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REVIEW article

Front. Mater.

Sec. Carbon-Based Materials

Volume 12 - 2025 | doi: 10.3389/fmats.2025.1639589

Research Advances in Carbon-Based Electrode Materials for Electrosorptive Separation of Uranium from Aqueous Solutions

Provisionally accepted
Ling  TangLing Tang1Tao  WeiTao Wei1Yanfeng  WeiYanfeng Wei1Yin  YuYin Yu2*
  • 1China University of Petroleum Beijing at Karamay, Karamay, China
  • 2Xinjiang Academy of Environmental Protection Science, Urumqi, China

The final, formatted version of the article will be published soon.

Electrosorptive removal of uranium from aqueous solutions has emerged as an auspicious approach for mitigating radioactive pollution, with carbon-based materials serving as pivotal electrode components due to their exceptional conductivity, tunable surface chemistry, and structural versatility. This review thoroughly examines recent progress in carbon-based capacitive deionization (CDI) electrodes for U(VI) removal and systematically assesses critical modification approaches, including heteroatom doping, functional group modification, and metal oxide loading. Each strategy is critically examined regarding its underlying mechanism, material design principles, and influence on uranium adsorption capacity and selectivity. A particular emphasis is placed on synergistic effects from combined modification approaches, which consistently outperform single-component systems. Bridging insights from environmental science and energy storage technologies, this work proposes an integrated optimization framework that establishes fundamental structure-performance relationships for CDI electrodes. By systematically synthesizing current research progress while identifying key knowledge gaps, this review offers strategic guidance for the rational design of next-generation carbon-based materials to enable efficient, selective, and sustainable radioactive wastewater remediation.

Keywords: Uranium, Electrosorption, Carbon-based electrodes, Water treatment, Electrode modification

Received: 04 Jun 2025; Accepted: 18 Jul 2025.

Copyright: © 2025 Tang, Wei, Wei and Yu. This is an open-access article distributed under the terms of the Creative Commons Attribution License (CC BY). The use, distribution or reproduction in other forums is permitted, provided the original author(s) or licensor are credited and that the original publication in this journal is cited, in accordance with accepted academic practice. No use, distribution or reproduction is permitted which does not comply with these terms.

* Correspondence: Yin Yu, Xinjiang Academy of Environmental Protection Science, Urumqi, China

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