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ORIGINAL RESEARCH article

Front. Phys.

Sec. Optics and Photonics

Volume 13 - 2025 | doi: 10.3389/fphy.2025.1666117

Enhancing Methane Detection Limit of OA-ICOS: A Combined Approach of White Noise Perturbation and Savitzky-Golay Filtering

Provisionally accepted
Ce  YangCe Yang1Zongheng  ChenZongheng Chen1*Chen  ChenChen Chen2*Chunguang  LiChunguang Li2Siqing  LiuSiqing Liu1Jianyu  HuangJianyu Huang1Yu  LiYu Li1Laiyong  SongLaiyong Song1Hongbin  LiHongbin Li1
  • 1Guangzhou Marine Geological Survey, Guangzhou, China
  • 2Jilin University, Changchun, China

The final, formatted version of the article will be published soon.

In the context of global clean energy demand and climate change, the dynamic monitoring of methane is crucial for carbon cycle research and greenhouse gas assessment. In order to solve the problem of cavity mode noise limiting measurement performance in the off-axis integrated cavity output spectroscopy (OA-ICOS) system, an optimization method based on white noise injection was proposed. A broadband white noise perturbation is introduced into the distributed feedback (DFB) laser, and the Savitzky-Golay (S-G) filtering algorithm is used to further reduce the noise. It effectively suppresses the coherence of cavity mode noise, reduces the noise floor, and improves the signal-to-noise ratio and measurement sensitivity of the system. Experiments show that when white noise with a modulation depth of 30% is injected, the signal-to-noise ratio of the system is increased by about 3.16 times, and the methane measurement limit is optimized from 5.32 ppm to 2.22 ppm of the original system, which is about 2.4 times. The Allan deviation showed a significant increase in minimum detectable limit. Further verification by methane dynamic test shows that the system response time is about 1 minute, showing reliable measurement stability. This study provides an innovative technical solution for high-precision methane measurement, which is of great significance for promoting in-situ greenhouse gas monitoring and climate model optimization.

Keywords: Methane measurement, OA-ICOS, White noise perturbation, Savitzky-Golay filtering, enhancingmeasurement limit, Cavity mode noise

Received: 15 Jul 2025; Accepted: 04 Sep 2025.

Copyright: © 2025 Yang, Chen, Chen, Li, Liu, Huang, Li, Song and Li. This is an open-access article distributed under the terms of the Creative Commons Attribution License (CC BY). The use, distribution or reproduction in other forums is permitted, provided the original author(s) or licensor are credited and that the original publication in this journal is cited, in accordance with accepted academic practice. No use, distribution or reproduction is permitted which does not comply with these terms.

* Correspondence:
Zongheng Chen, Guangzhou Marine Geological Survey, Guangzhou, China
Chen Chen, Jilin University, Changchun, China

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