ORIGINAL RESEARCH article

Front. Phys., 07 May 2024

Sec. Optics and Photonics

Volume 12 - 2024 | https://doi.org/10.3389/fphy.2024.1381156

Design, fabrication, and test of bi-functional metalenses for the spin-dependent OAM shift of optical vortices

  • 1. Department of Physics and Astronomy “G. Galilei”, University of Padova, Padova, Italy

  • 2. Padua Quantum Technologies Research Center, University of Padova, Padova, Italy

  • 3. Department of Information Engineering, University of Padova, Padova, Italy

  • 4. CNR-IOM Istituto Officina dei Materiali, Trieste, Italy

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Abstract

The ability to encode different operations into a single miniaturized optical device is required to reduce the complexity and size of optical paths for light manipulation, which usually employs dynamic optical components, interferometric setups, and/or multiple bulky elements in cascade. A very efficient solution is provided by metalenses, which are flat optical elements able to generate and manipulate structured light beams in a compact and efficient way, offering a powerful and attractive tool in many fields, such as life science and telecommunications. In this work, we present the design and test of transmission dielectric bi-functional metalenses that exploit both the dynamic and the geometric phases, to enable the spin-controlled manipulation of different focused orbital angular momentum (OAM) beams, depending on the circularly polarized state in input. In detail, we provide numerical algorithms for the design and simulation of the meta-optics in the telecom infrared, the fabrication processes, and the optical characterization under different impinging polarized optical vortices. This solution provides new integrated flat optics for applications in imaging, optical tweezing and trapping, optical computation, and high-capacity telecommunication and encryption.

1 Introduction

Allen and co-workers’ seminal paper [1] paved the way for the research field of structured light, leading to scientific milestones and innovative applications in many areas, such as life science, information and communication technology, and quantum technologies [24]. In particular, wavefields carrying orbital angular momentum (OAM), so-called OAM beams or optical vortices (OVs), are endowed with peculiar ring-like intensity distributions and twisted wavefronts which revealed powerful applications in high-resolution microscopy [5], optical micro-manipulation [68], security [9], and light-matter interaction [10], while offering a new degree of freedom to encode information both in classical [11, 12] and single-photon regimes [1315].

Spiral phase plates (SPPs) [16] represent one of the first stable, efficient, and compact optical elements proposed to generate structured light carrying orbital angular momentum from ordinary non-structured beams. These optics have 3D staircase profiles resembling the twisted wavefront imparted to the impinging beam [17]. It is possible to generate high-purity and multi-ring OAM beams using SPPs with both azimuthal and radial discontinuities, to enable the excitation of higher-order modes by exploiting high-resolution lithographic techniques [1820]. Nevertheless, spiral phase plates are limited to a single functionality. The advent of metasurfaces promoted the evolution of SPPs into the so-called q-plates [21] acting on the geometric phase to impart a polarization-dependent beam shaping [21]. Rather than shaping the wavefront by changing the local thickness of an isotropic material, i.e., the dynamic phase, in q-plates the thickness is fixed while the phase is manipulated by controlling the local anisotropy of the effective material. In particular, the imparted phase is equal to twice the local orientation of the extraordinary axis, and the sign is dependent on the handedness of the circular polarization in input. The first solutions relied on controlling the inherent anisotropy of liquid crystals [2123], then artificial anisotropy was introduced by using properly oriented digital gratings [24, 25] or dielectric resonators [26, 27], so-called metaunits, to induce an effective form of birefringence. Metasurfaces represented a revolution in optics. Moving from 3D sculptured optics to 2D flat digital meta-optics exploiting silicon manufacturing has enabled the merging of optics and silicon photonics [28, 29]. Furthermore, the metasurface paradigm has included polarization as an additional degree of freedom for light structuring, extending the optical functionalities to enable the possibility of decoupling spin from phase reshaping and building up spin-dependent optical elements [30] [31]. One solution is offered by dual-functional metasurfaces [3235], which act locally on both the dynamic and the geometric phases. That is achieved using anisotropic nanopillars, which have different tailored shapes to act on the dynamic phase and control their local fast-axis orientation to adjust the polarization-dependent geometric phase contribution.

In this work, we present the fabrication and optical characterization of dual-functional metalenses working in the telecom infrared, specifically designed for the generation of two distinct focused OAM beams, depending on the polarization state of the impinging light. In particular, we show that by switching the input polarization handedness, it is possible to select a spin-dependent OAM shift of the desired optical vortex in input at a specific position in space. This approach improves the functionality and integration level of standard spiral phase plates and q-plates, providing new advanced optical elements for applications to high-resolution microscopy, optical micro-manipulation, and classical and quantum information.

2 Material and methods

2.1 Dual-functional metalenses design

In this work, we propose a spin-dependent dielectric metasurface made of a squared lattice (period of the lattice u = 600 nm) of birefringent metaunits (MUs), so-called metaatoms (MAs), acting both on the geometric and dynamic phases. Each metaunit is represented by a crystalline silicon (c-Si) nanofin on a c-Si substrate. The cross-section of each metaunit is chosen within a library of 13 different nanostructures with different shapes and/or orientations but the same height. In detail, as reported in our previous works [36], we find a set of rectangular-based, elliptical-based and pairs of different bevelledrectangular-based nanofins. At the same time, the height was optimized at 850 nm in order to cover the 0-2π dynamic phase range that is mandatory to satisfy the dual-functional paradigm. Since the metaunit size is below the diffraction limit, input light experiences an effective uniaxial medium with dynamic phase delays δx and δy on the two axes, referring to TM and TE linear polarizations, respectively. All the nanostructures of the library act as half-wave plates (HWP) in order to maximize the polarization conversion and, therefore, the optical efficiency [3739]. Then, a rotation by an angle θ of the anisotropic metaunit introduces a spin-dependent geometric phase equal to ± , depending on the handedness of the impinging circular polarization state, while the local dynamic phase depends on the metaunit cross-section. Thus, combining these two properties and selecting judiciously the metaunits pixel-by-pixel on the whole metasurface area, the metalens can behave differently depending on whether the input beam is right-handed (RCP) or left-handed circularly polarized (LCP).

The objective is that two circularly polarized beams with opposite handedness (i.e., RCP and LCP) experience different phase patterns and , which are related to the dynamic and geometric phase according to the constitutive relations Eqs (1)(3):

While the dynamic phase imparts the same contribution to both the RCP and LCP input beams, the geometric phase implies the transfer of symmetrical (opposite) phase delays for the two circularly polarized states, which combine to induce the desired spin-dependent phase modulation, that is:

J is the Jones matrix of the anisotropic metaatom [40, 41].

As well known, it is possible to describe a linearly polarized beam as the linear combination of a left-handed circularly polarized state () and a right-handed circularly polarized one (). Thus, by illuminating the metasurface with a linearly polarized beam, it is possible to activate simultaneously the two functionalities designed for impinging circularly polarized light.

As we are interested in generating focused OAM beams, we need to properly design the local phase delay imparted by each metaunit in order to transfer the desired topological charge and focus the optical vortex onto two distinct points in space. To this aim, we encoded a converging lens profile :

being the amount of OAM per photon (in units of ) (or topological charge) transferred to the beam, the wavevector, the focal length, and the focus coordinates on the focal plane perpendicular to the propagation axis (z) and placed at a distance [4246].

To impart two different topological charges in two distinct positions, we can rewrite Eq. (6) using the notations of Eqs 4, 5:where are the topological charges imparted to the impinging left-handed and right-handed circularly polarized beams respectively, while represent the corresponding positions of the focal planes.

2.2 FEM simulations

The library of metaatoms was extrapolated by performing numerical simulations with Finite-Element Method (FEM) in the wavelength domain (COMSOL Multiphysics®). Each subunit was modelled as a silicon nanopillar (nSi = 3.5030) surrounded by air (nAir = 1) designed on the top of a silicon substrate (nSi = 3.5030), and all the materials were considered as non-absorbing [n = Re(n), Im(n) = 0]. Among all the possible configurations, a set of 13 pillars has been selected, covering the whole 2π range of dynamic phase and satisfying the conditions of half-wave plate and equal transmissions for TE and TM polarizations. Full details regarding metaunits shape and corresponding phase delays are reported in [36]. In detail, to ensure the HWP behaviour of each meta-unit, we selected metaatoms having a maximum phase difference of 0.03 rad from the HWP condition (), concurrently, we fixed , being Tx,i and Ty,i the transmittance of the ith metaatom for TE and TM polarizations, respectively, to ensure the validity of above Eqs 4, 5. Moreover, we imposed a maximum difference of 0.1 in transmittance among the 13 different metaatoms to guarantee a homogeneous transmittance over the whole metalens. We used custom MatLab scripts to transfer the maps of dynamic and geometric phases into a GDSII file encoding the cross-sections of the meta unit in each cell of the 2D metasurface lattice with period 600 nm in the x- and y-directions. Finally, the CAD file was uploaded to the software of the electron-beam lithographic system, and the design was materialized after exposure and development on the resist layer.

2.3 Fabrication

The designed metaoptics was fabricated via a two-step fabrication procedure. High-resolution electron beam lithography (EBL) was employed to transfer the optimized computational pattern onto a resist layer. In particular, a thin PMMA resist layer, deposited on a ⟨100⟩ silicon substrate, was patterned using an EBL system (Carl Zeiss Sigma 300, 30 keV beam voltage). Subsequently, a lift-off process was executed exploiting a thin mask of Al2O3. Finally, the pattern was transferred onto the underlying silicon substrate through Inductively Coupled Plasma Reactive Ion Etching (ICP-RIE). ICP-RIE was performed in a STS Multiplex ASE using a mixture of SF6:C4F8:Ar (3:6:1). The plasma conditions and etching time were optimized in order to reach the optimal thickness and, thus, reduce the zero-order contribution [47, 48].

2.4 Optical characterization setup

The beam illuminating the metasurface was produced employing a Liquid Crystal on Silicon (LCoS) spatial light modulator (SLM) (X13267-08, Hamamatsu, pixel pitch 12.5 μm) through a technique involving both phase and amplitude modulation. Collimation of the output from a DFB laser (λ = 1310 nm, 1310LD34 1-2-2-1 CCSI, AeroDiode) at the termination of a single mode fiber was achieved using an aspheric lens with a focal length of 7.5 mm (A375TM-C, Thorlabs). The beam was then linearly polarized (LPIREA100-C, Thorlabs), expanded by a first telescope (f1 = 3.5 cm, f2 = 10.0 cm), and directed towards the display of the SLM for reshaping and/or optical vortex generation (Figure 1).

FIGURE 1

A 50:50 beam-splitter was positioned before the SLM, directing the reflected structured beam into the desired optical path and enabling an additional optical path for interferometric analysis. A 4-f system (f3 = 20.0 cm, f4 = 12.5 cm) was put in cascade with an aperture in the Fourier plane to isolate the first-order encoded mode and adjust the desired illuminating beam waist. In between, a quarter-wave plate (QWP) (WPQ10M-1310, Thorlabs) or a half-wave plate (HWP1) (WPH05M-1310, Thorlabs) were used to generate circularly polarized states from the original horizontally polarized one or rotate the polarization plane of the beam exiting the SLM, respectively. The polarized beam illuminated the meta-optics, mounted on a 6-axis kinematic mount (K6XS, Thorlabs). Finally, the OAM-shifted beam was collected using a ×10 Objective (CFI E Plan Achromat ×10, Nikon) positioned on a micrometric translator stage (LX20/M, Thorlabs). The image was captured by a CCD camera (WiDy SWIR 640U-S, pixel pitch 12.5 μm). It was possible to generate an interferometric pattern using the additional optical arm, opening the iris (D2). The microscope objective was necessary to properly extract and magnify the generated beams since the focal lengths were too short to collect the beam directly on the CCD camera.

3 Results

Exploiting the dual-functional mechanism described in the previous section, we designed a spin-decoupled metalens which imparts two different topological charges and to left-handed and right-handed circularly polarized light, and focuses the output beams at a distance of and from the optical element, respectively.

At first, we simulated the spin-decoupled behavior under the illumination of a Gaussian beam with a waist of 175 µm. To test the two different polarization-dependent responses simultaneously, we chose a linearly polarized light in input.

Figure 2 depicts, as expected, the simultaneous generation of two distinct OAM beams with the desired topological charges at 500 µm and 1000 µm. It is clear how the beam generated from the right-handed contribution has a larger waist and a lower intensity profile because it carries a higher topological charge and is focused on a plane placed at a larger distance.

FIGURE 2

Then, we simulated the behaviour of the metalens under the illumination of beams that already carry a topological charge (i.e., from −3 to 3). In particular, we modelled the impinging structured beam as a perfect vortex (PV) having a ring radius () of 125 µm and a ring width () of 50 µm, as described by the equation Eq (8):

Figure 3 presents the results we have obtained. In the first row (in blue), the phase and intensity pattern of the impinging perfect vortex are reported. The second (yellow) and third (orange) rows report the generated structured beams under LCP and RCP illumination, respectively. Due to the half-wave plate behaviour, each metaatom reverses the handedness of the impinging light as reported in Eqs 4, 5, so the OAM beam focused at 500 µm is right-handed circularly polarized. Instead, the one generated at 1,000 µm is left-handed circularly polarized. As expected, we can see that the metalens acts as a dual-functional shifter of topological charge. In fact, the resulting generated beam carries a topological charge equal to the sum of the topological charge of the illuminating beam with the spin-dependent topological charge imparted by the metalens. Moreover, the generated beams increase their waist with the resulting topological charge. As a matter of fact, in the far-field we collect the Fourier transform of a perfect vortex, which is well described by a Bessel-Gaussian beam. With respect to perfect vortices, the intensity profile of those beams is not OAM-independent, thus the radius of the inner intensity rings increases with the carried topological charge.

FIGURE 3

Subsequently, we numerically estimated the purity of the generated OAM modes by analyzing the OAM spectrum of the generated beam at the focal plane using the expression Eq (9) [49]:where .

In Figure 4, we report the OAM spectrum analysis of the output beams under the illumination conditions mentioned above. The OAM shift of the output beams with respect to the input one confirms what expected from the metalens design. The generated OAM beams show no significative presence of spurious terms for the two outgoing circularly polarized beams. The spurious contributions are lower than 0.05 for all the different impinging configurations, proving that the conversion efficiency is very high.

FIGURE 4

Then, we fabricated the metasurface with a radius of 400 µm using the procedure described in Section 2.3.

Figure 5 displays several SEM images of the fabricated silicon metasurface.

FIGURE 5

Finally, we optically characterized the performances of the designed metalens using the optical setup reported in Section 2.4. As expected, the two output beams present an intensity pattern that varies depending on the impinging perfect vortex, suggesting an increase of the output orbital angular momentum, because of the interaction with the metalens (Figure 6B). To confirm this, we measured the interferogram pattern, which gave us information on the carried phase. It is clearly visible that the number of arms of the spiral, indicating the topological charge carried by the beam, are dictated by the sum of the impinging OAM plus the charge imparted by the metalens, which depends on the polarization state (Figure 6A).

FIGURE 6

4 Discussion and conclusion

This work presents the design, fabrication, and test of dual-functional silicon metalenses for the polarization-controlled manipulation of OAM beams. The optical element was designed to properly generate different non-overlapping focused beams carrying orbital angular momentum depending on the polarization state of the illuminating light. This optical behaviour is achieved by exploiting the dual-functional metalens capability to act on the dynamic and geometric phases simultaneously in order to introduce spin-dependent phase delays. The metaoptics has been fabricated using a two-step process: lithography of a resist mask with EBL and subsequent pattern transfer into the silicon substrate using ICP-RIE. Finally, we have characterized the optical response of the fabricated metalens to prove the effective polarization-dependent device as a topological charge shifter. The experimental results agree with the simulations, proving the design quality and the fabrication protocols optimization. While in this paper we present the generation of OAM beam, the method can be extended to the design of any metaoptics aimed to impart given phase patterns with high dimensionality or complex symmetry [50] to the different impinging circularly polarized states of light. In particular, we generated a single wavelength library, but by selecting more complicated coupled resonant metaunits, it is possible to achieve full achromaticity [51, 52]. Dual-functionality represents a tool that boosts the optical operations of previous optical devices, such as diffractive elements or metasurfaces acting only on geometric or dynamic phases. This attractive solution can inspire advanced applications in imaging, microscopy, particle manipulation, and quantum technologies, wherever tiny and compact multi-functional optical devices, fabricated using silicon technology manufacturing, are required.

Statements

Data availability statement

The raw data supporting the conclusion of this article will be made available by the authors, with under reasonable request.

Author contributions

AV: Conceptualization, Methodology, Software, Writing–original draft, Writing–review and editing. DB: Methodology, Writing–original draft, Writing–review and editing. SD: Methodology, Writing–original draft, Writing–review and editing. FR: Funding acquisition, Supervision, Writing–original draft, Writing–review and editing. GR: Funding acquisition, Supervision, Writing–original draft, Writing–review and editing, Methodology, Software.

Funding

The author(s) declare that financial support was received for the research, authorship, and/or publication of this article. This work was supported by the project STRADA (Italian Presidency of the Council of Ministers) and also partially supported by the European Union under the Italian National Recovery and Resilience Plan (NRRP) of NextGenerationEU, partnership on “Telecommunications of the Future” (PE0000001–program “RESTART”).

Conflict of interest

The authors declare that the research was conducted in the absence of any commercial or financial relationships that could be construed as a potential conflict of interest.

Publisher’s note

All claims expressed in this article are solely those of the authors and do not necessarily represent those of their affiliated organizations, or those of the publisher, the editors and the reviewers. Any product that may be evaluated in this article, or claim that may be made by its manufacturer, is not guaranteed or endorsed by the publisher.

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Summary

Keywords

metalens, meta-optics, flat optics, orbital angular momentum, structured light

Citation

Vogliardi A, Bonaldo D, Dal Zilio S, Romanato F and Ruffato G (2024) Design, fabrication, and test of bi-functional metalenses for the spin-dependent OAM shift of optical vortices. Front. Phys. 12:1381156. doi: 10.3389/fphy.2024.1381156

Received

02 February 2024

Accepted

04 April 2024

Published

07 May 2024

Volume

12 - 2024

Edited by

Bertrand Kibler, UMR6303 Laboratoire Interdisciplinaire Carnot de Bourgogne (ICB), France

Reviewed by

Vin-Cent Su, National United University, Taiwan

Yijie Shen, Nanyang Technological University, Singapore

Updates

Copyright

*Correspondence: Gianluca Ruffato,

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