Abstract
The nuclear ground state properties of 63Co and 63Ni nuclei have been investigated within the framework of the relativistic mean field (RMF) approach. The RMF model with density-dependent meson-exchange (DD-ME2) interaction is used to calculate the potential energy curves (PECs) and nuclear ground state deformation parameters of 63Co and 63Ni. The blocking effects of the unpaired nucleon are considered using the equal filling approach for the odd-A system. Later, the -decay properties, including the stellar weak rates and Gamow–Teller (GT) strength of 63Co and 63Ni, are studied using the proton-neutron quasiparticle random-phase approximation (pn-QRPA) model. The values computed from the RMF model are employed in the pn-QRPA framework as an input parameter for the calculations of -decay properties for 63Co and 63Ni. The stellar rates are compared with the projected shell model (PSM) results. For all densities, the pn-QRPA rates are found to be higher than the stellar rates computed via the PSM to a factor of 1.3 or more. The findings reported in the present investigation might be useful for simulating the late-stage stellar evolution of massive stars and the -process of nucleosynthesis.
1 Introduction
The rapid neutron-capture process (-process) is the primary nucleosynthesis mechanism responsible for the production of nuclei more massive than iron [1, 2]. The -process often occurs in a stellar exploding scenario with a high neutron density flux. It was noted that at the same astrophysical parameters of constant density and temperature, it is not possible to synthesize all of the nuclear matter simultaneously [3, 4]. Hence, neutron capture proceeds far more quickly than competing beta decay. The larger neutron-flux matter, which has comparably little and roughly constant (neutron separation energy), is followed by the -process route. The -process flow of matter slows at neutron magic shell isotones. The trajectory of the -process and the abundance distribution are significantly influenced by the half-life predictions.
The Gamow–Teller (GT) transition is widely believed to contribute to the stellar rates [5]. GT distributions have been produced experimentally using various approaches [6, 7]. The GT strength may be measured by charge-exchange reactions for nuclei in or close to the beta stability valley under terrestrial conditions when the parent nuclei stay in their ground states [8]. Several nuclei located beyond the beta stability valley play a crucial role in various astrophysical processes, including the -process, the -process, and neutron star cooling. In extremely hot and dense stellar scenarios, nuclei may become thermally populated in their excited states. Existing study techniques are still insufficient to conduct a thorough investigation into the GT strength of nuclei beyond the beta stability valley or when the parent nuclei exist in their excited states.
Weak interactions between finite nuclei hold significance in various disciplines, including particle physics and nuclear astrophysics [9–11]. Reliable weak-interaction rates of finite nuclei in high temperatures and high-densities stellar scenarios are crucial for understanding astrophysical challenges like stellar advancement and the origins of heavy elements. There are three different sorts of implications from stellar weak-interaction processes: converting neutrons to protons, reducing the density of positrons or electrons inside the stellar environment, and neutrino emissions [12–17]. Understanding the core-collapse supernova is therefore dependent on the stellar weak rates [18], the -process (slow neutron-capture process) [19, 20], the -process (rapid neutron-capture process) [21], and the process (rapid proton-capture process) [22].
The GT strength and the weak-interaction rates have been studied theoretically using a variety of nuclear structure models that have been developed over the past few decades. Fuller, Fowler, and Newman (FFN) accomplished groundbreaking work for the systematic calculation of nuclear stellar weak-interaction rates [12–14]. For the analysis of GT transition and stellar weak-interaction rate, the most dependable approach in current practice is the shell model (SM), which has a full diagonalization of an effective Hamiltonian in a selected model space [23]. Additional methods are anticipated for the GT strength and stellar weak rates in applications, such as the hybrid model based on the shell model Monte Carlo approach and the random-phase approximation (RPA) [24], the quasiparticle random-phase approximation (QRPA) [25], and the most recent traditional projected shell model (PSM) [26, 27].
Massive stars have an onion-like structure prior to the supernova stage, where the Fe, Co, and Ni mass-region nuclei play crucial roles in the core. Depending on neutron excess, nuclear beta decays and electron captures compete before the core collapses [28]. However, it is anticipated that most heavy nuclei close to or inside the beta stability valley originated from the -process. 63Ni is a potential candidate for the -process and similarly, 63Co is a potential candidate in the pre-supernova collapse stage.
In the present work, we employed the RMF approach with density-dependent meson-exchange interactions to examine the nuclear ground state properties, including the binding energies and related to = 63 (63Co and 63Ni). We analyzed the potential energy curves (PECs) that are important for the extraction of . For the analysis of GT strength and stellar weak rates of 63Co and 63Ni, we utilized the pn-QRPA approach. We revised the calculations based on our present recipes to investigate beta decay properties. For example, our first aim is to extract the ground state deformation parameter from the minima of relative energy curves computed via the RMF framework. Then, we will check the potential effects of on the GT strength distributions and stellar weak rates for 63Co and 63Ni. The present model-based analysis is compared with previously observed and predicted data.
The paper is organized as follows. In Section 2, we provide a brief explanation of the RMF and pn-QRPA models used to calculate the nuclear structure and -decay properties, respectively. Section 3 presents our results with relevant discussion. Section 4 concludes the findings of the current investigation.
2 Theoretical framework
2.1 The RMF model
The RMF model is a theoretical tool used for the description of nuclear structure properties of nuclei (see [29] and related references). The preliminary model [30] struggled to describe nuclear surface features and the incompressibility of nuclear matter. To address this, a nonlinear model was developed [29]. The later versions of the model were termed covariant density functional theory and included a density-dependent meson-exchange model [31]. In the present investigation, the ground state parameters for nuclei have been determined by employing the density-dependent meson-exchange (DD-ME2) [32] version of the RMF framework. According to the RMF model, nucleons interact by exchanging various mesons and photons [30]. The first version of the RMF model ran into several issues while attempting to describe the incompressibility of nuclear matter and the surface characteristics of nuclei. This led to the introduction of the model’s nonlinear variant [29]. Subsequent versions of the RMF framework, known as covariant density functional theory, developed with elements including point coupling (PC) and meson-exchange (ME) [31, 33, 34]. We utilized the density-dependent -(ME) framework in our analysis. The density-dependent meson-exchange variant of the RMF model considers the isoscalar scalar meson, the isoscalar vector meson, and the isovector vector meson fields for the analysis of nuclear matter and single-particle nuclear properties. In the DD-ME model, the coupling constants are self-consistently governed by nuclear functions. The definition of the Lagrangian density is given below.In Equation 1, the terms , , and depend on the (nucleon) density, which is further defined by Equation 2:where i is generalized for the , , and , respectively. Similarly, is the ratio of (density of baryon), and (density of baryon at saturation). is defined for the or meson by Equation 3:whereas for the meson, is defined by Equation 4:The DD-ME2 interactions ([35–38]) are often employed as covariant density functionals in the DD-ME model.
Studying even-even systems within the mean field approach is a good approximation. In this case, the configurations, neglected above the mean field ground state, are 4- or higher-quasiparticle (qp) configurations. The 2-qp configurations do not couple to the Hamiltonian . Mixing configurations are relatively few and separated by the pairing gaps. The exact solution has only a small admixture of higher qp configurations (4-qp and higher). On the other hand, investigating odd-A nuclei using the RMF model is rather challenging. In this case, there are many 3-qp states in the region close to the ground state, which may mix. The pairing gap even increases the level density of neighboring 1-qp states. Only a few of the matrix elements vanish. The mean field approximation in odd-A cases is not as good as in even-even nuclei. Of course, sometimes symmetries help (-value in deformed nuclei), but this is not always the case. We performed the HFB calculations in odd-A systems by using the blocking technique. The blocking was carried out by replacing one -vector with the corresponding -vector (see Section 6.3.2 of [39]). We carried out the blocking calculations with small modifications of the HFB code [40]. Pairing correlations play an important role for open-shell nuclei, and the Bardeen–Cooper–Schrieffer (BCS) approximation was used to tackle these correlations. Furthermore, constant G approximation [41] was used for the PEC calculations.
2.2 The pn-QRPA model
The pn-QRPA model is employed to analyze GT strength distributions and stellar weak rates. The Hamiltonian configuration in the pn-QRPA model may be characterized using Equation 5:The Hamiltonian for a single particle is denoted as , while represents the interaction between nucleons. The terms and correspond to interactions involving particle-particle and particle-hole GT interactions, respectively. Wave functions and energies of individual particles are calculated via the Nilsson model [42]. The oscillator constant is determined using . Other crucial factors affecting weak-interaction rates consist of , the nucleon pairing gap , parameters of the Nilsson potential (PNP), and the -values. The PNP parameters were sourced from [43], and -values were derived through the calculation of mass excess values as presented in the compilation [44]. In order to obtain proton and neutron quasiparticle energies and occupation probabilities, the BCS equations were solved with pairing gaps computed using Equations 6, 7:where () is the separation energy of protons and neutrons, respectively. As mentioned earlier, the values were determined using the RMF model. is determined by using Equation 8:where denotes the electric quadrupole moment chosen from [45] or the RMF framework. In the pn-QRPA model, the charge-changing reaction transitions are defined by phonon creation operators. The pn-QRPA phonons are given as Equation 9:Here, the summation is taken on all the p-n pairs having = − = 0, 1, and () represents the angular momentum third component of the neutron (proton). The operators signify the creation of a quasiparticle (q.p) state for either a neutron or a proton, and represents the time-reversed state of p. In the context of QRPA phonons, the theory defines the ground state as the vacuum, symbolized by = 0. The phonon operator’s excitation energy and amplitudes () are acquired by solving Equation 10, which is the well-known RPA equation.Here, X(Y) represent forward (backward) amplitudes. The shows the energy eigenvalues of the eigenfunctions, and the two sub-matrices are specified by Equations 11, 12:Here, the shows the q.p energies of the neutron (proton), whereas and represent the occupation and unoccupation amplitudes and are treated in the BCS theory. The detailed solution of the RPA matrix equation can be seen in [46]. The pairing force is calculated using the BCS approximation. These calculations were performed separately for both proton and neutron. We took a constant pairing force of strength ( and for protons and neutrons, respectively),where is orbital angular momentum, and summation over and is restricted to positive values. The proton-neutron residual interactions take place through the pp and ph GT forces, which were characterized by interaction constants and , respectively, in the pn-QRPA framework. The GT force is explained using Equations 14, 15:withIn order to calculate the GT force, we used Equations 16, 17:withThe and interaction strengths were determined using the relation and , respectively, taken from [47]. Our results fulfilled the model-independent Ikeda sum rule [48]. The reduced GT transition probabilities were calculated using Equation 18:where is the spin operator, and = are the isospin raising and lowering operators, respectively. The model-independent Ikeda sum rule may be evaluated using Equation 19 for the operators:where represents the parent state, and represents the daughter state connected via the GT operator. For further details, see [49–51].
The stellar -decay (we subsequently refer to this as electron emission ) and positron capture rates between parent level and daughter state have been determined utilizing Equation 20:where corresponds to the GT and Fermi transitions shown in Equations 21–23:The construction of low-lying excited levels and computation of nuclear matrix elements in our present analysis may be found in [46]. is the phase space and depends on the core temperature , core density , and Fermi energy . It was calculated using Equation 24:for decay rates. The for were computed using Equation 25:where is the kinetic energy of the electron, and is the total capture threshold energy. The Fermi functions, , were calculated using the method described in [52]. The total decay energy was determined using Equation 26:where is the excitation energy of the daughter nucleus having mass , while is the corresponding quantities of parent nucleus with mass . The distribution functions have been determined with Equations 27, 28:where is the Boltzmann constant. The electron number density, which is related to nuclei and protons, was determined using Equation 29:Here, represents the Avogadro number, is the ratio of the electron number to the baryon number, and represents the momentum of positron/electron. The total stellar weak rates were computed using Equation 30:where , which was calculated using the Boltzmann distribution, is the occupancy probability of the parent excited states. We continued to sum the initial and final states until our rate computation reached the necessary degree of convergence.
3 Result and discussion
In the initial phase of our Investigation, we are focusing on the nuclear structure properties of 63Co and 63Ni isobars by utilizing the DD-ME2 interaction parameters within the RMF framework. The odd nuclei are considered in the present investigation utilizing the relativistic Hartree–Bogoliubov (RHB) approach. We consider the blocking effects of the unpaired nucleon, which are included in the equal filling assumption, in order to compute the odd- system. We examined the for 63Co and 63Ni in detail. To accomplish this, we analyzed the PECs for 63Co and 63Ni within the RMF framework. The constraints on the quadrupole moment are implemented in order to compute binding energy for the analysis of PECs.
In Figure 1, the PECs are expressed as a function of for 63Co and 63Ni. For the analysis of PECs, the lowest binding energy is used as a reference. The PECs are derived by analyzing the differences between the predicted binding energy for certain values and the reference binding energy for 63Co and 63Ni. Nuclear shapes are determined by the PEC minima. Prolate nuclei resulted from PEC minima located on the positive value of , whereas for the oblate shape nuclei, the PEC minima are found on the negative values of . In the present investigation, the nuclear shapes in the ground state for 63Co and 63Ni are predicted to be prolate and oblate, respectively. Furthermore, one can see that two energy minima appear on both the prolate and oblate sides of the PECs. The oblate energy minimum for 63Co is more shallow than the prolate energy minimum. Therefore, the prolate shapes have a more probable occurrence in the ground state for 63Co. The oblate minimum existed at excitation energy 0.156 MeV. Similarly, 63Ni has an oblate shape in the ground state; however, it has prolate energy minima that existed at excitation energy 0.412 MeV. In addition to these structural changes, the present analysis predicts a prolate-oblate shape coexistence with a small energy difference, as displayed in Figure 1. The phenomenon of shape coexistence is associated with the occurrence of a low-lying state arising from intruder configurations in addition to the ground state. The computed via the RMF framework, where the DD-ME2 interaction for the 63Co is 0.188, and the interaction for 63Ni is −0.264. The earlier computed for 63Co was 0.108 and for 63Ni was 0.107 [45]. They predicted a prolate shape for both nuclei. Similarly, on the website [53], the information related to the PEC is displayed graphically, where 63Co has a prolate shape, and 63Ni has an oblate shape.
FIGURE 1
The nuclear deformations computed via the RMF model are used as an input parameter in the pn-QRPA model to perform self-consistent calculations of the -decay properties, including the GT strength and stellar rates of 63Co and 63Ni.
At higher temperatures and densities, 63Co is one of the most important candidates in the core collapse of a massive star. Figure 2 depicts the present model-based computed GT strength along with the measured GT strength [54] and previously computed GT strength based on PSM [27] within the -window. It is obvious from Figure 2 that the present computed GT strength agrees well with the results of [54]. The pn-QRPA calculation based on the RMF interactions predicted the strength distribution better than [27]. The splitting of the GT strength into a strong and weak state close to 2.0 MeV fits well with the experimental results. We observe that the present scheme seems able to predict effects due to the fine nuclear structure.
FIGURE 2
The temperature conditions in the stellar environment are so high (in order of K) that parent nuclei in excited states have high likelihood of occupancy. This means that the contributions of each excited state to the total weak rates are quantifiable. Consequently, all partial decay rates resulting from distinct parent excited states must be included in the analysis of the microscopic rate. This state-by-state analysis of weak rates is the foundation of the pn-QRPA model. The pn-QRPA model was initially used to determine microscopic weak-interaction rates for a large number of nuclei far from the stability line. The pn-QRPA technique utilizes a mean field basis and potentials, including the Woods–Saxon potential, the Nilsson potential, and the finite-range droplet model. Here, we investigated the rates of 63Co 63Ni at = g . At high temperatures, the various excited states of the daughter nucleus have a sizeable impact that could additionally contribute to stellar weak decay rates. It is obvious from Figure 3 that at lower densities and high temperatures, the rates are maximum. The present pn-QRPA-based analysis provides larger decay rates than the PSM and smaller decay rates than the results mentioned in [5]. For example, at = g and = 10, the present model-based rates are higher by a factor 1.3 than PSM. Meanwhile, at the same temperature and density, the rates of [5] exceeded the pn-QRPA rates by a factor of 4. Almost the same behavior is followed at = g and = 10. At higher density = g , the pn-QRPA rates almost collapse with the PSM and [5] computed rates as mentioned in Figure 3. The GT strength has a dominant impact on the stellar beta decay rates.Furthermore, we analyzed the stellar rates for 63Ni 63Cu in the -process environments at = g and 1. The present model-based results for rates, along with the predictions of PSM [27], are depicted in Figure 4. We found that at 1, the present pn-QRPA based predictions for rates at all densities ( = g ) show good agreement with the rates computed via PSM in [27]. One should note that the stellar weak rates computed at lower temperatures are considerably smaller than rates computed at higher temperatures. The primary factor contributing to the decay rates at low temperatures is the transition between ground states. As the temperature increases, the stellar population probability of the parent nucleus (63Ni) in the ground state decreases while the excited state increases, leading to an increase in the decay rates with the temperature. The stellar weak-interaction rates for both nuclei, that is, 63Co and 63Ni, have been computed within a complete microscopic fashion without assuming the Brink–Axel hypothesis for the analysis of GT strength in the excited states. The small difference is attributed to the usage of the Brink–Axel hypothesis and the incorporation of the quenching factor in the shell model calculation.
FIGURE 3
FIGURE 4
4 Conclusion
The RMF model has been utilized to analyze the nuclear structural properties, including PECs and deformation parameters for 63Co and 63Ni. The analysis was performed using the DD-ME2 interaction under the blocking technique. The RMF-based analysis predicted an oblate shape for 63Co and a prolate shape for the 63Ni in their ground states. The values computed via the RMF framework are later utilized as input parameters in the pn-QRPA model to perform the analysis of the GT strength and stellar weak rates. The calculated GT distributions were found to be in reasonable agreement with the measured data. The stellar weak-interaction rates for 63Co and 63Ni have been computed within a complete microscopic fashion without assuming the Brink–Axel hypothesis for the analysis of GT strength in the excited states. The pn-QRPA-based computed weak rates have been compared with the previously shell model-based computed rates. The reported weak rates are larger than the previous calculations by as much as a factor of 4. The difference is attributed to the usage of the Brink–Axel hypothesis and the incorporation of the quenching factor in the shell model calculation. The reported stellar rates could prove useful for -process nucleosynthesis calculations and simulations of late-time stellar evolution.
Statements
Data availability statement
The raw data supporting the conclusions of this article will be made available by the authors, without undue reservation.
Author contributions
AK: conceptualization, investigation, software, supervision, writing–original draft, and writing–review and editing. J-UN: investigation and writing–original draft. HA: funding acquisition, project administration, software, and writing–review and editing. IA: data curation and writing–review and editing. N-UR: investigation and writing–review and editing.
Funding
The author(s) declare that financial support was received for the research, authorship, and/or publication of this article. This research was funded by Taif University, Saudi Arabia, Project No. TU-DSPP-2024-33.
Acknowledgments
The authors extend their appreciation to Taif University, Saudi Arabia, for supporting this work through project number (TU-DSPP-2024-33). Jameel-Un Nabi would like to acknowledge the support of Higher Education Commission Pakistan through the project number 20-15394/NRPU/R&D/HEC/2021.
Conflict of interest
The authors declare that the research was conducted in the absence of any commercial or financial relationships that could be construed as a potential conflict of interest.
Publisher’s note
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Summary
Keywords
pn-QRPA, β-decay properties, GT strength distribution, deformation parameter, RMF model, stellar rates
Citation
Kabir A, Nabi J-U, Almujibah H, Anwaar I and Raza N-UA (2025) Re-examining the impact of 63Co and 63Ni in the stellar environment. Front. Phys. 13:1484460. doi: 10.3389/fphy.2025.1484460
Received
21 August 2024
Accepted
08 January 2025
Published
10 March 2025
Volume
13 - 2025
Edited by
Ignazio Bombaci, University of Pisa, Italy
Reviewed by
Andres Arazi, National Atomic Energy Commission, Argentina
Shashi K. Dhiman, Himachal Pradesh University, India
Parada Tobel Paraduan Hutauruk, Pukyong National University, Republic of Korea
Updates
Copyright
© 2025 Kabir, Nabi, Almujibah, Anwaar and Raza.
This is an open-access article distributed under the terms of the Creative Commons Attribution License (CC BY). The use, distribution or reproduction in other forums is permitted, provided the original author(s) and the copyright owner(s) are credited and that the original publication in this journal is cited, in accordance with accepted academic practice. No use, distribution or reproduction is permitted which does not comply with these terms.
*Correspondence: Abdul Kabir, kabirkhanak1@gmail.com
Disclaimer
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