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ORIGINAL RESEARCH article

Front. Phys., 25 November 2025

Sec. Nuclear Physics​

Volume 13 - 2025 | https://doi.org/10.3389/fphy.2025.1688864

Estimation of the effect of Tsallis non-extensive statistics on the 14C(n,γ)15C reaction rate

  • 1Department of Science, Eurasian Technological University, Almaty, Kazakhstan
  • 2Faculty of Physics and Technology, Al-Farabi Kazakh National University, Almaty, Kazakhstan

The total cross-section of the radiative neutron capture reaction 14С(n0+1)15C—for energies ranging from 10 meV to 5 MeV—is considered. Calculations performed in the framework of the modified potential cluster model with forbidden states show an agreement of total cross-section σ (23.3 keV) = 4.75 μb with the presently recommended value 4.86(48) μb by Ma et al., 2020. The efficiency of carbon isotope 15C production is illustrated by the 14С(n0+1)15C reaction rate calculated at temperatures from T9 = 0.001 to T9 = 10. The conventional Maxwell–Boltzmann weighted reaction rate σvMB of the present work is comparable, with less than 10% accuracy, with the latest calculations by Ma et al., 2020 and Bhattacharyya et al., 2021. The estimation of non-extensive effects is implemented using our data on the reaction rate σvMB as reference values. The efficiency of carbon isotope production in radiative capture reactions 12-14С(n,γ)13-15C is estimated based on the calculated reaction rates. The influence of the Maxwellian-weighted 12-14C(n,γ)13-15C reaction rates on the ratios 12C/13C and 13C/14C is examined. Tsallis statistics is applied for the first time to the calculation of the 14С(n0)15C reaction rate with values of non-extensive parameter 0.7 ≤ q ≤ 1.3 on the background of Maxwell–Boltzmann statistics corresponding to q = 1. The reaction rate σvq shows a factor ∼4 increase for q = 0.7 and a factor ∼0.6 decrease for q = 1.3 compared to q = 1.

1 Introduction

The role of carbon isotope 14С in the stellar environment of asymptotic giant branch (AGB) stars was examined nearly 30 years ago by Forestini and Charbonnel, 1997, as part of research concerning the nucleosynthesis of light elements in low-metallicity intermediate-mass stars of 37M [1, 2]. We found it very interesting how the authors incorporated the isotope 14С into the scenario of AGB star evolution as some of their perspectives can now be validated with contemporary data. To reconstruct the AGB evolution, the network of neutron-, proton-, and 4He-induced reactions was considered on some selected nuclides, particularly 14С(n,γ), 14С(p,γ), 14С(α,γ), and 14С(α,n) processes, with 14С as the seed nucleus [1, 2]. The production of 14С is provided by two reactions: 13C(n,γ)14С and 14N(n,p)14C, so it is important to briefly discuss the status of these processes today.

The results of [1] are presented as an estimation of isotope abundance in carbon pockets:

C12/C13=44±3,C13/C14>1400,N14/N15>5300.(1)

These numbers turned out to be reference values, to some extent, for subsequent studies of AGB stars. Some original papers and reviews provide observables for the 12C/13C and 14N/15N ratios in AGB stars [36]. Note that ratios in Equation 1 strongly depend on the mutually connected reaction chains, such as neutron-induced reactions

Cn,γ12Cn,γ13Cn,γ14Cβ12N15,(2)

where the evolution of carbon isotopes 12-15C occurs, and finally nitrogen 15N is created. Hydrogen burning, 12-14C(p,γ)13-15N, is the source of nitrogen isotopes, providing the 14N/15N ratio while also regulating the carbon fractions. We are not concerned with the mechanism of 4He combustion since it mainly relates to the outer helium shell of AGB stars, which is beyond the scope of the present work.

We intend to discuss [5], purposely, the situation with the radiative neutron capture reaction 14С(n,γ)15C in the context of the following questions:

i. how reliable is the reaction rate determined today?;

ii. how may modern data on the reaction rate change the isotopic ratio (Equation 1)?;

iii. are there any reasons to shift from the traditional Maxwell–Boltzmann (MB) weighted reaction rate to non-extensive statistics?

While calculating the ratios (Equation 1), Forestini and Charbonnel, 1997 [1], used as input information for the constructed network the rate of the 14С(n,γ)15C reaction obtained in [7], which was nearly a factor of 5 lower than that of the earlier calculations in [8]. As a result, it was concluded that the reaction 14С(n,γ)15C(β)15N plays an insignificant role in the formation of 15N, with the process of radiative capture of protons 14С(p,γ)15N dominating.

This “factor of 5 difference” triggered, to some extent, the following year’s experimental study of the cross section of 14С(n,γ)15C reaction [912]. The value of the total cross section σ(E) at Ec.m.=23.3 keV is a benchmark today for comparing experimental methods and theoretical models. We suggest, for analysis, the set of results for σ23.3 keV from [7, 9, 1119, 49] and the recently published data by [20].

To determine the consistency of the results on the MB-weighted rate of the 14С(n,γ)15C reaction, we use data from [7, 8, 11, 18, 19] along with the present model calculations to address question (i). Since we employed the modified potential cluster model (MPCM) (see, for details, [21, 22]), the comparison of rates for the neutron-induced reactions 12-14С(n,γ)13-15C calculated within the same framework provides a way to re-estimate the 13C/14C ratio (ii).

Question (iii) is a new issue in the study of the 14С(n,γ)15C reaction. The subject of non-equilibrium phenomena in the context of stars is related to the application of non-extensive Tsallis statistics, as suggested in [23]. For the first time, [24] (final version, 2017 [25]), pointed out the strong sensitivity of thermonuclear reaction rates of light nuclei during Big Bang nucleosynthesis to the non-extensive parameter q. Further investigations concern the effect of Tsallis statistics on primordial BBN in the context of addressing the lithium problem [26, 27]. A summary of the research [24, 25] suggested extending the study of non-extensive effects to the formation of nuclei with masses beyond the BB seeds, i.e., with A>7. The authors foresee a possible new comprehension of the synthesis of heavy elements. In the present work, we applied the formalism of Tsallis statistics [24, 25] to illustrate its effect on the 14С(n,γ)15C reaction rate.

2 Elements of MPCM input data for the 14C(n0+1)15C reaction

The details of the study of the 14С(n0+1)15C reaction in the framework of the MPCM are presented in [28]. In this study, we still consider radiative E1 neutron capture on 14С, scattering p-waves to the ground state (GS) and first excited state (1st ES) of 15C, with respective quantum numbers P1/22+2P3/22S1/2 and P3/222D5/2. The interaction potential used for the calculation of continuum and bound states is of the Gauss type

Vr,JLS=V0JLSexpαJLSr2,(3)

where V0 is the potential depth and α is a parameter defining the asymptotic decrease in the potential at long relative distances r. Parameters V0 and α in Equation 3 are fitted for the bound states so that they match the channel binding energy Еb, charge radius Rch, and matter radius Rm. A set of parameters is found for each partial wave with quantum numbers JLS. The nodal or nodeless r-dependence of the relative wave functions is determined by the classification of orbital symmetry using Young diagrams, as implemented for the n+14C system in [28].

Another experimental characteristic is the asymptotic normalization coefficient ANC (ANC), which is related to the dimensional asymptotic constant C via the spectroscopic factor SF as follows: ANC2=SF×C2 [29]. We work in the formalism of the dimensionless asymptotic constant Cw, which is related to C by Cw=C/2ko, where the wave number k0 corresponds to the channel binding energy Eb=2ko2/2μ and μ is the reduced mass. The asymptotic constant Cw is determined by matching the numerical radial function to the analytical Whittaker function: χLr=2k0CwWηL+1/22k0r. In the case of neutron-induced reactions, η=0. The corresponding results are provided in Table 1.

Table 1
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Table 1. Parameters of the ground and excited state potential for 15C nucleus in the n14C channel and results of MPCM calculations of Еb, Rch, Rm, and Cw with the listed parameters V0 and α.

To calculate Rch(15C) and Rm(15C), we follow the definitions from [21]. The input numerical information includes the masses of the constituent particles, mn = 1.008665 amu and m14C = 14.003242 amu; the averaged value of Rch(14C) = 2.48 fm from [3032]; and the latest data for Rm(14C) = 2.367(35) fm from[33]. The recent experimental data on the ground state charge Rch and matter radius Rm for 15C, presented in Table 2, show good agreement with the MPCM results (see Table 1).

Table 2
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Table 2. Data on the experimentally measured charge radius Rch and matter radius Rm of 15C.

The results for Cw in Table 1 were obtained over the interval 7–27 fm. Selected later data on the ANC and their recalculated values for Cw, presented in Table 3, show reasonable agreement with the MPCM results for the GS, as well as for the first excited state.

Table 3
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Table 3. Asymptotic constant data for 15C in the n14C channel.

Initially, we proceeded from the data in work [37], where for the resonant states 2P1/2 at 3.103 MeV and 2P3/2 at 4.657 MeV, the reaction 14С(n,γ)15C does not occur, which means that these states are excited or formed in stripping or pickup reactions. In some studies, the narrow resonance at 3.103 MeV (Гn = 42 keV) is included in 14С(n,γ)15C cross-section calculations as a Breit–Wigner resonance; for example, see recent references [18, 20]. Their estimates show that its contribution is very small, even compared to the capture to the first excited state.

In the present study, we assume the 2P1/2 and 2P3/2 states to be non-resonant in the n + 14C channel. Since in the MPCM, the partial 2P waves do not contain forbidden states [22, 28], which are present in the spectrum of solutions of the Schrödinger equation only as bound states and require sufficiently deep attractive potentials [21], we assume the corresponding potentials to be zero.

Our choice of the zero depth for the P-wave scattering interaction potentials is supported by Ref. [16], where the role of different interaction parameters sets in the continuum n+14C channel is examined for the Coulomb breakup of 15C, and from these data the radiative capture 14С(n0)15C cross sections are recalculated.

3 Total cross sections of the n14C capture reaction

Comparison of the total cross sections for the 14С(n0+1)15C reaction, calculated using the MPCM potential parameters from Table 1, with experimental data is presented in Figure 1a. It is clearly observed that there is a noticeable input from the (n1) capture to the first ES starting from energies Ec.m.1 MeV.

Figure 1
Two graphs show nuclear reaction cross-sections for \(^{14}\text{C}(n, \gamma)^{15}\text{C}\) versus energy \(E_{c.m.}\). Both graphs include data points from various studies: Jiang et al. 2025, Nakamura et al. 2009, Reifarth et al. 2008, Horvath et al. 2002, and Beer et al. 1992. The left graph (a) presents \(E_{c.m.}\) from \(10^{-2}\) to 50 MeV with fitted lines for MPCM present work. The right graph (b) covers a broader energy range from \(10^{-8}\) to \(10^4\) MeV. Different fits and error bars indicate uncertainties and model comparisons.

Figure 1. Total cross sections of the 14С(n0+1)15C reaction. Experiment: www.frontiersin.org , [20]; www.frontiersin.org , [12]; www.frontiersin.org , [11]; www.frontiersin.org , [10]; www.frontiersin.org , [9]; www.frontiersin.org , [7]. Curves: MPCM calculations. (a) Ec.m. = 5 keV–5 MeV. (b) Ec.m. = 10−8–5 MeV; green dash-dotted curve–results of [28].

Note that the data by [12] are the result of a recalculation of the Coulomb breakup of 15C and corresponds to the photodisintegration reaction C15γ,n14C by virtual photons. When compared to direct photodisintegration by real γ-quanta, the results may differ. In general, it should be acknowledged that the measurement errors are very large, and all experimental points refer to the GS radiative capture 14С(n0)15C process.

Figure 1b illustrates the total cross sections for Ec.m. shows the results from our earlier work [28]. These cross sections are somewhat lower than the present cross sections since in [28], the radial matrix elements for the cross sections were calculated only up to 30 fm. Based on the low binding energy Eb of the n14C system, we have extended the integration interval for the overlapping integrals up to a distance of 100 fm.

The energy dependence of σ(Ec.m.) at Ec.m.10 keV (red solid curve in Figure 1b) can be approximated by the simple functional form:

σapμb=AEc.m.keV.(4)

The constant A = 1.002 μb·keV-1/2 in equation 4 is determined from a single point of σEc.m. at the minimum energy of 10 MeV. The value A=0.782μb·keV1/2 obtained earlier in [28] is approximately 20% lower. The accuracy of approximation (Equation 4) is estimated as ME=σapEσtheorE/σtheorE. The relative deviation of the calculated theoretical cross section σtheorE and its approximation σapE by the above function at energies less than 10 keV does not exceed 0.8%. Relation (Equation 4) allows determining the value of the thermal cross section: σth25.3  meV0.005μb.

The thermal cross section is too small to be measured; therefore, the available experimental value of σEc.m. at Ec.m.=23.3 keV is a benchmark for comparing different experimental methods and the results obtained from various theoretical models. The summary at σ23.3keV is presented in Table 4. We note the good agreement of our calculations with the data of [16], [18], [19], and with the evaluated values suggested as the presently recommended values.

Table 4
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Table 4. Comparison of the 14C neutron capture cross sections at Ec.m.=23.3 keV.

Figure 2 shows the neutron capture cross section divided by E1/2, i.e., SnE=σE/E. It should be noted that the theoretical calculations [13, 18] and the present MPCM results agree well. At an energy of 10−8 MeV, Sn(E) = 1.002 μb·keV-1/2 for the total cross section and Sn(E) = 0.949 μb·keV-1/2 for capture to the GS, corresponding to ∼95% dominance. The contribution of the first ES is ∼5% at low energies.

Figure 2
Graph showing the cross-section of the reaction \(^{14}\)C(n,γ)\(^{15}\)C as a function of center-of-mass energy (E\(_{c.m.}\)) in MeV. Data points from various studies are indicated by different symbols and colors. The main graph shows a range from \(10^{-8}\) to \(10^0\) MeV and \(10^{-2}\) to \(10^1\) μb keV\(^{-1/2}\). A smaller inset graph presents a zoomed section, comparing experimental data with theoretical models labeled

Figure 2. Total cross sections of the radiative n14С capture divided by E1/2. The inset shows the comparison of the theoretical calculations of [13, 18] and the MPCM results.

4 14C(n0+1)15C reaction rate

The astrophysical rate of the 14С(n0+1)15C reaction, calculated in MPCM, is shown in Figure 3. We approximated the MPCM reaction rates using an expression of the form T9=109K:

NAσv=a1/T92/3expa2/T91/31.0+a3T91/3+a4T92/3+a5T9+a6T94/3+a7T95/3+a8T9a9.(5)

Figure 3
Graph showing the reaction rates for the process \(^{14}\text{C}(n,\gamma)^{15}\text{C}\). The x-axis represents \(T_9\) (temperature in billions of Kelvins), and the y-axis shows the reaction rate \(N_A \langle \sigma v \rangle\) in cm\(^3\)mol\(^{-1}\)s\(^{-1}\). Two curves are displayed: a blue dashed line for GS and a solid red line for GS + 1st ES. An inset compares data from different studies: Reifarth et al. (2008), Ma et al. (2020), Bhattacharyya et al. (2021), and the present work.

Figure 3. Rate of the 14C(n,γ)15C reaction. MPCM reaction rates: red solid curve, –GS + first ES; blue dashed curve, GS. Inset: comparison of the reaction rates from [18] (dot magenta curve), [11] (dash-dot-dot blue curve), and [19] (dash-dot black curve) normalized to the MPCM rate.

Corresponding parameters ai for the GS and total reaction rates are provided in Table 5 according (Equation 5). The approximation yields χ2 = 0.0005 and χ2 = 0.0006, respectively, with an accuracy of 5% for the calculated reaction rates.

Table 5
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Table 5. Reaction rate approximation parameters for (Equation 5).

The inset in Figure 3 shows a comparison of present results and reaction rates calculated by [11], [18], and [19] normalized to the rate of the present work. The rate [18] based on the ANC formalism in the interval T9=0.0035 shows agreement with the MPCM rate within +5% on average, which is very close to that of [11]. The reaction rate in [19] derived from the Coulomb dissociation data is near ∼10% lower than the MPCM rate at the temperatures of T9=0.011. In summary, the results of the MPCM are in very good agreement with the modern data from [18, 19].

In Figure 3, we do not present the results from [20] directly, but we compare our reaction rate with the tabulated data of [20]. The authors note that their rate is ∼25% lower than that provided in [11] and ∼2.5–4 times higher than that provided in [7]. Comparison with our rate shows that our data exceeds the rate from [20] by a factor of 1.20. We may conclude that our results are more consistent with those reported in [11, 18, 19].

5 12-14C(n,γ)13-15C reaction rates and 12C/13C and 13C/14C ratios

Answer to question (i): The MPCM passed the cross-check; therefore, reliable data on the rate of the 14С(n0+1)15C reaction may be considered well determined today within ∼10% accuracy. This conclusion allows us to discuss possible corrections to the isotopic ratios 12C/13C, 13C/14C, and 14N/15N, following sequence 2 by comparing the early values from Ref. [1] (Equation 1) and addressing question (ii). The first observation concerns the near factor-of-5 difference in the reaction rates reported by [7] and [8], as shown in Figure 4. This difference changes the ratio C13/14C>1400 to C13/14C>280. Results obtained by Wiescher et al. 25 years ago have been confirmed today.

Figure 4
Log-log plot showing the nuclear reaction rate \(N_A\langle \sigma v \rangle \) in \(\text{cm}^3 \text{mol}^{-1} \text{s}^{-1}\) versus temperature \(T_9\). The red line represents MPCM, the green band shows Beer et al., 1992, and the blue band displays Wiescher et al., 1990. The reaction \(^{14}\text{C}(n,\gamma)^{15}\text{C}\) is labeled at the top.

Figure 4. Comparison of MPCM results with the modeless calculations implemented by [7] and [8].

Further changes in isotopic ratios may come from the results on reaction rates of the radiative neutron capture on carbon isotopes 12C(n,γ)13C [38] 13C(n,γ)14C [39], and 14C(n,γ)15C (present work) calculated in the same model—MPCM. These rates are shown in Figure 5.

Figure 5
Graph showing reaction rates as a function of temperature (T9). The x-axis represents temperature in units of T9 ranging from 0.01 to 10, and the y-axis shows reaction rates in cm^3 mol^-1 s^-1 from 10^1 to 10^5. Three curves are plotted: a blue curve (12C to 13C), a red curve (13C to 14C), and a green curve (14C to 15C). The graph highlights regions where specific reactions dominate, with labels indicating reactions.

Figure 5. Comparison of the astrophysical 12C(n0+1+2+3)13C [38], 13C(n0+1+2)14C [39], and 14C(n0+1)15C reaction rates in the range T9 = 0.01–10. Colored areas correspond to the interchange of the reaction rates (see comments in text).

Radiative neutron capture reactions may change the balance of 13C/14C as the ratio of reaction rates RC13/C14T9=σvC12n,γ13C/σvC13n,γ14C at temperatures T9=0.010.025 varies in the range of 2.9–3.2. These rates become equal at T90.2 RC13/C14=1, and then, up to T91.5, the production of 14C exceeds the creation of 13C (RC13/C140.5 at T91.1).

Comparison of 13C(n0+1+2)14C and 14C(n0+1)15C rates in Figure 5 shows the temperature intervals where slow production of 15C exceeds the creation of 14C. The low energy interval is T9 = 0.1–0.2, which refers to the equality of the corresponding reaction rates σvC13n,γ14C=σvC14n,γ15C with values of ≃ 290 and ≃ 620 cm3mol-1s-1 at the edges. At temperatures T9 ≳ 3, the rate of 15C production noticeably prevails over the rate of 14C formation. It is not meaningful to discuss the unobservable ratio of 14C/15C isotopes, but the relative enhancement in the 14C(n0+1)15C reaction rate may, to some extent, affect the nitrogen ratio 14N/15N.

The production of 14С in low-metallicity AGB stars is provided by two reactions: 13C(n,γ)14С and 14N(n,p)14C [40, 41]. Measurements by Wallner et al. [41] reported cross section at 23.3 keV σn,γ=6.7μb, σn,p=1.74 mb, and σn,p/σn,γ=260. The recent measurements of the Maxwellian averaged cross sections (MACS) derived from the n_TOF cross section reported the value σn,pMACS=1.77±0.04 mb [42] for the kT=25 keV, while the data from [41] are σn,pMACS=2.03±0.04 mb and σn,γMACS=20.6±2.7μb. Corresponding ratios σn,pMACS/ σn,γMACS are 98.5 and 86, respectively. The difference in MACS between Wallner et al. [41] and Torres et.al. [41] becomes noticeable for kT>15 keV and reaches a factor ∼3 at kT=100 keV.

In simpler terms, the ratio of these two reactions 13C(n,γ)14С and 14N(n,p)14C is approximately two orders of magnitude. Hence, the relative concentrations of accumulated nuclei 13C and 14N set the balance between these two reactions, which provides the abundance of 14C sufficient for a change in the elemental content of carbon pockets. Reaction 14N(n,p)14C changes the ratio 14N/15N, and at the same time, this ratio may be affected by increasing the number of 15N via the reaction С14n,γ15Cβ15N.

6 Rate of the 14C(n0)15C reaction with Tsallis statistics

It has been established that thermal pulses arise during the evolution of AGB stars and lead to temperature and density fluctuations in the convective envelope, which can locally disrupt the equilibrium particles’ velocity distribution [1, 2]. The Maxwell–Boltzmann distribution may also be violated due to turbulence and sudden energetic events, such as helium and hydrogen flashes. This provides the motivation for applying Tsallis statistics [2325], κ-distributions [4345], and superstatistics [46] when calculating nuclear reaction rates in AGB models.

The application of Tsallis statistics is our first step toward examining non-extensive effects in stellar plasma, for example, the 14С(n0)15C reaction, which may be incorporated into the analysis of the processes occurring in the carbon pockets of AGB stars [1, 4, 6]. The reason for applying Tsallis statistics concerns several aspects. The interpretation of non-extensive parameter q in the velocity distribution fq(v) is quite straightforward; i.e., in case, q > 1, the Maxwell–Boltzmann fMB(v) symmetric distribution is violated due to a damping in the number of particles with high energies, whereas case q < 1 implies an enhancement in the low energy component in the fq(v) distribution compared to the fMB(v). We also find that the Tsallis formalism is rather simple in application for calculating reaction rate integrals as it allows for convergent control of the results to those of the Maxwell–Boltzmann distribution.

Following [24] and [25], we recalculated the rate of the 14С(n,γ)15C reaction simulating the non-extensive effect of Tsallis statistics versus the Maxwell–Boltzmann by changing the velocity distribution from fMB(v) to fq(v). Explicit expressions and normalizing conditions for the velocity distributions of non-relativistic particles with an energy E=μv2/2 in the center-of-mass system are

fMBv=4πμ2πkT3/2eμv22kTv2,0fMBvdv=1,(6)
fqv=Bq4πμ2πkT321q1μv22kT1q1v2,fqqdv=1.(7)

Note that limq11q1EkT1q1=eEkT, so the case q=1 of the non-extensive parameter refers to the MB velocity distribution. Normalizing condition in Equation 7 allows us to calculate analytically the normalizing constants Bq and express them via the gamma-function Γz:

Bq=1q3/2Γ11qΓ11q32, if 13q<1,(8)
Bq=q13/21q1+321q1+12Γ1q1+12Γ1q1+1, if q>1.(9)

In the case of q<1, there is no limit of particles by the energy, i.e., Emax=. In the case of q>1, the kinetic energy is limited as Emax=kTq1, kT = 0.086173·T9 (MeV). In Table 6, a few values of Bq (Equations 8, 9) and Emax are presented.

Table 6
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Table 6. Normalizing constants Bq and values of Emax (for q>1).

The integral over the Maxwellian-weighted cross section (Equation 6) determines the reaction rate, which was derived in detail by Iliadis and is provided in a general form [47]:

NAσv=NA8πμ1/2kT3/20σEEexpEkTdE.(10)
Equation 10 along with substituted numerical values for the constants is expressed as:
NAσvMB=3.7313·104μ1/2T93/20σEEexp11.605E/T9dE.(11)

In the case of Tsallis statistics and following definition for fq(v) distribution (Equation 7), Equation 11 can be transformed to

NAσvq=Bq·3.7313·104μ1/2T93/20EmaxσEE1q1·11.605E/T91q1dE.(12)

In Figure 6 the results of the calculated σvq reaction rate of the radiative neutron capture to the GS of the 15C nucleus for the interval of non-extensive parameter 0.7q1.3 are presented. It is clear that the case q>1 corresponds to the inequality σvq<σvMB, which can be explained by looking at the Emax values of q in Table 6 and the energy dependence of the total cross section σE in Figure 1. Since no cut-off of integrand in Equation 12 in the case of q<1, the corresponding reaction rates are related as σvq>σvMB.

Figure 6
Graph showing nuclear reaction rates for \( {}^{14}\text{C}(n,\gamma_0){}^{15}\text{C} \) as a function of temperature \( T_9 \). It features three curves: red dashed line for \( q=0.7 \) (pink shading), black line for \( q=1 \), and blue dashed line for \( q=1.3 \) (blue shading). The x-axis ranges from \( 10^{-3} \) to \( 10^{1} \), and the y-axis from \( 10^{0} \) to \( 10^{4} \), measured in \( N_A \langle \sigma v \rangle_q \, \text{cm}^3\text{mol}^{-1}\text{s}^{-1} \).

Figure 6. Reaction rates calculated for the Tsallis statistics: q>1 – blue band, q<1 – red band relative to the Maxwellian-Boltzmann rate–black solid curve.

Figure 7 shows the numerical difference in reaction rates, considering the effect of the non-equilibrium Tsallis distribution compared to the MB distribution for 0.9q1.1. The difference in rates σvq/σvMB is ∼4%–35% increase for 0.99q1.1 and ∼4–20% decrease for 1.01q1.10. Figure 6 shows a factor ∼4 increase in σvq for q=0.7 and a factor ∼0.6 decrease for q=1.3.

Figure 7
Graph showing the ratio \(N_A\langle\sigma v\rangle_q / N_A\langle\sigma v\rangle_{MB}\) versus \(T_9\) on a logarithmic scale for \(^{14}C(n,\gamma_0)^{15}C\). Curves indicate varying \(q\) values: 0.9, 0.95, 0.99, 1.01, 1.05, and 1.10, demonstrating different behaviors as \(T_9\) increases.

Figure 7. Ratio of the Tsallis reaction rates to the Maxwell–Boltzmann rate.

In [20] Jiang et al., implemented the calculated 14С(n,γ)15C reaction rate σvMB for the estimation of the 15N abundance, which results in ∼20% increase of nitrogen-15 production, but only ∼0.2% impact on the final abundances of heavy elements with A > 90. As we mentioned above, the present σvMB rate for this reaction is ∼1.2 times higher than reported in [20]. If we assume the non-extensive parameter q = 0.7, the increasing factor for the reaction rate σvq is ∼5; therefore, 15N abundance may increase much higher than estimations based on the rate by Jiang et al., 2025. Note that the value q = 0.7 refers to a rather strong enhancement of the high-energy tails, which may arise from extreme events in the AGB environment.

Note that we have implemented a simplified calculation procedure, assuming that the effect of the center-of-mass correction, introduced by [26, 27], is not essential, as the seed nucleus 14C is much heavier than the light species with comparable masses involved at the stage of primordial BBN.

7 Conclusion

In summary, we show that the MPCM results on 14С(n0+1)15C are in good agreement with those reported in [18, 19]. Benchmark cross section σ23.3keV = 4.75 μb matches the presently recommended value 4.86(48) μb reported in [18]. The Maxwellian-weighted reaction rates calculated in the MPCM agree within ∼±10% deviations with the independent calculations of [8, 11, 18], and [19], therefore, the data on the MB rate of the 14C(n,γ)15C reaction can be considered well determined today.

The obtained values of reaction rates can be confidently conceived as the reference ones for the re-estimation of 12C/13C, 13C/14C, and 14N/15N via the neutron-induced reactions 12C(n0+1+2+3)13C, 13C(n0+1+2)14C, and 14C(n0+1)15C calculated in MPCM. We determined the temperature windows where the interchange of reaction rates is observed: σvC13n,γ14C>σvC12n,γ13C at T9 = 0.2–1.5; σvC14n,γ15C>σvC13n,γ14C at AGB stars’ actual temperatures T9 = 0.1–0.2 and at higher values T9 ≳ 3.

Here, in order to finalize the values of isotopic ratios, it is reasonable to consider the reaction rates 12-14C(n,γ)13-15C together with the proton-induced reactions 12-14C(p,γ)13-15N calculated in the same model. We took a step forward toward this goal by calculating the MPCM rate for the 12C(p,γ)13N reaction [48].

The Tsallis statistics allow one to vary the numerical values of the 14С(n0+1)15C reaction rate, as illustrated in the present calculations for the range of the non-extensive parameter 0.7q1.3. This provides a tool for the re-estimation of astrophysical processes occurring in low-metallicity AGB stars, in particular, the production and depletion carbon isotopes as reflected in the observed 13C/14C ratio. Note that the value of the 13C/14C ratio directly affects the ratio of nitrogen isotope yields, 14N/15N. Comparing these results with studies of BBN reactions [2527], the effect of non-extensivity in the case of the 14С(n0)15C reaction is moderate—not orders of magnitude—but can produce a maximum factor of ∼1.35 increase or ∼0.8 decrease in the MB reaction rate for 0.9q1.1. One reason for this moderate effect may be that, in the case of BBN, charged particles of comparable mass are involved in the reactions.

Data availability statement

The original contributions presented in the study are included in the article/supplementary material, further inquiries can be directed to the corresponding author.

Author contributions

AT: Conceptualization, Supervision, Writing – review and editing. NB: Formal analysis, Writing – original draft. BY: Data curation, Writing – review and editing. SD: Software, Validation, Writing – review and editing.

Funding

The author(s) declare that financial support was received for the research and/or publication of this article. This work was supported by the Ministry of Science and Higher Education of the Republic of Kazakhstan (Grant No. AP19676483).

Conflict of interest

The authors declare that the research was conducted in the absence of any commercial or financial relationships that could be construed as a potential conflict of interest.

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The author(s) declare that no Generative AI was used in the creation of this manuscript.

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Keywords: n14C system, radiative capture, thermonuclear reaction rate, potential cluster model, Tsallis statistics

Citation: Tkachenko AS, Burkova NA, Yeleusheva BM and Dubovichenko SB (2025) Estimation of the effect of Tsallis non-extensive statistics on the 14C(n,γ)15C reaction rate. Front. Phys. 13:1688864. doi: 10.3389/fphy.2025.1688864

Received: 19 August 2025; Accepted: 30 September 2025;
Published: 25 November 2025.

Edited by:

Chong Qi, Royal Institute of Technology, Sweden

Reviewed by:

Danyang Pang, Beihang University, China
Ruirui Xu, China Institute of Atomic Energy, China

Copyright © 2025 Tkachenko, Burkova, Yeleusheva and Dubovichenko. This is an open-access article distributed under the terms of the Creative Commons Attribution License (CC BY). The use, distribution or reproduction in other forums is permitted, provided the original author(s) and the copyright owner(s) are credited and that the original publication in this journal is cited, in accordance with accepted academic practice. No use, distribution or reproduction is permitted which does not comply with these terms.

*Correspondence: A. S. Tkachenko, dGthY2hlbmtvLmFsZXNzeWFAZ21haWwuY29t

ORCID: A.S. Tkachenko, orcid.org/0000-0002-9319-0135; N.A. Burkova, orcid.org/0000-0002-3122-1944; B.M. Yeleusheva, orcid.org/0000-0002-8739-1969; S.B. Dubovichenko, orcid.org/0000-0002-7747-3426

Disclaimer: All claims expressed in this article are solely those of the authors and do not necessarily represent those of their affiliated organizations, or those of the publisher, the editors and the reviewers. Any product that may be evaluated in this article or claim that may be made by its manufacturer is not guaranteed or endorsed by the publisher.