- 1Institut für Kernphysik, Technische Universität Darmstadt, Darmstadt, Germany
- 2Norwegian Nuclear Research Center and Department of Physics, University of Oslo, Oslo, Norway
- 3Research Center for Nuclear Physics, University of Osaka, Ibaraki, Japan
We review the experimental knowledge on the dipole polarizability (DP) of nuclei and its relation to the neutron skin thickness and properties of the neutron-rich matter equation of state (EOS). The discussion focuses on recent experiments using relativistic Coulomb excitation in inelastic proton scattering at extreme forward angles covering a mass range from 40Ca to 208Pb. Constraints on the neutron skins and the density dependence of the symmetry energy are derived from a systematic comparison to calculations based on density functional theory (DFT) and ab initio methods utilizing interactions derived from chiral effective field theory (
1 Introduction
The nuclear equation of state (EOS) describes the energy per nucleon of nuclear matter as a function of proton

Figure 1. (A) Predictions of the mass–radius relation of neutron stars from different EOS. Figure taken from [3]. (B) Theoretical constraints on the relation of
The nuclear matter EOS can be approximately written as a sum of the energy per nucleon of symmetric matter and an asymmetry term
where the nucleon density
The symmetry energy factor
Here,
The first term in Equation 1 representing symmetric nuclear matter is fairly well constrained by the compressibility derived from systematic measurements of the isoscalar giant monopole resonance (ISGMR) in nuclei [1]. Figures 1B,C [3, 10] illustrate the variety of experimental and theoretical constraints on
As detailed below, all relevant theoretical models predict a strong correlation between

Figure 2. Neutron and proton density distributions are schematically shown by the thick and thin solid lines, respectively. For a larger (smaller)
The neutron skin thickness is sensitive to the
The neutron skin thicknesses of medium-mass and heavy nuclei have been extracted from experiments studying elastic proton scattering [11], coherent
The dipole polarizability (DP) of nuclei can be obtained from measurements of the photoabsorption cross-sections. A connection between DP, neutron skin thickness, and parameters of the symmetry energy can only be made through models. Such calculations are presently based either on density functional theory (DFT) [20] or ab initio coupled-cluster calculations [21] using interactions derived from
While several experimental techniques to measure the DP are discussed, the present review mainly focuses on recent progress using relativistic Coulomb excitation in forward-angle proton scattering at energies of several hundred MeV [24]. One advantage of this method is consistent results across the neutron separation energy, while many of the other experimental techniques are limited to either the energy region below or above. Even more important, measurements of the
The paper is organized as follows. Section 2 discusses how information on the neutron skin thickness and symmetry energy can be inferred from model calculations based on DFT (Section 2.1) and ab initio methods (Section 2.2). Section 3 is devoted to experimental issues. A short discussion of the available techniques in Section 3.1 is followed by a description of methods to disentangle electric and magnetic contributions to the DP in Section 3.2. The relevance of experimental information in the energy region of the isovector giant dipole resonance (IVGDR), as well as below the neutron threshold and above the IVGDR, is compared in Section 3.3, Section 3.4, and Section 3.5. The comparison of experimental and theoretical results (Section 4) for a range of nuclei from 40Ca to 208Pb and constraints on neutron skin thickness and the parameters of the symmetry energy extracted thereof are presented in Section 4.1 for DFT and Section 4.2 for ab initio approaches. Section 4.3 focuses on the difficulties of simultaneously describing the results of parity-violating elastic electron scattering and DP experiments with present-day models. Finally, Section 4.4 discusses the systematics of the DP and the role of volume and surface contributions to the symmetry energy. A summary and an outlook are given in Section 5.
2 Relation between dipole polarizability, neutron skin thickness, and symmetry energy
In this section, we discuss how information on the neutron skin thickness and parameters of the symmetry energy can be inferred from the comparison of the experimental dipole polarizability to theoretical predictions. At the moment, there are two classes of models, based on either DFT or an ab initio coupled-cluster approach. Because isovector observables are not well constrained in DFT, quantitative predictions of the DP can vary considerably. However, one can establish a robust correlation between the parameters
The dipole polarizability
While the integral runs to infinity in principle, because of the inverse energy weighting a measurement of the
2.1 Connections in density functional theory
An approximately linear correlation between

Figure 3. (A) Correlation between the neutron skin thickness in 208Pb and
While this type of correlation is observed for all interactions, absolute values show large differences. In general, the magnitude of IV quantities like

Figure 4. (A) Dipole polarizability against neutron skin thickness in 208Pb Pb predicted by modern DFT interactions. (B) The same for dipole polarizability times symmetry energy at saturation density. The results are well described by a linear fit. Figures taken from [34], where the original references for the various interactions can be found.
2.2 Connections in ab initio models
Ab initio calculations based on interactions derived from

Figure 5. (A) Energy per particle in neutron matter (top row) and symmetric nuclear matter (bottom row) based on chiral interactions at
Predictions of
A major difference between the two theoretical approaches lies in the predicted relation between the proton and neutron radii. The DFT predictions of
3 Dipole polarizability from experiment
In this section, we discuss the experimental methods to extract the
3.1 Experimental methods
3.1.1 Photoneutron measurement
The photoexcitation of nuclei above the neutron separation energy was intensively studied by using photoneutron measurements. The photoneutron reaction is conventionally written as
Neutron emission is the dominant decay process after photoexcitation for a nucleus as heavy as 208

Figure 6. Comparison of the photoabsorption cross-sections of 208Pb from different experiments. Figure taken from [53], where the original references can be found.
Later, quasi-monoenergetic photon beams produced by laser Compton backscattering (LCBS) became available at the National Institute of Advanced Industrial Science and Technology (AIST) [54], the High Intensity
3.1.2 Total photoabsorption
Total photon absorption was studied by applying transmission measurements. In this method, the attenuation of photons in a thick target was measured as a function of the photon energy for extraction of the photoabsorption cross sections. At the Mainz electron accelerator, a narrow photon beam was produced by the bremsstrahlung of an electron beam. The average photon flux was
3.1.3 Compton scattering
Compton scattering from 208
3.1.4 Bremsstrahlung excitation functions
Photonuclear cross sections have been extracted from the radioactive decay of residual nuclei populated in particle emission after irradiation with thick-target bremsstrahlung. The excitation energy dependence can be determined by variation of the bremsstrahlung endpoint energy with an unfolding procedure [62]. However, this requires precise knowledge of the bremsstrahlung spectra, which is experimentally not available. While such spectra can be reliably calculated [63] with present-day Monte Carlo codes such as GEANT4 [64], older versions contained poor approximations [65]. Results deduced from phenomenological approximations or using the analytical description of thin-target bremsstrahlung have potentially very large systematic uncertainties, typically not included in the quoted errors.
3.1.5 Relativistic Coulomb excitation
Relativistic Coulomb excitation is an important experimental tool to study the electric dipole response at radioactive ion beam (RIB) facilities. At beam energies of several hundred MeV/nucleon, cross sections are large and cover an excitation energy range including the IVGDR. The small number of beam particles can be compensated for neutron-rich nuclei by placing a neutron detector under
The method has also been developed to study stable nuclei using inelastic proton scattering under extreme forward angles, including
3.1.6 Nuclear resonance fluorescence
Nuclear resonance fluorescence (NRF) or
3.2 Decomposition of and contributions
A general problem of all experimental methods discussed above is the removal of magnetic contributions to the photoabsorption cross sections and the derived DP. Overall, contributions of
No
In relativistic Coulomb excitation, the virtual photon spectrum in the forward direction is dominated by

Figure 7. (A) Top: Double differential cross sections of the 120Sn
An example of the MDA analysis is presented in Figure 7B for 40Ca [29]. Spectra at different scattering angles are displayed in the upper panel, demonstrating strongly forward-peaked cross sections in the energy region of the IVGDR expected for Coulomb excitation. The lower panel shows the partial contributions to the cross sections at the most forward angle measured resulting from the MDA:
3.3 Contributions from the IVGDR
The largest contribution to the DP stems from the IVGDR, whose energy centroids lie well above

Figure 8. Comparison of photoabsorption cross sections from different experiments. (A)
The
In general, studies of the
3.4 Contributions from the PDR
All particle-emission coincidence experiments accessing the
Most data on low-energy

Figure 9. (A) Comparison of
The origin of the low-energy
3.5 Contributions from high excitation energies
At excitation energies beyond the giant resonance region, photonuclear cross sections typically contribute a few percent only to the DP. However, for precision results, they must be considered. Data up to the pion threshold have been measured for a few cases, viz., natCa [58], natSn [104], and 208Pb [61, 51]. They show approximately constant cross sections as a function of excitation energy and were considered for the extraction of the DP from
The ratio of Coulomb excitation to quasifree cross sections in the
4 Extracting neutron skin thickness and symmetry energy properties from dipole polarizability data
In this section, we discuss constraints on the neutron skin thickness and symmetry energy properties derived from the comparison between model predictions and experimental studies of the DP. These refer to specific nuclei like 40Ca, 48Ca, and 208Pb but also systematic isotopic trends or a global mass dependence. The difficulties that presently available models have in simultaneously accounting for measured polarizabilities and asymmetries in parity-violating elastic electron scattering are illuminated.
4.1 Constraints based on density functional theory
The DPs of 40Ca and 48Ca have been studied in [29, 78], respectively. Figure 10A depicts their correlation and a comparison to selected DFT results. The four functionals are representative of widely used forms: non-relativistic Skyrme functionals SV [111] and RD [112] with different forms of density dependence, and relativistic functionals DD [113] with finite-range meson-exchange coupling and PC [114] with point coupling. All four have been calibrated to the same set of ground-state data to determine the model parameters.

Figure 10. (A) Correlation of the experimental DP of 40Ca and 48Ca (blue bands) in comparison with DFT calculations without (full ellipses) and with (dashed ellipses) inclusion of the experimental DP of 208Pb [36] in the parameter fit. (B)
The predictions are displayed as filled ellipses that represent the
The
A study of the DP in a long isotopic chain is particularly suited to investigate the connection with the neutron skin thickness. This can be best done in the Sn isotopes with neutron numbers between 50 and 82, where the proton shell closure stabilizes the g.s. deformation. There are many stable isotopes, and a study of the systematics of the DP was presented in [79]. The results are summarized in Figure 10C, which shows the evolution of
Roca-Maza et al. [106] combined the experimental DP data for 68Ni [26], 120Sn [30], and 208Pb [36] to test a large variety of density functionals. Because the DFT calculations do not include contributions from the quasi-deuteron process dominating the photoabsorption cross sections above the energy region of the IVGDR, these had to be removed for a comparison [106]. Figure 10D presents correlation plots between the experimental results and theoretical predictions from a wide range of DFT interactions. Only a handful (marked in red) are capable of simultaneously describing all three data points. Based on this reduced set, systematic predictions of
4.2 Constraints based on ab initio models
An experimental study of the DP in 48Ca [78] is of particular interest because it is accessible for both DFT and ab initio calculations, and a measurement of the neutron skin with parity-violating electron scattering is available [19]. The comparison is summarized in Figure 11A, where the blue band describes the experimental uncertainty. Ab initio results for the set of interactions from [38, 39] are displayed as green triangles, and a prediction from [40] based on a normalization to the 48Ca charge radius is displayed as a green bar. Results from the set of density functionals described in [40] are shown as red squares with some representative error bars, and the prediction from the analysis of [106] discussed above is shown as a black bar.

Figure 11. (A) Experimental DP in 48Ca (blue band) and predictions from ab initio results based on
The DFT results tend to be somewhat high compared to the experiment. The ab initio results show a significant dependence on the chosen interaction, but it can be well approximated by a linear dependence. In principle, this allows for the derivation of boundaries on the neutron skin thickness and the symmetry energy. However, while the ab initio results shown were truncated in the coupled-cluster expansion at the 2p-2h level, subsequent work [118] demonstrated that inclusion of 3p-3h correlations lowers the
As noted in Section 2.2, independent of the chosen interaction, a neutron skin thickness of approximately 0.14 fm is predicted for 48Ca, consistent with the value deduced from the measurement of the weak form factor [19]. The simultaneous description of the data in 40,48Ca and 68Ni implies that the underlying symmetry energy parameters are correct. A conservative estimate is provided by taking the full range of values from the set of ab initio interactions, viz.,
Recent work has, for the first time, been able to extend the range of ab initio DP calculations based on
4.3 Tension between polarizability and parity-violating elastic electron scattering in 208Pb
While in 48Ca there is fair agreement between the neutron skin thickness and symmetry energy properties derived from the different experiments, the parity-violating elastic electron scattering experiment on 208Pb [18] finds a much larger neutron skin
Because of the strong correlation between

Figure 12. (A) Experimental parity-violating asymmetry versus DP in 208Pb (gray bands) compared to calculations with a set of relativistic (red) and non-relativistic (green) DFT interactions. Sets with systematically varied symmetry energy
4.4 Volume and surface contributions to the symmetry energy
Another way of extracting properties of the symmetry energy is a study of the mass dependence of the DP. A simple power law

Figure 13. Experimental DP for a set of nuclei as a function of mass number (full squares). The green and blue lines are fits with the original Migdal model (Equations 1, 2) in [127]. The black lines are fits of Equation 5 allowing for a surface term of the symmetry energy, including (dashed-dotted) and excluding (full) the data point for 12C. The red line shows a fit with the prediction of [129] using the “
For masses
Here
5 Conclusion and outlook
We present a review of methods to measure the isovector
Constraints on the neutron skin thickness of nuclei and the parameters of the symmetry energy can be extracted from the strong correlations between these three quantities seen in all microscopic models. Results from nuclei covering a mass range between 40Ca and 208Pb consistently favor small neutron skins and a soft density dependence of the EOS around saturation density. In 208Pb serving as a benchmark for theory, this finding is at variance with the PREX results, while a similar study of 48Ca by the CREX collaboration conforms. The PREX result, hard to interpret in the framework of present theory, has led to an initiative (called Mainz radius experiment, or MREX) for a study with improved statistical and systematic errors at the new high-current Mainz energy-recovering superconducting accelerator (MESA) [132].
While the mass dependence of the DP is reasonably well-covered by the available data, future work should explore other degrees of freedom, such as the variation of neutron excess along isotopic chains and the role of deformation. The experimental uncertainties of the DP for key nuclei can be improved by the availability of independent measurements, as illustrated in Figure 6. New high-brilliance LCBS photon beam facilities are under construction at the Extreme Light Infrastructure–Nuclear Physics (ELI-NP) in Bucharest [133, 134] and the Shanghai Laser Electron Gamma Source (SLEGS) at the Shanghai Synchrotron Radiation Facility [135]. Combined with advanced techniques for neutron detection [136], these facilities promise a new quality of precision for
Major steps can be expected in the future at radioactive ion beam facilities, providing access to cases with much larger neutron excess than achievable for stable nuclei. Experimental tools for measuring relativistic Coulomb excitation in reverse kinematics are available, and pioneering studies of the dipole response in unstable nuclei have been performed at GSI [25, 26, 27]. First results for the neutron-rich isotope 52Ca investigated at RIKEN have been reported [137]. Because of the high energy/nucleon availability, future experiments at FAIR are particularly promising for research on the dipole polarizability of exotic neutron-rich nuclei [138].
Author contributions
PN-C: writing – original draft and writing – review and editing. AT: writing – original draft and writing – review and editing.
Funding
The author(s) declare that financial support was received for the research and/or publication of this article. This work was supported by the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) under Contract No. SFB 1245 (Project ID No. 79384907), by the Research Council of Norway through its grant to the Norwegian Nuclear Research Centre (Project No. 341985), by the JSPS KAKENHI Grant Number 25H00641, and by the Japan-South Africa Bilateral Funding Grant Number JPJSBP 120246502.
Acknowledgments
PvNC thanks the nuclear physics group at the University of Oslo for their kind hospitality during a stay where major parts of this work were done.
Conflict of interest
The authors declare that the research was conducted in the absence of any commercial or financial relationships that could be construed as a potential conflict of interest.
Generative AI statement
The author(s) declare that no Generative AI was used in the creation of this manuscript.
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Keywords: dipole polarizability, neutron skin thickness, symmetry energy, density functional theory, ab initio calculations
Citation: von Neumann-Cosel P and Tamii A (2025) Electric dipole polarizability constraints on neutron skin and symmetry energy. Front. Phys. 13:1629987. doi: 10.3389/fphy.2025.1629987
Received: 16 May 2025; Accepted: 16 June 2025;
Published: 22 August 2025.
Edited by:
Masayuki Matsuzaki, Fukuoka University of Education, JapanReviewed by:
Shuichiro Ebata, Saitama University, JapanPraveen C Srivastava, Indian Institute of Technology Roorkee, India
Copyright © 2025 von Neumann-Cosel and Tamii. This is an open-access article distributed under the terms of the Creative Commons Attribution License (CC BY). The use, distribution or reproduction in other forums is permitted, provided the original author(s) and the copyright owner(s) are credited and that the original publication in this journal is cited, in accordance with accepted academic practice. No use, distribution or reproduction is permitted which does not comply with these terms.
*Correspondence: Peter von Neumann-Cosel, dm5jQGlrcC50dS1kYXJtc3RhZHQuZGU=