Green Nanotechnologies Sdn Bhd (Cambridge, United Kingdom)Liquid12.5
Armour-ZenBotry-Zen Limited (Dunedin, New Zealand)Liquid14.4
BiorendBioagro S.A. (Chile)Liquid1.25
KiforceAlba Milagro (Milan, Italy)Liquid6
FreshSealBASF Corporation (Mount Olive, NJ, United States)Liquid2.5
ChitoClearPrimex ehf (Siglufjordur, Iceland)Powder100
BioshieldSeafresh (Bangkok, Thailand)Powder100
Biochikol 020 PCGumitex (Lowics, Poland)Liquid2
KadozanLytone Enterprise, Inc. (Shanghai Branch, China)Liquid2
Kendal copsValagro (Atessa, Italy)Liquid4
Chitosan 87%Korea Chengcheng Chemical Company (China)TC (Technical material)87
Chitosan 2%Korea Chengcheng Chemical Company (China)SLX (Soluble concentrate)2

Some chitosan-based commercial products that are available for control of postharvest diseases of fruit and vegetables.

Concluding Remarks

The effectiveness of chitosan application arises from the integrated combination of its three mechanisms of action. There are increasing consumer requests for fruit and vegetables to be free from residues of synthetic pesticides, such that the rules defined by the public administration have become more limiting in terms of the active ingredients allowed and the maximum residue limits. Also, large stores compete with each other to further reduce these limits, compared to the legal thresholds (Romanazzi et al., 2016b). These trends make the concept of the application of alternatives to synthetic fungicides more popular, and among these the main one that is already used in human medicine is chitosan, which is particularly welcomed by public opinion. These aspects have promoted further studies based on the multiple actions of chitosan on fruit and vegetables. Therefore, further increases in our knowledge are expected following the widespread practical application of chitosan due to the regulation of its use in agriculture and the interest of companies to promote chitosan-based products, with potential benefits for the growers, the consumers and the environment.

Statements

Author contributions

GR proposed the review, collected data on chitosan popularity over time and on commercial products, coordinated the authors, and wrote the article. EF collected papers on effectiveness of chitosan on temperate fruit and on the mechanisms of action in the tables, and helped with the writing. DS collected papers on effectiveness of chitosan on tropical fruit and on the mechanisms of action in the tables, and helped with the writing.

Conflict of interest

The authors declare that the research was conducted in the absence of any commercial or financial relationships that could be construed as a potential conflict of interest.

References

  • 1

    AllanC. R.HadwigerL. A. (1979). The fungicidal effect of chitosan on fungi of varying cell wall composition.Exp. Mycol.3285287. 10.1016/S0147-5975(79)80054-7

  • 2

    Al-QurashiA. D.MohamedS. A. (2015). Postharvest chitosan treatment affects quality, antioxidant capacity, antioxidant compounds and enzymes activities of ‘El-Bayadi’ table grapes after storage.Sci. Hortic.197393398. 10.1016/j.scienta.2015.09.065

  • 3

    Al-SheikhH.YehiaR. S. S. (2016). In vitro antifungal efficacy of Aspergillus niger ATCC 9642 chitosan-AgNPs composite against post-harvest disease of citrus fruits.Appl. Biochem. Microbiol.52413420. 10.1134/S0003683816040177

  • 4

    ArnonH.ZaitsevY.PoratR.PoverenovE. (2014). Effects of carboxymethyl cellulose and chitosan bilayer edible coating on postharvest quality of citrus fruit.Postharv. Biol. Technol.872126. 10.1016/j.postharvbio.2013.08.007

  • 5

    BadawyM.RabeaI. (2016). “Chitosan and its derivatives as active ingredients against plant pests and diseases,” inChitosan in the Preservation of Agricultural Commodities, edsBautista-BaòosS.RomanazziG.Jiménez-AparicioA. (Amsterdam: Elsevier), 179219. 10.1016/B978-0-12-802735-6.00007-0

  • 6

    BadawyM. E. I.RabeaE. I.El-NoubyM. A. M.IsmailR. I. A.TaktakN. E. M. (2017). Strawberry shelf life, composition, and enzymes activity in response to edible chitosan coatings.Int. J. Fruit Sci.17117136. 10.1080/15538362.2016.1219290

  • 7

    BarretoT.AndradeS. C.MacielJ. F.ArcanjoN. M. O.MadrugaM. S.MeirelesB.et al (2016). A Chitosan coating containing essential oil from Origanum vulgare L. to control postharvest mold infections and keep the quality of cherry tomato fruit.Front. Microbiol.7:1724. 10.3389/fmicb.2016.01724

  • 8

    Bautista-BaòosS.Hernandez-LauzardoA. N.Velazquez-del ValleM. G.Hernandez-LopezM.Ait BarkaE.Bosquez-MolinaE.et al (2006). Chitosan as a potential natural compound to control pre and postharvest diseases of horticultural commodities.Crop Prot.25108118. 10.1016/j.cropro.2005.03.010

  • 9

    Bautista-BaòosS.RomanazziG.Jiménez-AparicioA.(eds) (2016). Chitosan in the Preservation of Agricultural Commodities.Amsterdam: Elsevier.

  • 10

    BenhabilesM. S.DrouicheN.LouniciH.PaussA.MameriN. (2013). Effect of shrimp chitosan coatings as affected by chitosan extraction processes on postharvest quality of strawberry.J. Food Meas. Charact.7215221. 10.1007/s11694-013-9159-y

  • 11

    BillM.SivakumarD.KorstenL.ThompsonA. K. (2014). The efficacy of combined application of edible coating and thyme oil in inducing resistance components in avocado (Persea americana Mill.) against anthracnose during post-harvest storage.Crop Prot.64159167. 10.1016/j.cropro.2014.06.015

  • 12

    ChenJ.ZouX.LiuQ.WangF.FengW.WanN. (2014). Combination effect of chitosan and methyl jasmonate on controlling Alternaria alternata and enhancing activity of cherry tomato fruit defence mechanisms.Crop Prot.563136. 10.1016/j.cropro.2013.10.007

  • 13

    CindiM. D.ShittuT.SivakumarD.Bautista-BañosS. (2015). Chitosan boehmite-alumina nanocomposite films and thyme oil vapour control brown rot in peaches (Prunus persica L.) during postharvest storage.Crop Prot.72127131. 10.1016/j.cropro.2015.03.011

  • 14

    CoqueiroD. S. O.de SouzaA. A.TakitaM. A.RodriguesC. M.KishiL. T.MachadoM. A. (2015). Transcriptional profile of sweet orange in response to chitosan and salicylic acid.BMC Genomics16:288. 10.1186/s12864-015-1440-5

  • 15

    DaroltJ. C.Rocha NetoA. C.Di PieroR. M. (2016). Effects of the protective, curative, and eradicative applications of chitosan against Penicillium expansum in apples.Braz. J. Microbiol.4710141019. 10.1016/j.bjm.2016.07.007

  • 16

    de OliveiraC. E. V.MagnaniM.de SalesC. V.de Souza PontesA. L.Campos-TakakiG. M.StamfordT. C. M.et al (2014). Effects of post-harvest treatment using chitosan from Mucor circinelloides on fungal pathogenicity and quality of table grapes during storage.Food Microbiol.44211219. 10.1016/j.fm.2014.06.007

  • 17

    de OliveiraK. ÁR.BergerL. R. R.de AraújoS. A.CamaraM. P. S.de SouzaE. L. (2017). Synergistic mixtures of chitosan and Menta piperita L. essential oil to inhibit Colletorichum species and anthracnose development in mango cultivar Tommy Atkins.Food Microbiol.6696103. 10.1016/j.fm.2017.04.012

  • 18

    DengL.YinB.YaoS.WangW.ZengK. (2016). Postharvest application of oligochitosan and chitosan reduces calyx alterations of citrus fruit induced by ethephon degreening treatment.J. Agric. Food Chem.6473947403. 10.1021/acs.jafc.6b02534

  • 19

    DengZ.JungJ.SimonsenJ.WangY.ZhaoY. (2017). Cellulose nanocrystal reinforced chitosan coatings for improving the storability of postharvest pears under both ambient and cold storages.J. Food Sci.82453462. 10.1111/1750-3841.13601

  • 20

    DingF.NieZ.DengH.XiaoL.DuY.ShiX. (2013). Antibacterial hydrogel coating by electrophoretic co-deposition of chitosan/alkynyl chitosan.Carbohydr. Polym.9815471552. 10.1016/j.carbpol.2013.07.042

  • 21

    DuranM.AdayM. S.ZorbaN. N. D.TemizkanR.BüyükcanM. B.CanerC. (2016). Potential of antimicrobial active packaging “containing natamycin, nisin, pomegranate and grape seed extract in chitosan coating” to extend shelf life of fresh strawberry.Food Bioprod. Process.98354363. 10.1016/j.fbp.2016.01.007

  • 22

    El GhaouthA.ArulJ.GrenierJ.AsselinA. (1992). Antifungal activity of chitosan on two postharvest pathogens of strawberry fruits.Phytopatology82398402. 10.1094/Phyto-82-398

  • 23

    El HadramiA.AdamL. R.El HadramiI.DaayfF. (2010). Chitosan in plant protection.Mar. Drugs8968987. 10.3390/md8040968

  • 24

    ElbarbaryA. M.MostafaT. B. (2014). Effect of γ-rays on carboxymethyl chitosan for use as antioxidant and preservative coating for peach fruit.Carbohydr. Polym.104109117. 10.1016/j.carbpol.2014.01.021

  • 25

    FelipiniR. B.BonetiJ. I.KatsurayamaY.NetoA. C. R.VeleirinhoB.MaraschinM.et al (2016). Apple scab control and activation of plant defence responses using potassium phosphite and chitosan.Eur. J. Plant Pathol.145929939. 10.1007/s10658-016-0881-2

  • 26

    FelizianiE.LandiL.RomanazziG. (2015). Preharvest treatments with chitosan and other alternatives to conventional fungicides to control postharvest decay of strawberry.Carbohydr. Polym.132111117. 10.1016/j.carbpol.2015.05.078

  • 27

    FelizianiE.RomanazziG.MargosanD. A.MansourM. F.SmilanickJ. L.GuS.et al (2013a). Preharvest fungicide, potassium sorbate, or chitosan use on quality and storage decay of table grapes.Plant Dis.97307314. 10.1094/pdis-12-11-1043-re

  • 28

    FelizianiE.SantiniM.LandiL.RomanazziG. (2013b). Pre- and postharvest treatment with alternatives to synthetic fungicides to control postharvest decay of sweet cherry.Postharv. Biol. Technol.78133138. 10.1016/j.postharvbio.2012.12.004

  • 29

    FreitasP. M.López-GálvezF.TudelaJ. A.GilM. I.AllendeA. (2015). Postharvest treatment of table grapes with ultraviolet-C and chitosan coating preserves quality and increases stilbene content.Postharv. Biol. Technol.1055157. 10.1016/j.postharvbio.2015.03.011

  • 30

    GaoP.ZhuZ.ZhangP. (2013). Effects of chitosan-glucose complex coating on postharvest quality and shelf life of table grapes.Carbohydr. Polym.95371378. 10.1016/j.carbpol.2013.03.029

  • 31

    GayedA. A. N. A.ShaarawiS. A. M. A.ElkhishenM. A.ElsherbiniN. R. M. (2017). Pre-harvest application of calcium chloride and chitosan on fruit quality and storability of “Early Swelling” peach during cold storage.Ciência Agrot.41220231. 10.1590/1413-70542017412005917

  • 32

    GolN. B.PatelP. R.RaoT. V. R. (2013). Improvement of quality and shelf-life of strawberries with edible coatings enriched with chitosan.Postharv. Biol. Technol.85185195. 10.1016/j.postharvbio.2013.06.008

  • 33

    GuerraI. C. D.De OliveiraP. D. L.SantosM. M. F.LúcioA. S. S. C.TavaresJ. F.Barbosa-FilhoJ. M.et al (2016). The effects of composite coatings containing chitosan and Mentha (piperita L. or x villosa Huds) essential oil on postharvest mold occurrence and quality of table grape cv. Isabella.Innov. Food Sci. Emerg. Technol.34112121. 10.1016/j.ifset.2016.01.008

  • 34

    GuoH.XingZ.YuQ.ZhaoY.ZhuE. (2017). Effectiveness of preharvest application of submicron chitosan dispersions for controlling Alternaria rot in postharvest jujube fruit.J. Phytopathol.165425431. 10.1111/jph.12576

  • 35

    Gutierrez-MartinezP.Bautista-BañosS.Berúmen-VarelaS.Ramos-GuerreroA.Hernández-IbaézA. M. (2017). In vitro response of Colletotrichum to chitosan. Effect on incidence and quality on tropical fruit. Enzymatic expression in mango.Acta Agron.62282289. 10.15446/acag.v66n2.53770

  • 36

    IrkinR.GuldasM. (2014). Chitosan coating of red table grapes and fresh-cut honey melons to inhibit Fusarium oxysporum growth.J. Food Process. Preserv.3819481956. 10.1111/jfpp.12170

  • 37

    JiangX.LinH.ShiJ.NeethirajanS.LinY.ChenY.et al (2018). Effects of a novel chitosan formulation treatment on quality attributes and storage behavior of harvested litchi fruit.Food Chem.252134141. 10.1016/j.foodchem.2018.01.095

  • 38

    JongsriP.RojsitthisakP.WangsomboondeeT.SeraypheapK. (2017). Influence of chitosan coating combined with spermidine on anthracnose disease and qualities of ‘Nam Dok Mai’ mango after harvest.Sci. Hortic.224180187. 10.1016/j.scienta.2017.06.011

  • 39

    KanetisL.ExarchouV.CharalambousZ.GoulasV. (2017). Edible coating composed of chitosan and Salvia fruticosa Mill. extract for the control of grey mould of table grapes.J. Sci. Food Agric.97452460. 10.1002/jsfa.7745

  • 40

    KaurM.KaliaA.ThakurA. (2017). Effect of biodegradable chitosan–rice-starch nanocomposite films on post-harvest quality of stored peach fruit.Starch69:1600208. 10.1002/star.201600208

  • 41

    KhalifaI.BarakatH.El-MansyH. A.SolimanS. A. (2016). Improving the shelf-life stability of apple and strawberry fruits applying chitosan-incorporated olive oil processing residues coating.Food Packag. Shelf Life91019. 10.1016/j.fpsl.2016.05.006

  • 42

    KhalifaI.BarakatH.El-MansyH. A.SolimanS. A. (2017). Preserving apple (Malus domestica var. Anna) fruit bioactive substances using olive wastes extract-chitosan film coating.Inform. Process. Agric.49099. 10.1016/j.inpa.2016.11.001

  • 43

    KouX. H.GuoW. L.GuoR. Z.LiX. Y.XueZ. H. (2014a). Effects of chitosan, calcium chloride, and pullulan coating treatments on antioxidant activity in Pear cv. “Huang guan” during storage.Food Bioprocess. Technol.7671681. 10.1007/s11947-013-1085-9

  • 44

    KouX. H.WangS.ZhangY.GuoR. Z.WuM. S.ChenQ.et al (2014b). Effects of chitosan and calcium chloride treatments on malic acid-metabolizing enzymes and the related gene expression in post-harvest pear cv. “Huang guan.”Sci. Hortic.165252259. 10.1016/j.scienta.2013.10.034

  • 45

    KouakouI. M.ClementineM.DidierM.GérardL.Ducamp-CollinM. N. (2013). Antimicrobial and physical properties of edible chitosan films enhanced by lactoperoxidase system.Food Hydrocoll.30576580. 10.1016/j.foodhyd.2012.07.018

  • 46

    LandiL.De Miccolis AngeliniR. M.PollastroS.FelizianiE.FaretraF.RomanazziG. (2017). Global transcriptome analysis and identification of differentially expressed genes in strawberry after preharvest application of benzothiadiazole and chitosan.Front. Plant Sci.8:235. 10.3389/fpls.2017.00235

  • 47

    LandiL.FelizianiE.RomanazziG. (2014). Expression of defense genes in strawberry fruits treated with different resistance inducers.J. Agric. Food Chem.6230473056. 10.1021/jf404423x

  • 48

    LeiJ.YangL.ZhanY.WangY.YeT.DengH.et al (2014). Plasma treated polyethylene terephthalate/polypropylene films assembled with chitosan and various preservatives for antimicrobial food packaging.Coll. Surf. Biointerfaces1146066. 10.1016/j.colsurfb.2013.09.052

  • 49

    LiH.WangY.LiuF.YangY.WuZ.CaiH.et al (2015). Effects of chitosan on control of postharvest blue mold decay of apple fruit and the possible mechanisms involved.Sci. Hortic.1867783. 10.1016/j.scienta.2015.02.014

  • 50

    LiuK.YuanC.ChenY.LiH.LiuJ. (2014). Combined effects of ascorbic acid and chitosan on the quality maintenance and shelf life of plums.Sci. Hortic.1764553. 10.1016/j.scienta.2014.06.027

  • 51

    LopesU. P.ZambolimL.CostaH.PereiraO. L.FingerF. L. (2014). Potassium silicate and chitosan application for gray mold management in strawberry during storage.Crop Prot.63103106. 10.1016/j.cropro.2014.05.013

  • 52

    LuL.LiuY.YangJ.AzatR.YuT.ZhengX. (2014). Quaternary chitosan oligomers enhance resistance and biocontrol efficacy of Rhodosporidium paludigenum to green mold in satsuma orange.Carbohydr. Polym.113174181. 10.1016/j.carbpol.2014.06.077

  • 53

    MaZ.YangL.YanH.KennedyJ. F.MengX. (2013). Chitosan and oligochitosan enhance the resistance of peach fruit to brown rot.Carbohydr. Polym.94272277. 10.1016/j.carbpol.2013.01.012

  • 54

    MohammadiA.HashemiM.HosseiniS. M. (2015). Nanoencapsulation of Zataria multiflora essential oil preparation and characterization with enhanced antifungal activity for controlling Botrytis cinerea, the causal agent of gray mould disease.Innov. Food Sci. Emerg. Technol.287380. 10.1016/j.ifset.2014.12.011

  • 55

    MoussaS. H.TayelA. A.AlsohimA. S.AbdallahR. R. (2013). Botryticidal activity of nanosized silver-chitosan composite and its application for the control of gray mold in strawberry.J. Food Sci.7815891594. 10.1111/1750-3841.12247

  • 56

    MunhuweyiK.OluwafemiJ. C.LennoxC. L.van ReenenA. J.OparaL. U. (2017). In vitro and in vivo antifungal activity of chitosan-essential oils against pomegranate fruit pathogens.Postharv. Biol. Technol.129922. 10.1016/j.postharvbio.2017.03.002

  • 57

    MuzzarelliR. A. A. (1986). “Filmogenic properties of chitin/chitosan,” inChitin in Nature and Technology, edsMuzzarelliR. A. A.JeuniauxC.GoodayG. W. (New York, NY: Plenum Press), 389396. 10.1007/978-1-4613-2167-5_48

  • 58

    PagliaruloC.SansoneF.MocciaS.RussoG. L.AquinoR. P.SalvatoreP.et al (2016). Preservation of strawberries with an antifungal edible coating using peony extracts in chitosan.Food Bioprocess. Technol.919511960. 10.1007/s11947-016-1779-x

  • 59

    PapenfortK.BasslerB. L. (2016). Quorum sensing signal–response systems in Gram-negative bacteria.Nat. Rev. Microbiol.14576588. 10.1038/nrmicro.2016.89

  • 60

    PasquarielloM. S.Di PatreD.MastrobuoniF.ZampellaL.ScortichiniM.PetriccioneM. (2015). Influence of postharvest chitosan treatment on enzymatic browning and antioxidant enzyme activity in sweet cherry fruit.Postharv. Biol. Technol.1094556. 10.1016/j.postharvbio.2015.06.007

  • 61

    PerdonesÁVargasM.AtarésL.ChiraltA. (2014). Physical, antioxidant and antimicrobial properties of chitosan-cinnamon leaf oil films as affected by oleic acid.Food Hydrocoll.36256264. 10.1016/j.foodhyd.2013.10.003

  • 62

    PetriccioneM.MastrobuoniF.ZampellaL.NobisE.CaprioloG.ScortichiniM. (2017). Effect of chitosan treatment on strawberry allergen-related gene expression during ripening stages.J. Food Sci. Technol.5413401345. 10.1007/s13197-017-2554-3

  • 63

    RomanazziG.FelizianiE.Bautista-BaòosS.SivakumarD. (2017). Shelf life extension of fresh fruit and vegetables by chitosan treatment.Crit. Rev. Food Sci. Nutr.57579601. 10.1080/10408398.2014.900474

  • 64

    RomanazziG.FelizianiE.SantiniM.LandiL. (2013). Effectiveness of postharvest treatment with chitosan and other resistance inducers in the control of storage decay of strawberry.Postharv. Biol. Technol.752427. 10.1016/j.postharvbio.2012.07.007

  • 65

    RomanazziG.LichterA.Mlikota GablerF.SmilanickJ. (2012). Recent advances on the use of natural and safe alternatives to conventional methods to control postharvest gray mold of table grapes.Postharv. Biol. Technol.63141147. 10.1016/j.postharvbio.2011.06.013

  • 66

    RomanazziG.Mlikota GablerF.MargosanD. A.MackeyB. E.SmilanickJ. L. (2009). Effect of chitosan dissolved in different acids on its ability to control postharvest gray mold of table grape.Phytopathology9910281036. 10.1094/PHYTO-99-9-1028

  • 67

    RomanazziG.SanzaniS. M.BiY.TianS.Gutierrez-MartinezP.AlkanN. (2016). Induced resistance to control postharvest decay of fruit and vegetables.Postharv. Biol. Technol.1228294. 10.1016/j.postharvbio.2016.08.003

  • 68

    RomanazziG.ManciniV.FelizianiE.ServiliA.EndeshawS.NeriD. (2016a). Impact of alternative fungicides on grape downy mildew control and vine growth and development.Plant Dis.100739748. 10.1094/PDIS-05-15-0564-RE

  • 69

    RomanazziG.SmilanickJ. L.FelizianiE.DrobyS. (2016b). Integrated management of postharvest gray mold on fruit crops.Postharv. Biol. Technol.1136976. 10.1016/j.postharvbio.2015.11.003

  • 70

    SaavedraG. M.FigueroaN. E.PobleteL. A.CherianS.FigueroaC. R. (2016). Effects of preharvest applications of methyl jasmonate and chitosan on postharvest decay, quality and chemical attributes of Fragaria chiloensis fruit.Food Chem.190448453. 10.1016/j.foodchem.2015.05.107

  • 71

    SangsuwanJ.PongsapakworawatT.BangmoP.SutthasupaS. (2016). Effect of chitosan beads incorporated with lavender or red thyme essential oils in inhibiting Botrytis cinerea and their application in strawberry packaging system.Food Sci. Technol.741420. 10.1016/j.lwt.2016.07.021

  • 72

    Shanmuga PriyaD.SuriyaprabhaR.YuvakkumarR.RajendranV. (2014). Chitosan-incorporated different nanocomposite HPMC films for food preservation.J. Nanopart. Res.16:2248. 10.1007/s11051-014-2248-y

  • 73

    ShaoX.CaoB.XuF.XieS.YuD.WangH. (2015). Effect of postharvest application of chitosan combined with clove oil against citrus green mold.Postharv. Biol. Technol.993743. 10.1016/j.postharvbio.2014.07.014

  • 74

    ShenY.YangH. (2017). Effect of preharvest chitosan-g-salicylic acid treatment on postharvest table grape quality, shelf life, and resistance to Botrytis cinerea-induced spoilage.Sci. Hortic.224367373. 10.1016/j.scienta.2017.06.046

  • 75

    TayelA. A.MoussaS. H.SalemM. F.MazrouK. E.El-TrasW. F. (2016). Control of citrus molds using bioactive coatings incorporated with fungal chitosan/plant extracts composite.J. Sci. Food Agric.9613061312. 10.1002/jsfa.7223

  • 76

    Treviño-GarzaM. Z.GarcíaS.Flores-GonzálezM.delS.Arévalo-NiñoK. (2015). Edible active coatings based on pectin, pullulan, and chitosan increase quality and shelf life of strawberries (Fragaria × ananassa).J. Food Sci.80M1823M1830. 10.1111/1750-3841.12938

  • 77

    ValenzuelaC.TapiaC.LópezL.BungerA.EscalonaV.AbugochL. (2015). Effect of edible quinoa protein-chitosan based films on refrigerated strawberry (Fragaria × ananassa) quality.Electron. J. Biotechnol.18406411. 10.1016/j.ejbt.2015.09.001

  • 78

    VelickovaE.WinkelhausenE.KuzmanovaS.AlvesV. D.Moldão-MartinsM. (2013). Impact of chitosan-beeswax edible coatings on the quality of fresh strawberries (Fragaria × ananassa cv Camarosa) under commercial storage conditions.Food Sci. Technol.528092. 10.1016/j.lwt.2013.02.004

  • 79

    WaewthongrakW.PisuchpenS.LeelasuphakulW. (2015). Effect of Bacillus subtilis and chitosan applications on green mould (Penicilium digitatum Sacc.) decay in citrus fruit.Postharv. Biol. Technol.994449. 10.1016/j.postharvestbio.2014.07.016

  • 80

    WangY.LiB.ZhangX.PengN.MeiY.LiangY. (2017). Low molecular weight chitosan is an effective antifungal agent against Botryosphaeria sp. and preservative agent for pear (Pyrus) fruits.Int. J. Biol. Macromol.9511351143. 10.1016/j.ijbiomac.2016.10.105

  • 81

    WuT.DaiS.CongX.LiuR.ZhangM. (2017). Succinylated soy protein film coating extended the shelf life of apple fruit.J. Food Process. Preserv.411302413034. 10.1111/jfpp.13024

  • 82

    Xoca-OrozcoL. A.Cuellar-TorresE. A.González-MoralesS.Gutiérrez-MartinezP.López-GarciaU.Herrera-EstrellaL.et al (2017). Transcriptomic analysis of avocado Hass (Persea americana Mill) in the interaction system fruit-chitosan- Colletotrichum.Front. Plant Sci.8:956. 10.3389/fpls.2017.00956

  • 83

    ZhangH.LiR.LiuW. (2011). Effects of chitin and its derivative chitosan on postharvest decay of fruits: a review.Int. J. Mol. Sci.12917934. 10.3390/ijms12020917

  • 84

    ZhengW.LiL.PanS.LiuM.ZhangW.LiuH.et al (2017). Controls postharvest decay and elicits defense response in kiwifruit.Food Bioprocess. Technol.1119371945. 10.1007/s11947-017-1957-5

  • 85

    ZhouY.ZhangL.ZengK. (2016). Efficacy of Pichia membranaefaciens combined with chitosan against Colletotrichum gloeosporioides in citrus fruits and possible modes of action.Biol. Control963947. 10.1016/j.biocontrol.2016.02.001

Summary

Keywords

antimicrobial activity, biopolymer, coating, induced resistance, natural fungicide

Citation

Romanazzi G, Feliziani E and Sivakumar D (2018) Chitosan, a Biopolymer With Triple Action on Postharvest Decay of Fruit and Vegetables: Eliciting, Antimicrobial and Film-Forming Properties. Front. Microbiol. 9:2745. doi: 10.3389/fmicb.2018.02745

Received

04 July 2018

Accepted

26 October 2018

Published

04 December 2018

Volume

9 - 2018

Edited by

Boqiang Li, Institute of Botany (CAS), China

Reviewed by

Xianghong Meng, Ocean University of China, China; Hongbing Deng, Wuhan University, China

Updates

Copyright

*Correspondence: Gianfranco Romanazzi,

This article was submitted to Food Microbiology, a section of the journal Frontiers in Microbiology

Disclaimer

All claims expressed in this article are solely those of the authors and do not necessarily represent those of their affiliated organizations, or those of the publisher, the editors and the reviewers. Any product that may be evaluated in this article or claim that may be made by its manufacturer is not guaranteed or endorsed by the publisher.

Outline

Figures

Cite article

Copy to clipboard


Export citation file


Share article

Article metrics